Non-local Quantum Electrodynamics. II. Possibility of correlated 2n-photon absorption in gases leading to VERY High frequency spontaneous emission and Very high order Harmonic Generation
In a recent work [Mod. Phys. Lett A13, p-1265 (1998)] we expounded a non-local Quantum Electrodynamics (QED) which predicted a linear two-photon absorption by an atom placed in a laser field of appropriate intensity and frequency. In this paper we extend our earlier work to show that the theory allows for linear 2n-photon absorption by gaseous matter where, under suitable conditions, n may literally run upto thousands. The consequences of this extension of the theory are outlined and predictions are made which may be verified in laboratories.
In a recent work [Mod. Phys. Lett A13, p-1265 (1998)] we expounded a non-local Quantum Electrodynamics (QED) which predicted a linear two-photon absorption by an atom placed in a laser field of appropriate intensity and frequency. In this paper we extend our earlier work to show that the theory allows for linear 2n-photon absorption by gaseous matter where, under suitable conditions, n may literally run upto thousands. The consequences of this extension of the theory are outlined and predictions are made which may be verified in laboratories.
The generation of higher-order harmonic radiation originating from the interaction of intense laser pulses with matter is typically described semiclassically: While the electronic structure and dynamics of matter is described quantum mechanically, the intense light field is described classically---and accordingly the generated harmonic radiation. However, pioneering experiments on quantum optical properties of high-order harmonic generation (HHG) in atomic gases from the group of P. Tzallas [I. Gonoskov et al., Sci. Rep. 6, 32821 (2016) and N. Tsatrafyllis et al., Nat. Commun. 8, 15170 (2017)], and theoretical investigations from the group of M. Lewenstein [M. Lewenstein et al., Nat. Phys. 17, 1104 (2021) and P. Stammer et al., Phys. Rev. Lett. 128, 123603 (2022)] have impressively demonstrated that light's quantum properties are observable in the strong-field realm. In this paper, we develop a quantum optical description of HHG in a bulk semiconductor originating from the nonlinear Bloch current. This mechanism of HHG, known as the intraband current, constitutes the major contribution to the emission spectrum for harmonic with energies of quanta roughly below the bandgap. Under certain approximations, employing a quantum description of both light and matter, we obtain analytical solutions, which allow us to analyze the classical and quantum optical characteristics of the fundamental mode of light and the harmonic modes. We find intricate but sufficiently mild modifications of the photon statistics of the fundamental mode and coherent displacements depending on the parameters of the driving laser field. Similar to high-harmonic generation in atoms, the fundamental and emitted harmonic field modes are entangled. Moreover, our analytical model predicts parameter ranges where these quantum optical properties will be most pronounced, allowing protocols for quantum information processing with high photon numbers over a large range of frequencies.
Ultrafast strong-field laser--plasma physics is shown to offer a promising framework for relativistic nonlinear quantum electrodynamics (QED). As one of its key advantages, this approach to relativistic nonlinear QED does not require an external beam of relativistic particles. Instead, high-energy electrons are produced in this setting as a part of ultrafast strong-field laser--plasma interactions. An intense ultrashort laser pulse generates and accelerates dense electron bunches to relativistic energies, giving rise to photon-pair emission confined to the nanometer scale in space and the attosecond scale in time. As a lowest-order nonlinear QED process, relativistic electrons in laser-driven plasmas are shown to give rise to attosecond bursts of two-photon emission, providing an ultrabroadband source of correlated photon pairs. As a physically insightful estimate, the rate of this two-photon emission is expressed via a product $ α^2 γω_{turn}$, where α is the fine-structure constant, γ is the Lorentz factor, and $ ω_{turn}$ is the local relativistic curvature frequency. Photon pairs with strongest correlations, providing a resource for photon entanglement, are emitted at a much lower rate, estimated as $ α^2 γ^2 ω_{turn} E_{\perp} /E_S$, where E⊥ is the laser electromagnetic field, determining the transverse Lorentz force, and ES is the Schwinger critical field. Our study offers a clear guidance on how quantum aspects of laser-driven relativistic plasma electrodynamics can be isolated from their classical counterparts, enabling a physically justifiable approach to the analysis of nonlinear QED phenomena in complex laser--plasma interactions driven by ultrashort high-intensity laser pulses.
