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arXiv:quant-ph/0302109 · Journal of Modern Optics

Applications of coherent population transfer to quantum information processing

Raymond G. Beausoleil, W. J. Munro, T. P. Spiller

Published Jul 1, 2004• 35 citations
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Abstract

We develop a theoretical framework for the exploration of quantum mechanical coherent population transfer phenomena, with the ultimate goal of constructing faithful models of devices for classical and quantum information processing applications. We begin by outlining a general formalism for weak-field quantum optics in the Schrödinger picture, and we include a general phenomenological representation of Lindblad decoherence mechanisms. We use this formalism to describe the interaction of a single stationary multilevel atom with one or more propagating classical or quantum laser fields, and we describe in detail several manifestations and applications of electromagnetically induced transparency. In addition to providing a clear description of the nonlinear optical characteristics of electromagnetically transparent systems that lead to ‘ultraslow light’, we verify that—in principle—a multi-particle atomic or molecular system could be used as either a low power optical switch or a quantum phase shifter. However, we demonstrate that the presence of significant dephasing effects destroys the induced transparency, and that increasing the number of particles weakly interacting with the probe field only reduces the nonlinearity further. Finally, a detailed calculation of the relative quantum phase induced by a system of atoms on a superposition of spatially distinct Fock states predicts that a significant quasi-Kerr nonlinearity and a low entropy cannot be simultaneously achieved in the presence of arbitrary spontaneous emission rates. Within our model, we identify the constraints that need to be met for this system to act as a one-qubit and a two-qubit conditional phase gate.

