We analyze the effects of the environment on the spin tunneling process of paramagnetic and superparamagnetic particles and conclude that the “bare” macroscopic tunneling rate is hardly affected in such case, but other more effective processes come up to change the magnetization state of the particle. We measure the degree of coherence loss by the linear entropy which will account for all correlations present in the process. We conclude that for both paramagnetic and superparamagnetic particles, the decoherence time scale is extremely short (~10 -8 ... -16 s), indicating that coherent tunneling should be strongly suppressed in favor of incoherent tunneling, i.e., the population of higher levels with subsequent decay. Interestingly enough, the ground state tunneling rate is hardly affected by such dissipative mechanisms. However other processes immediately give rise to new (incoherent) possibilities of crossing the barrier.
We analyze the effects of the environment on the spin tunneling process of paramagnetic and superparamagnetic particles and conclude that the “bare” macroscopic tunneling rate is hardly affected in such case, but other more effective processes come up to change the magnetization state of the particle. We measure the degree of coherence loss by the linear entropy which will account for all correlations present in the process. We conclude that for both paramagnetic and superparamagnetic particles, the decoherence time scale is extremely short (~10 -8 ... -16 s), indicating that coherent tunneling should be strongly suppressed in favor of incoherent tunneling, i.e., the population of higher levels with subsequent decay. Interestingly enough, the ground state tunneling rate is hardly affected by such dissipative mechanisms. However other processes immediately give rise to new (incoherent) possibilities of crossing the barrier.
The tunneling probability for a system modelling macroscopic quantum tunneling is computed. We consider an open quantum system with one degree of freedom consisting of a particle trapped in a cubic potential interacting with an environment characterized by a dissipative and a diffusion parameter. A representation based on the energy eigenfunctions of the isolated system, i. e. the system uncoupled to the environment, is used to write the dynamical master equation for the reduced Wigner function of the open quantum system. This equation becomes very simple in that representation. The use of the WKB approximation for the eigenfunctions suggests an approximation which allows an analytic computation of the tunneling rate, in this real time formalism, when the system is initially trapped in the false ground state. We find that the decoherence produced by the environment suppresses tunneling in agreement with results in other macroscopic quantum systems with different potentials. We confront our analytical predictions with an experiment where the escape rate from the zero voltage state was measured for a current-biased Josephson junction shunted with a resistor.
We investigate numerically the tunneling effect under influence of another particle in a double well system. Such influence from only one degree of freedom makes decoherence and quantum-classical transition, i.e., suppression of the tunneling effect. The decoherence happens even for cases that the influence is from a particle of very small mass, and it has virtually no effect in the corresponding classical dynamics. There are cases similar to dynamical localization that the suppressed tunneling rate is several times smaller than the classical counterpart. This result is relevant for understanding quantitatively the dynamical process of decoherence and quantum to classical transition.
Quantum tunneling remains unexplored in many regimes of many-body quantum physics, including the effect of quantum phase transitions on tunneling dynamics. In general, the quantum phase is a statement about the ground state and has no relation to far-from-equilibrium dynamics. Although tunneling is a highly dynamical process involving many excited states, we find that the quantum phase of the Bose-Hubbard model determines phase-dependent tunneling outcomes for the quantum tunneling escape, or quasi-bound problem. Superfluid and Mott insulator correlations lead to a new quantum tunneling rate, the quantum fluctuation rate. This rate shows surprising and highly dynamical features, such as oscillatory interference between trapped and escaped atoms and a completely different macroscopic quantum tunneling behavior for superfluid and Mott insulator phases. In the superfluid phase we find that escape dynamics are wave-like and coherent, leading to interference patterns in the density with a rapid decay process which is non-exponential. Quantum entropy production peaks when about half the atoms have escaped. In the Mott phase, despite stronger repulsive interactions, tunneling is significantly slowed by the presence of a Mott gap, creating an effective extra barrier to overcome. Only one atom can tunnel at a time, yet the decay process is nearly linear, completely defying the single-particle exponential model. Moreover, quantum entropy peaks when only about one quarter of the atoms have escaped. These and many other such effects go beyond the usual notions of single-particle quantum tunneling, quantum statistical effects on tunneling, and well-known semi-classical approaches from WKB to instanton theory. These results thus open up a new regime of exploration of far-from-equilibrium dynamics for quantum simulators and quantum dynamics.