A formulation of quantum electrodynamics is given that applies to atoms in a strong laser field by perturbation theory in a non-relativistic regime. Dipole approximation is assumed. The dual Dyson series, here discussed by referring it to the Birkhoff theorem for singularly perturbed linear differential equations, can be applied and a perturbation series obtained transforming the Hamiltonian by a Pauli-Fierz transformation. But, if just few photons are present high-order harmonics cannot be generated. So, it is proven that odd high-order harmonics only appear when the laser field is intense and one can substitute the creation and annihilation operators by the square root of the mean number of photons taken to be huge, the field retaining its coherency property as observed experimentally for harmonics. In this case, the Hamiltonian for perturbation theory comes to the Kramers-Henneberger form. The theory has a dipolar contribution when the free-electron quiver motion amplitude is larger than the atomic radius. For a Coulomb potential one has that the outer electron is periodically kicked, and so a prove is given that the same should happen to Rydberg atoms in intense microwave fields. The distribution representing the kicking has a Fourier series with just odd terms. Using a modified Rayleigh-Schrödinger perturbation theory, it is shown that under the same condition of validity of the quiver motion amplitude to atomic radius ratio, the atomic wave function is only slightly modified by the laser field due to the way the energy levels rearrange themselves. This gives a prove of stabilization in the limit of laser frequency going to infinity. Then, perturbation theory can be applied when the Keldysh parameter becomes smaller with respect to the shifted distance between the energy levels of the atom.
In recent years, the study of quantum electrodynamics (QED) in light-matter interactions has discovered various interesting phenomenons that orient many applications. However, due to the ambient entanglement among photons and atoms, few-particle dynamics remains challenging to analyze precisely and limits the progress in several fields. In few-particle systems, different number of atoms interacting with the light field generates drastically different results, even when there is only a single photon involved in the system. The interference between individual atom’s spontaneous emission wavefunctions can cooperatively alter the effective atom-light coupling strength. Depending on the spatial distance between individual of atoms and the involved cavities in the interaction progresses, the collective spontaneous emission rate can alter drastically from superradiance, where the emission rate is enhanced to a high value proportional to the atom number, to subradiance, where the excited atom ensemble stays in a dark state with the light trapped forever. Superradiance provides a promising mechanism to create an ultra-strong light-matter coupling environment, which is an important ingredient for the design of ultra-fast optical devices, frequency comb generation and quantum mirrors. The dark state of subradiance, on the other hand, is essential for the quantum memory implementation. Also, nontrivial phenomenons also occur when multiple photons interacting with a single atom simultaneously. When a finite number of photons incidents on an atom, their scattering through an atom is highly nonlinear, and one special eigenstate component of such nonlinear process, namely photonic bound states, exhibits many interesting properties in nonlinear quantum optical systems. The photons in such state are strongly bunched with each other, as if a virtual attractive force is in effect. Also, the frequency of photons are anti-correlated so that their total frequency remains a constant value, no matter how arbitrary the frequency of any individual is. Thesefeatures benefit certain nonlinear quantum processes for quantum computing and quantum imaging. Specially for two-photon excitation imaging, the same-parity two-level fluorophore molecules suffers from extremely low excitation efficiencies due to the far off-resonant intermediate states. However, by replacing the current commonly used ultrashort laser pulse illuminations with two photon bound state photon pairs, namely photonic dimers, the efficiency can be enhanced to orders of magnitude higher. Such exceptionally high excitation efficiency can potentially bring the current in vivo deep brain imaging depth from millimeter level to several centimeters. To obtain a stable source of such photonic dimers, it is found that a laser structure with gain medium of two-photon emission materials is capable of generating the coherent state of photonic dimer and can serve as a promising light source for nonlinear quantum optical devices.
In Part I [1], we presented a quantum theory of third-harmonic generation (THG) under two-photon absorption in a two-level atomic medium. We studied the time evolution of the third-harmonic field and its coherence properties by neglecting the depletion of the pump power. In this paper we extend the theory by taking the depletion of pump power into account. The density matrix for the third-harmonic field is derived. The study of the growth rate of the density matrix in time shows the quantum mechanical effects more clearly. The effects of detuning in the two-photon interactions and atomic motion are pointed out. The results are compared with the earlier results and differences are brought out.
Intense laser-matter interactions are at the center of interest in research and technology since the development of high-power lasers.They have been widely used for fundamental studies in atomic, molecular, and optical physics, and they are at the core of attosecond physics and ultrafast optoelectronics.Although the majority of these studies have been successfully described using classical electromagnetic fields, recent investigations based on fully quantized approaches have shown that intense laser-atom interactions can be used for the generation of controllable high-photon-number entangled coherent states and coherent state superpositions.In this tutorial, we provide a comprehensive fully quantized description of intense laseratom interactions.We elaborate on the processes of high-harmonic generation, above-threshold ionization, and we discuss new phenomena that cannot be revealed within the context of semiclassical theories.We provide the description for conditioning the light field on different electronic processes, and their consequences for quantum state engineering of light.Finally, we discuss the extension of the approach to more complex materials, and the impact to quantum technologies for a new photonic platform composed of the symbiosis of attosecond physics and quantum information science.