DOI
10.1080/09500340408232474

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We develop a theoretical framework for the exploration of quantum mechanical coherent population transfer phenomena, with the ultimate goal of constructing faithful models of devices for classical and quantum information processing applications. We begin by outlining a general formalism for weak-field quantum optics in the Schrödinger picture, and we include a general phenomenological representation of Lindblad decoherence mechanisms. We use this formalism to describe the interaction of a single stationary multilevel atom with one or more propagating classical or quantum laser fields, and we describe in detail several manifestations and applications of electromagnetically induced transparency. In addition to providing a clear description of the nonlinear optical characteristics of electromagnetically transparent systems that lead to ‘ultraslow light’, we verify that—in principle—a multi-particle atomic or molecular system could be used as either a low power optical switch or a quantum phase shifter. However, we demonstrate that the presence of significant dephasing effects destroys the induced transparency, and that increasing the number of particles weakly interacting with the probe field only reduces the nonlinearity further. Finally, a detailed calculation of the relative quantum phase induced by a system of atoms on a superposition of spatially distinct Fock states predicts that a significant quasi-Kerr nonlinearity and a low entropy cannot be simultaneously achieved in the presence of arbitrary spontaneous emission rates. Within our model, we identify the constraints that need to be met for this system to act as a one-qubit and a two-qubit conditional phase gate.
We develop a theoretical framework for the exploration of quantum mechanical coherent population transfer phenomena, with the ultimate goal of constructing faithful models of devices for classical and quantum information processing applications.We begin by outlining a general formalism for weak-field quantum optics in the Schrödinger picture, and we include a general phenomenological representation of Lindblad decoherence mechanisms.We use this formalism to describe the interaction of a single stationary multilevel atom with one or more propagating classical or quantum laser fields, and we describe in detail several manifestations and applications of electromagnetically induced transparency.In addition to providing a clear description of the nonlinear optical characteristics of electromagnetically transparent systems that lead to "ultraslow light," we verify that -in principle -a multi-particle atomic or molecular system could be used as either a low power optical switch or a quantum phase shifter.However, we demonstrate that the presence of significant dephasing effects on the metastable levels destroys the induced transparency.Finally, a detailed calculation of the relative quantum phase induced by a system of atoms on a superposition of spatially distinct Fock states predicts that a significant quasi-Kerr nonlinearity and a low entropy cannot be simultaneously achieved in the presence of arbitrary spontaneous emission rates.Within our model, we identify the constraints that need to be met for this system to act as a one-qubit and a two-qubit conditional phase gate.
We provide a broad outline of the requirements that should be met by components produced for a Quantum Information Technology (QIT) industry, and we identify electromagnetically induced transparency (EIT) as potentially key enabling science toward the goal of providing widely available few-qubit quantum information processing within the next decade. As a concrete example, we build on earlier work and discuss the implementation of a two-photon controlled phase gate and a one-photon phase gate using the approximate Kerr nonlinearity provided by EIT. We rigorously the dependence of the performance of these gates on atomic dephasing and field detuning and intensity, and we calculate the optimum parameters needed to apply a pi phase shift in a gate of a given fidelity. Although high-fidelity gate operation will be difficult to achieve with realistic system dephasing rates, the moderate fidelities that we believe will be needed for few-qubit QIT seem much more obtainable.
We provide a broad outline of the requirements that should be met by components produced for a Quantum Information Technology (QIT) industry, and we identify electromagnetically induced transparency (EIT) as potentially key enabling science toward the goal of providing widely available few-qubit quantum information processing within the next decade. As a concrete example, we build on earlier work and discuss the implementation of a two-photon controlled phase gate (and, briefly, a one-photon phase gate) using the approximate Kerr nonlinearity provided by EIT. In this paper, we rigorously analyze the dependence of the performance of these gates on atomic dephasing and field detuning and intensity, and we calculate the optimum parameters needed to apply a π phase shift in a gate of a given fidelity. Although high-fidelity gate operation will be difficult to achieve with realistic system dephasing rates, the moderate fidelities that we believe will be needed for few-qubit QIT seem much more obtainable.
The appearance of quantum interference in the microscopic world is one of the deepest mysteries at the very root of quantum mechanics. When light interacts with atoms, it can induce transitions by way of distinct but indistinguishable pathways and yield unexpected and often counter-intuitive results. Electromagnetically Induced Transparency (EIT), Coherent Population Trapping (CPT), and Lasing Without Inversion (LWI) are modern examples of phenomena where the traditional rules that govern absorption and dispersion undergo major revisions. Spectacular consequences of this new state of affairs include the ability of a light beam to propagate through a normally absorbing medium with little or no absorption, or to undergo amplification even if the active medium is not prepared in a state of population inversion. Light signals have been shown to travel with strongly subluminal group velocities of only a handful of meters per second and, even, to propagate at speed greater than the ordinary speed of light, but without violation of causality or of the established rules that control the transfer of optical information through space. Three-level atoms can interact with two coherent electromagnetic fields according to three different systems, known as Cascade, Lambda and Vee systems. The propagation of a weak probe field can be deeply affected by the presence of a second stronger beam, the so-called coupling field. Transparency windows, splitting of emission and absorption lines and enormously enhanced dispersion have been documented in numerous experiments. In this thesis we explore the physical origin of the transparency induced in these systems by the simultaneous interplay of the coupling and probe fields. We focus our attention on the Cascade system and study its two configurations, Cascade-EIT and Cascade-AT. We develop a variety of complementary approaches for the description of these two configurations, some semiclassical and others fully quantum mechanical. We prove the existence of quantum interference in Electromagnetically Induced Transparency and also the surprising absence of interference in a closely related phenomenon, known as the Autler-Townes effect. Finally we complement the traditional machinery of theoretical quantum optics with techniques borrowed from quantum scattering theory, and offer what we believe is the most convincing physical evidence for the appearance, or for the absence, of quantum interference effects.
Chapter 7 initially discusses mechanical effects on light and their application to optical tweezers. This leads to a discussion of laser cooling of gases and solids, magneto-optic traps, and velocity-selective coherent population trapping. Coherent population transfer is a counterintuitive way of altering the occupation of energy levels in an exceptionally efficient manner. Coherent transverse optical magnetism explores an optical effect mediated by the Lorentz force of light. Induced magnetic scattering is discussed and a closed form solution presented. Electromagnetically induced transparency is an interference effect that is useful for rendering opaque media transparent and enhancing high-order nonlinear optical processes via intermediate steps that may be fully resonant. Slow light is discussed. Squeezed light is given as an example of a coherent state with altered noise properties. Cavity quantum electrodynamics treats the interaction of atoms with light fields inside cavities, showing that strong atom-field interactions are possible in which the energy structure of the atoms is altered. A section on quantum information processing explains how quantum bits may be realized in practice and used to perform logic operations for quantum computing.
Coherent preparation by laser light of quantum states of atoms and molecules can lead to quantum interference in the amplitudes of optical transitions. In this way the optical properties of a medium can be dramatically modified, leading to electromagnetically induced transparency and related effects, which have placed gas-phase systems at the center of recent advances in the development of media with radically new optical properties. This article reviews these advances and the new possibilities they offer for nonlinear optics and quantum information science. As a basis for the theory of electromagnetically induced transparency the authors consider the atomic dynamics and the optical response of the medium to a continuous-wave laser. They then discuss pulse propagation and the adiabatic evolution of field-coupled states and show how coherently prepared media can be used to improve frequency conversion in nonlinear optical mixing experiments. The extension of these concepts to very weak optical fields in the few-photon limit is then examined. The review concludes with a discussion of future prospects and potential new applications.