For the realistic theoretical descriptions of quantum devices, we have to take the unavoidable coupling to their surrounding environment into account. A lot of effort in theoretical physics has been made to describe decoherence effects and the corresponding quantum to classical transition in the past. In these studies, baths are coupled to certain observables making their behavior more classical. In the most general case, a quantum device is affected by environments coupled to different observables. In this thesis, we study the differences emerging from coupling the bath to different observables. In particular, we investigate the situation, where two baths are coupled simultaneously to two conjugate variables (e.g. xˆ and pˆ, denoted dissipative frustration). We study how the interplay of these two baths can lead to interesting effects. After an introduction of the topic, we discuss the results of this thesis in Part II and Part III. In Part II, we study the effect of quantum tunneling in presence of a dissipative interaction with two Ohmic environments to the position xˆ and/or to the momentum pˆ of a particle. In chapter 2, we consider a symmetric double well potential which is important in the context of coherent state preparation, as its ground state is a superposition of being in the left and in the right well. Using the semiclassical approximation to calculate instanton paths within the path integral method, we find that momentum dissipation enhances the coherent tunnel splitting. In presence of dissipative couplings to xˆ and pˆ, the momentum dissipation acts in favor of the delocalization of the particle shifting the critical coupling strength of the dissipative phase transition induced by the position dissipation. Chapter 3 contains a study of the escape rate out of a metastable well in presence of dissipation. Here we find that the incoherent tunneling rate is exponentially enhanced in presence of momentum dissipation. We further show that the influence of momentum dissipation depends on the slope of the part of barrier the particle escaping through. In presence of both dissipative couplings, we find a non-monotonic behavior of the escape rate as a function of the dissipative couplings strengths. In Part III, we show that it is possible to realize the situation of "dissipative frustration" in Josephson junction chains. In particular, we introduce charge dissipation as a physical realization of the afore introduced momentum coupling. After presenting the circuit elements needed for charge dissipation, we study a chain of Josephson junctions affected by Ohmic baths coupled to the charge and/or the phase. Using a self-consistent harmonic approximation, we determine the phase diagram at zero temperature which exhibits a quantum phase transition between an ordered phase, corresponding to the superconducting state, and a disordered phase, corresponding to the insulating state with localized superconducting charge. Interestingly, we find that the critical line separating the two phases has a non-monotonic behavior as a function of the dissipative coupling strength. Moreover, within the self-consistent harmonic approximation, we analyze the dissipation induced crossover between a first and second order phase transition, showing that dissipative frustration increases the range in which the phase transition is second order. The non-monotonic behavior is also reflected in the purity of the system that quantifies the degree of correlation between the system and the environment, and in the logarithmic negativity as an entanglement measure that encodes the internal quantum correlations in the chain.
Abstract This work proposes a series of quantum experiments that can, at least in principle, allow for examining microscopic mechanisms associated with decoherence. These experiments can be interpreted as a quantum-mechanical version of non-equilibrium mixing between two volumes separated by a thin interface. One of the principal goals of such experiments is in identifying non-equilibrium conditions when time-symmetric laws give way to time-directional, irreversible processes, which are represented by decoherence at the quantum level. The rate of decoherence is suggested to be examined indirectly, with minimal intrusions—this can be achieved by measuring tunnelling rates that, in turn, are affected by decoherence. Decoherence is understood here as a general process that does not involve any significant exchanges of energy and governed by a particular class of the Kraus operators. The present work analyses different regimes of tunnelling in the presence of decoherence and obtains formulae that link the corresponding rates of tunnelling and decoherence under different conditions. It is shown that the effects on tunnelling of intrinsic decoherence and of decoherence due to unitary interactions with the environment are similar but not the same and can be distinguished in experiments.
The quantum dynamics of mesoscopic or macroscopic systems is always complicated by their coupling to many `environmental' modes. At low T these environmental effects are dominated by localized modes, such as nuclear and paramagnetic spins, and defects (which also dominate the entropy and specific heat). This environment, at low energies, maps onto a `spin bath' model. This contrasts with `oscillator bath' models (originated by Feynman and Vernon) which describe delocalized environmental modes such as electrons, phonons, photons, magnons, etc. The couplings to N spin bath modes are independent of N (rather than the ~O(1/( N ) 1/2 ) dependence typical of oscillator baths), and often strong. One cannot in general map a spin bath to an oscillator bath (or vice versa); they constitute distinct `universality classes' of quantum environment. We show how the mapping to spin bath models is made, and then discuss several examples in detail, including moving particles, magnetic solitons, nanomagnets, and SQUIDs, coupled to nuclear and paramagnetic spin environments. We then focus on the `central spin' model, which couples a central two-level system to a background spin bath. It is the spin bath analogue of the famous `spin-boson' oscillator model, and describes, e.g., the tunnelling dynamics of nanoscopic and mesoscopic magnets and superconductors. We show how to average over (or `integrate out') spin bath modes, using an operator instanton technique, to find the central spin dynamics. The formal manouevres involve four separate averages - each average corresponds physically to a different `decoherence' mechanism acting on the central spin dynamics. Each environmental spin has its own topological `spin phase', which by interacting with the phase of the central system, decoheres it - this can happen even without dissipation. We give analytic results for the central spin correlation functions, under various conditions. We then describe the application of this theory to magnetic and superconducting systems. Particular attention is given to recent work on tunnelling magnetic macromolecules, where the role of the nuclear spin bath in controlling the tunnelling is very clear; we also discuss other magnetic systems in the quantum regime, and the influence of nuclear and paramagnetic spins on flux dynamics in SQUIDs. Finally, we discuss decoherence mechanisms and coherence experiments in superconductors and magnets. We show that a spin bath environment causes decoherence even in the T 0 limit. Control of this decoherence will be essential in the effort to construct `qubits' for quantum computers.