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arXiv:quant-ph/0203138 · Physical Review A

Multipulse control of decoherence

Chikako Uchiyama, Masaki Aihara

Published Sep 23, 2002• 73 citations
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Abstract

We present a general formulation to suppress pure dephasing by multipulse control. The formula is free from a specific form of interaction and is expressed in terms of the correlation function of an arbitrary system-reservoir interaction. We first apply the formula to a phenomenological two-level model where the correlation function of the interaction decays exponentially. In this case, we show analytically that the pure dephasing time is effectively lengthened by the multipulse control. Secondly, we apply the formula to the spin-boson model where a spin interacts nonlinearly with a boson reservoir. We find the multipulse control works well when the pulse interval is sufficiently shorter than the correlation time of the system-reservoir interaction. Moreover, in this case, the pure dephasing can also be suppressed by adjusting the pulse interval to the period of dynamical motion of the reservoir.

DOI
10.1103/physreva.66.032313

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We present a general formulation to suppress pure dephasing by multipulse control. The formula is free from a specific form of interaction and is expressed in terms of the correlation function of an arbitrary system-reservoir interaction. We first apply the formula to a phenomenological two-level model where the correlation function of the interaction decays exponentially. In this case, we show analytically that the pure dephasing time is effectively lengthened by the multipulse control. Secondly, we apply the formula to the spin-boson model where a spin interacts nonlinearly with a boson reservoir. We find the multipulse control works well when the pulse interval is sufficiently shorter than the correlation time of the system-reservoir interaction. Moreover, in this case, the pure dephasing can also be suppressed by adjusting the pulse interval to the period of dynamical motion of the reservoir.
We present a strategy for multipulse control over decoherence. When a two-level system interacts with a reservoir characterized by a specific frequency, we find that the decoherence is effectively suppressed by synchronizing the pulse-train application with the dynamical motion of the reservoir. We discuss the applicability of this strategy by studying the dependence of the decoherence suppression on the shape of the coupling spectral density. We find that the effectiveness of this strategy arises from the non-Markovian nature of dynamical motion of the reservoir.
The pulse control of decoherence in a qubit interacting with a quantum environment is studied with focus on a general case where decoherence is induced by both pure dephasing and population decay. To observe how the decoherence is suppressed by periodic pi pulses, we present a simple method to calculate the time evolution of a qubit under arbitrary pulse sequences consisting of bit-flips and/or phase-flips. We examine the effectiveness of the two typical sequences: bb sequence consisting of only bit-flips, and bp sequence consisting of both bit- and phase-flips. It is shown that the effectiveness of the pulse sequences depends on a relative strength of the two decoherence processes especially when a pulse interval is slightly shorter than qubit-environment correlation times. In the short-interval limit, however, the bp sequence is always more effective than, or at least as effective as, the bb sequence.
We investigate the effectiveness of different dynamical decoupling protocols for storage of a single qubit in the presence of a purely dephasing bosonic bath, with emphasis on comparing quantum coherence preservation under uniform versus nonuniform delay times between pulses. In the limit of instantaneous bit-flip pulses, this is accomplished by establishing a different representation of the controlled qubit evolution, where the decoherence behavior after an arbitrary number of pulses is directly expressed in terms of the uncontrolled decoherence function. In particular, analytical expressions are obtained for approximation of the long- and short-term coherence behavior for both Ohmic and supra-Ohmic environments. By focusing on the realistic case of pure dephasing in an excitonic qubit, we quantitatively assess the impact of physical constraints on achievable pulse separations, and show that little advantage of high-level decoupling schemes based on concatenated or optimal design may be expected if pulses cannot be applied sufficiently fast. In such constrained scenarios, we demonstrate how simple modifications of repeated periodic-echo protocols can offer significantly improved coherence preservation in realistic parameter regimes. We expect similar conclusions to be relevant to other constrained qubit devices exposed to quantum or classical phase noise.
In this thesis, we discuss the possibilities for suppression of decoherence, the loss of purity in an open quantum system, and the related process of dephasing. In the first chapter, we review the literature on the subject of open system dynamics, decoherence and methods of decoherence suppression. In the second chapter, we focus on the specific case of a rotationally hot diatomic molecule as an example of an open quantum system, where molecular vibrational wavepackets are subject to dephasing due to rovibrational coupling. We report analytical and numerical results addressing whether the dephasing rate can be controlled by adjustment of the initial wavepacket phases. It appears that over long timescales, phase-only control is not possible, but for earlier timescales the possibility of phase-only control of dephasing remains. In addition, we point out that the time-dependence of the dephasing process depends significantly upon the degeneracy of the rotational environment states. In the final chapter, we discuss the same system, but apply a qualitatively different method of dephasing suppression based on the nonlinear resonance effect in a driving field. We extend previous work on the topic (Shapiro et al. [1]) by considering the effect of using a train of laser pulses as the driving field, in place of a two-colour continuous-wave laser field. We demonstrate that the pulse train method can be more effective at suppressing dephasing than the two-colour CW case.