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arXiv:quant-ph/0203023 · Physical Review Letters

Recording Quantum Properties of Light in a Long-Lived Atomic Spin State: TowardsQuantum Memory

C. Schori, Brian Julsgaard, Jens Lykke Sørensen, Eugene Simon Polzik

Published Jul 15, 2002• 88 citations
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Abstract

We report an experiment on mapping a quantum state of light onto the ground state spin of an ensemble of Cs atoms with the lifetime of 2 ms. Recording of one of the two quadrature phase operators of light is demonstrated with vacuum and squeezed states of light. The sensitivity of the mapping procedure at the level of approximately 1 photon/sec per Hz is shown. The results pave the road towards complete (storing both quadrature phase observables) quantum memory for Gaussian states of light. The experiment also sheds new light on fundamental limits of sensitivity of the magneto-optical resonance method.

DOI
10.1103/physrevlett.89.057903

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We report an experiment on mapping a quantum state of light onto the ground state spin of an ensemble of Cs atoms with the lifetime of 2 ms. Recording of one of the two quadrature phase operators of light is demonstrated with vacuum and squeezed states of light. The sensitivity of the mapping procedure at the level of approximately 1 photon/sec per Hz is shown. The results pave the road towards complete (storing both quadrature phase observables) quantum memory for Gaussian states of light. The experiment also sheds new light on fundamental limits of sensitivity of the magneto-optical resonance method.
A reversible quantum memory allowing us to store and retrieve quantum information serves as a key necessity for implementing many of novel quantum information protocols. As light serves as a reliable long-range carrier of quantum information, and atoms offer the possibility of long storage times, current attempts at creating quantum memories focus on the transfer of the quantum fluctuations of light onto atomic coherences. The work in this thesis focuses on the development of a quantum memory for squeezed light using an ensemble of cold Cesium atoms stored in a magneto-optical trap. Our two major milestones were the development of a source of nonclassical light, and the development of a suitable atomic medium for storage. We first present the results of our efforts to generate a source of squeezed vacuum states resonant with the Cesium D2 line using a PPKTP nonlinear crystal inside of an optical parametric oscillator. Additionally, we characterize these squeezed states by carrying out a quantum state tomography using an iterative maximum likelihood approach. Next we look at the development of a new experiment which would allow us to use cold Cesium atoms as a storage medium in our recently developed magneto-optical trap. As this requires an array of novel tools and experimental techniques, we will discuss the development of these elements, and how they have furthered our progress towards storing quantum states onto our Cesium atoms, and eventually entangling two atomic ensembles.
Summary form only given. A new approach to the problem of the quantum interface between light and atoms has been recently developed. The method utilizes free space dispersive interaction between pulses of light and spin polarized atomic ensembles. Entanglement between the polarization state of light and the collective spin state of atoms is established by measurement, more precisely by detection of light in a certain polarization basis. In the first demonstration of this approach we have generated a long-lived entangled state of two separate macroscopic atomic samples by a polarization measurement on light transmitted through the samples. We then have shown that this approach also works for mapping of a quantum state of light onto long-lived atomic spin state paving the road towards realization of the quantum memory for light. Recently we have also extended the free space light-atoms interface beyond the continuous variables in the proposal, where a coherent superposition "cat" state of an atomic ensemble is generated by a measurement sequence. Progress with other communication protocols such as atomic state teleportation and multiparty networks will be presented.
Quantum memories feature a reversible conversion of optical fields into long-lived atomic spin waves, and are therefore ideal for operating as sensitive atomic sensors. However, up to now, atom-light interferometers have lacked an efficient approach to exploit their ultimate atomic sensing performance, since an extra optical delay line is required to compensate for the memory time. Here, we report a new protocol that records the photocurrent via heterodyne mixing with a stable local oscillator. The obtained complex quadrature amplitude that carries information imprinted on its phase by an external magnetic field, is successfully recovered from the interference patterns between the light and the atomic spin wave, without the stringent requirement of having them overlap in time. Our results reveal that the sensitivity scales favorably with the lifetime of the quantum memory. Our work may have important applications in building distributed quantum networks through quantum memory-assisted atom-light interferometers.
Abstract The ability to efficiently realize storage and readout of optical squeezed states plays a key roll in continuous-variables quantum information processing. Here we study the quantum memory for squeezed state of propagating light in atoms based on the hybrid photon echo re-phasing. The optical quantum state is recorded in two sublevels of the ground state of an atomic ensemble to realize long-lived quantum memory. Taking into account the noise effect due to atomic decay, our estimation indicates that high fidelities larger than the classical fidelity threshold 81.5% are obtainable even with currently available techniques. Moreover, our result shows that the decay rate of atoms restricts the maximal fidelity. Our work provides some practical guidance for the realization of efficient and faithful photon-echo-based memory for squeezed light.
Long-lived quantum memories are essential components of a long-standing goal of remote distribution of entanglement in quantum networks. These can be realized by storing the quantum states of light as single-spin excitations in atomic ensembles. However, spin states are often subjected to different dephasing processes that limit the storage time, which in principle could be overcome using spin-echo techniques. Theoretical studies suggest this to be challenging due to unavoidable spontaneous emission noise in ensemble-based quantum memories. Here, we demonstrate spin-echo manipulation of a mean spin excitation of 1 in a large solid-state ensemble, generated through storage of a weak optical pulse. After a storage time of about 1 ms we optically read-out the spin excitation with a high signal-to-noise ratio. Our results pave the way for long-duration optical quantum storage using spin-echo techniques for any ensemble-based memory.
We show that a quasiperfect quantum-state transfer between an atomic ensemble and fields in an optical cavity can be achieved in electromagnetically induced transparency (EIT). A squeezed vacuum field state can be mapped onto the long-lived atomic spin associated to the ground-state sublevels of the $\ensuremath{\Lambda}$-type atoms considered. The EIT on-resonance situation show interesting similarities with the Raman off-resonant configuration. We then show how to transfer the atomic squeezing back to the field exiting the cavity, thus realizing a quantum memory--type operation.