Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:quant-ph/0202065 · The Journal of Chemical Physics

Design of strongly modulating pulses to implement precise effective Hamiltonians for quantum information processing

Evan M. Fortunato, Marco A. Pravia, Nicolas Boulant, Grum Teklemariam, Timothy F. Havel, David G. Cory

Published May 1, 2002• 243 citations
arXivHTMLPDF

Abstract

We describe a method for improving coherent control through the use of detailed knowledge of the system’s Hamiltonian. Precise unitary transformations were obtained by strongly modulating the system’s dynamics to average out unwanted evolution. With the aid of numerical search methods, pulsed irradiation schemes are obtained that perform accurate, arbitrary, selective gates on multiqubit systems. Compared to low power selective pulses, which cannot average out all unwanted evolution, these pulses are substantially shorter in time, thereby reducing the effects of relaxation. Liquid-state nuclear magnetic resonance techniques on homonuclear spin systems are used to demonstrate the accuracy of these gates both in simulation and experiment. Simulations of the coherent evolution of a three-qubit system show that the control sequences faithfully implement the unitary operations, typically yielding gate fidelities on the order of 0.999 and, for some sequences, up to 0.9997. The experimentally determined density matrices resulting from the application of different control sequences on a three-spin system have overlaps of up to 0.99 with the expected states, confirming the quality of the experimental implementation.

DOI
10.1063/1.1465412

Related papers

Preparation of subspace effective-pure state for NMR QIP by means of strongly modulating pulses

Zhou Xian-yi

An alternative method for preparing an effective-pure state in a subsystem of a three-spin system for quantum information processing(QIP) in liquid-state nuclear magnetic resonance(NMR) was demonstrated experimentally.With the aid of numerical search methods,strongly modulating pulses(SMP) scheme was obtained and can perform accurate,arbitrary,selective gates on a three-qubit system.Compared with low-power(nuclear-selective) pulse scheme,the number of shaped pulses and the width of each pulse were both reduced.A pair of two-qubit subspace effective-pure states within a three-spin system was acquired simultaneously.The tomography for the spin system agreed with theoretical predictions,which shows that the experiments were successfully implemented.The short pulse-width of SMP substantially reduced the effects of relaxation within the period of pulse.This is very useful for NMR QIP involving larger numbers of qubits.

•Jan 1, 2008•0 citations

Coherent control for quantum information processing

Gaurav Bhole

An exquisite control over the dynamics of a quantum system is essential for realizing any quantum technology. This thesis presents some practical and efficient strategies for coherent quantum control: a paradigm for controlling quantum dynamics using electromagnetic fields. Coherent control is a common framework for describing the physical implementation of quantum logic gates in several quantum information processing platforms including superconducting qubits and trapped ions. For the purpose of demonstration, however, liquid-state Nuclear Magnetic Resonance (NMR) is used in this thesis as it is an ideal test-bed for developing, testing and benchmarking coherent control tools and techniques. Coherent control was revitalised in 2005 by the development of Gradient Ascent Pulse Engineering (GRAPE), a powerful optimal control technique that is widely used for designing shaped pulses for a variety of tasks. GRAPE, like any other closed-loop optimal control algorithm, requires multiple evaluations of the computationally expensive matrix exponential and the full time-evolution propagator. To this end, I present strategies to sidestep the explicit evaluation of matrix exponentials, thereby offering substantial speed-ups over conventional implementations of the GRAPE algorithm. The results are demonstrated experimentally in NMR, but also in simulations of ultracold molecules and superconducting qubits. Beyond GRAPE, this thesis also considers methods for designing spin-echo sequences for implementing any arbitrary network of controlled-Z gates in a system of qubits with zz-couplings. First, a method based on linear-programming provides near time-optimal sequences in fully-coupled systems having up to a few hundred qubits. Further, an analytic method based on graph colouring finds near time-optimal spin echo sequences in engineered systems with any number of qubits having only nearest and next-nearest neighbour-couplings.

•Jan 1, 2020•0 citations

Efficient synthesis of quantum gates on indirectly coupled spins

Haidong Yuan, Daxiu Wei, Yajuan Zhang +2 more

Experiments in coherent nuclear and electron magnetic resonance and quantum computing in general correspond to control of quantum-mechanical systems, guiding them from initial to final target states by unitary transformations. The control inputs (pulse sequences) that accomplish these unitary transformations should take as little time as possible so as to minimize the effects of relaxation and decoherence and to optimize the sensitivity of the experiments. Here, we derive a time-optimal sequences as fundamental building blocks to synthesize unitary transformations. Such sequences can be widely implemented on various physical systems, including the simulation of effective Hamiltonians for topological quantum computing on spin lattices. Experimental demonstrations are provided for a system consisting of three nuclear spins.

arXiv:1309.3837•Physical Review A•Apr 17, 2014•14 citations

Selective-pulse-network compilation on a liquid-state nuclear-magnetic-resonance system

Jun Li, Jiangyu Cui, Raymond Laflamme +1 more

In creating a large-scale quantum information processor, the ability to construct control pulses for implementing an arbitrary quantum circuit in a scalable manner is an important requirement. For liquid-state nuclear-magnetic-resonance quantum computing, a circuit is generally realized through a sequence of selective soft pulses, in which various control imperfections exist and are to be corrected. In this work, we present a comprehensive analysis of the errors arisen in a selective pulse network by using the zeroth- and first-order average Hamiltonian theory. Effective correction rules are derived for adjusting important pulse parameters such as irradiation frequencies, rotational angles, and transmission phases of the selective pulses to increase the control fidelity. Simulations show that applying our compilation procedure for a given circuit is efficient and can greatly reduce the error accumulation.

