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arXiv:quant-ph/0208138 · Physical Review A

Maximal entanglement versus entropy for mixed quantum states

Tzu-Chieh Wei, Kae Nemoto, Paul M. Goldbart, Paul G. Kwiat, William J. Munro, Frank Verstraete

Published Feb 28, 2003• 321 citations
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Abstract

Maximally entangled mixed states are those states that, for a given mixedness, achieve the greatest possible entanglement. For two-qubit systems and for various combinations of entanglement and mixedness measures, the form of the corresponding maximally entangled mixed states is determined primarily analytically. As measures of entanglement, we consider entanglement of formation, relative entropy of entanglement, and negativity; as measures of mixedness, we consider linear and von Neumann entropies. We show that the forms of the maximally entangled mixed states can vary with the combination of (entanglement and mixedness) measures chosen. Moreover, for certain combinations, the forms of the maximally entangled mixed states can change discontinuously at a specific value of the entropy. Along the way, we determine the states that, for a given value of entropy, achieve maximal violation of Bell's inequality.

DOI
10.1103/physreva.67.022110

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Maximally entangled mixed states are those states that, for a given mixedness, achieve the greatest possible entanglement. For two-qubit systems and for various combinations of entanglement and mixedness measures, the form of the corresponding maximally entangled mixed states is determined primarily analytically. As measures of entanglement, we consider entanglement of formation, relative entropy of entanglement, and negativity; as measures of mixedness, we consider linear and von Neumann entropies. We show that the forms of the maximally entangled mixed states can vary with the combination of (entanglement and mixedness) measures chosen. Moreover, for certain combinations, the forms of the maximally entangled mixed states can change discontinuously at a specific value of the entropy. Along the way, we determine the states that, for a given value of entropy, achieve maximal violation of Bell's inequality.
We consider mixed states of two qubits and show under which global unitary operations their entanglement is maximized. This leads to a class of states that is a generalization of the Bell states. Three measures of entanglement are considered: entanglement of formation, negativity, and relative entropy of entanglement. Surprisingly all states that maximize one measure also maximize the others. We give a complete characterization of these generalized Bell states and prove that these states for fixed eigenvalues are all equivalent under local unitary transformations. Furthermore we characterize all nearly entangled states closest to the maximally mixed state and derive a lower bound on the volume of separable mixed states.
We qualify the entanglement of arbitrary mixed states of bipartite quantum systems by comparing global and marginal mixednesses quantified by different entropic measures. For systems of two qubits we discriminate the class of maximally entangled states with fixed marginal mixednesses, and determine an analytical upper bound relating the entanglement of formation to the marginal linear entropies. This result partially generalizes to mixed states the quantification of entanglement with marginal mixednesses holding for pure states. We identify a class of entangled states that, for fixed marginals, are globally more mixed than product states when measured by the linear entropy. Such states cannot be discriminated by the majorization criterion.
Recently, Munro, Nemoto, and White (The Bell Inequality: A Measure of Entanglement?, quant-ph/0102119) tried to indicate that the reason behind a state $\ensuremath{\rho}$ having a higher amount of entanglement (as quantified by the entanglement of formation) than a state ${\ensuremath{\rho}}^{\ensuremath{'}},$ but producing the same amount of Bell violation, is due to the fact that the amount of mixedness (as quantified by the linearized entropy) in $\ensuremath{\rho}$ is higher than that in ${\ensuremath{\rho}}^{\ensuremath{'}}.$ We counter their argument with examples. We extend these considerations to the von Neumann entropy. Our results suggest that the reason as to why equal amount of Bell violation requires different amounts of entanglement cannot, at least, be explained by mixedness alone.
The relation between the violation of the Bell-CHSH inequalities and entanglement properties of quantum states is not clear so one may consider the mixedness of the system to understand the entanglement properties better than the Bell-CHSH inequality. In this respect, we prove that if the mixedness of the state measured by the linear entropy is less than 2/3 but strictly greater than zero then the two qubit states are entangled. But if the linear entropy is greater or equal to 2/3 then the state may or may not be entangled. Further we show that our entanglement criterion detects larger set of entangled state than Bell-CHSH inequality and Santos's entropic criterion [Phys. Rev. A 69, 022305 (2004)]. Lastly we illustrate our result by citing few examples.
Amplitude damping changes entangled pure states into usually less-entangled mixed states. We show, however, that even local amplitude damping of one or two qubits can result in mixed states more entangled than pure states if one compares the relative entropy of entanglement (REE) for a given degree of the Bell--Clauser-Horne-Shimony-Holt inequality violation (referred to as nonlocality). By applying Monte Carlo simulations, we find the maximally entangled mixed states and show that they are likely to be optimal by checking the Karush-Kuhn-Tucker conditions, which generalize the method of Lagrange multipliers for this nonlinear optimization problem. We show that the REE for mixed states can exceed that of pure states if the nonlocality is in the range (0,0.82) and the maximal difference between these REEs is 0.4. A former comparison [Phys. Rev. A 78, 052308 (2008)] of the REE for a given negativity showed analogous property but the corresponding maximal difference in the REEs is one order smaller (i.e., 0.039) and the negativity range is (0,0.53) only. For appropriate comparison, we normalized the nonlocality measure to be equal to the standard entanglement measures, including the negativity, for arbitrary two-qubit pure states. We also analyze the influence of the phase-damping channel on the entanglement of the initially pure states. We show that the minimum of the REE for a given nonlocality can be achieved by this channel, contrary to the amplitude-damping channel.
It is well known that the violation of Bell's inequality in the form given by Clauser, Horne, Shimony, and Holt (CHSH) in two-qubit systems requires entanglement, but not vice versa, i.e., there are entangled states which do not violate the CHSH inequality. Here we compare some standard entanglement measures with violations of the CHSH inequality (as given by the Horodecki measure) for two-qubit states generated by Monte Carlo simulations. We describe states that have extremal entanglement according to the negativity, concurrence, and relative entropy of entanglement for a given value of the CHSH violation. We explicitly find these extremal states by applying the generalized method of Lagrange multipliers based on the Karush-Kuhn-Tucker conditions. The found minimal and maximal states define the range of entanglement accessible for any two-qubit states that violate the CHSH inequality by the same amount. We also find extremal states for the concurrence versus negativity by considering only such states which do not violate the CHSH inequality. Furthermore, we describe an experimentally efficient linear-optical method to determine the highest Horodecki degree of the CHSH violation for arbitrary mixed states of two polarization qubits. By assuming to have access simultaneously to two copies of the states, our method requires only six discrete measurement settings instead of nine settings, which are usually considered.