arXiv:1608.00674•Physical Review A•Sep 15, 2016•10 citations

Using Nuclear Magnetic Resonance to Assess and Optimize the Precision of Methods for Controlling Quantum Dynamics

David G. Cory, Timothy F. Havel

The most significant achievements of this project were: (1) Development and validation of the hardware and software needed to implement "strongly modulating pulses", by which high precision quantum gates can be obtain in realistic systems of up to 12 qubits; (2) A detailed analysis and evaluation of a 3-qubit quantum Fourier transform via full quantum process tomography; (3) An extensive set of mathematical and computational techniques to accomplish these goals, including Hadamard products, the real density matrix, and methods of fitting superoperators to experimental data; (4) Creation of a 3-qubit "noiseless subsystem", of a Bell state on two 2-qubit decoherence-free subspaces (DFS), and the invention of "partial" pseudopure states which will enable us to demonstrate robust methods for controlling multi-DFS-qubit systems by NMR; (5) Implementation of several quantum chaotic maps, and the discovery that these provide a scalable approach to determining the magnitude and kind of errors present in complex quantum computations; (6) The invention of a "spin amplifier", by which entanglement can be used to enable single spin measurement, and a small-scale demonstration by NMR; (7) Experiments demonstrating that the foregoing advances enable implementation of complex entangling unitary and decoherent operations, culminating in creation of a 12-qubit CAT state.

•Jul 31, 2005•0 citations

Experimental demonstration of an entanglement swapping operation and improved control in NMR quantum-information processing

Nicolas Boulant, Karina Montilla Edmonds, Jerry Zhijian Yang +2 more

We demonstrate the implementation of an entanglement swapping operation on a four-qubit liquid-state nuclear-magnetic-resonance (NMR) quantum-information processor. We use this experiment as a benchmark to illustrate the progress made in the field of quantum control using strongly modulating pulses and a correction scheme for removing distortions introduced by the nonlinearities in the transmitter and probe circuits. The advances include compensating for incoherent errors caused by the spatial variation of the system Hamiltonian in the NMR sample. The goal of these control sequences is to cause the collapse of the Kraus operator-sum representation of the superoperator into one unitary operator so that the ensemble appears to evolve as one coherent whole.

Physical Review A•Sep 11, 2003•35 citations
We describe a method for improving coherent control through the use of detailed knowledge of the system’s Hamiltonian. Precise unitary transformations were obtained by strongly modulating the system’s dynamics to average out unwanted evolution. With the aid of numerical search methods, pulsed irradiation schemes are obtained that perform accurate, arbitrary, selective gates on multiqubit systems. Compared to low power selective pulses, which cannot average out all unwanted evolution, these pulses are substantially shorter in time, thereby reducing the effects of relaxation. Liquid-state nuclear magnetic resonance techniques on homonuclear spin systems are used to demonstrate the accuracy of these gates both in simulation and experiment. Simulations of the coherent evolution of a three-qubit system show that the control sequences faithfully implement the unitary operations, typically yielding gate fidelities on the order of 0.999 and, for some sequences, up to 0.9997. The experimentally determined density matrices resulting from the application of different control sequences on a three-spin system have overlaps of up to 0.99 with the expected states, confirming the quality of the experimental implementation.
An alternative method for preparing an effective-pure state in a subsystem of a three-spin system for quantum information processing(QIP) in liquid-state nuclear magnetic resonance(NMR) was demonstrated experimentally.With the aid of numerical search methods,strongly modulating pulses(SMP) scheme was obtained and can perform accurate,arbitrary,selective gates on a three-qubit system.Compared with low-power(nuclear-selective) pulse scheme,the number of shaped pulses and the width of each pulse were both reduced.A pair of two-qubit subspace effective-pure states within a three-spin system was acquired simultaneously.The tomography for the spin system agreed with theoretical predictions,which shows that the experiments were successfully implemented.The short pulse-width of SMP substantially reduced the effects of relaxation within the period of pulse.This is very useful for NMR QIP involving larger numbers of qubits.
An exquisite control over the dynamics of a quantum system is essential for realizing any quantum technology. This thesis presents some practical and efficient strategies for coherent quantum control: a paradigm for controlling quantum dynamics using electromagnetic fields. Coherent control is a common framework for describing the physical implementation of quantum logic gates in several quantum information processing platforms including superconducting qubits and trapped ions. For the purpose of demonstration, however, liquid-state Nuclear Magnetic Resonance (NMR) is used in this thesis as it is an ideal test-bed for developing, testing and benchmarking coherent control tools and techniques. Coherent control was revitalised in 2005 by the development of Gradient Ascent Pulse Engineering (GRAPE), a powerful optimal control technique that is widely used for designing shaped pulses for a variety of tasks. GRAPE, like any other closed-loop optimal control algorithm, requires multiple evaluations of the computationally expensive matrix exponential and the full time-evolution propagator. To this end, I present strategies to sidestep the explicit evaluation of matrix exponentials, thereby offering substantial speed-ups over conventional implementations of the GRAPE algorithm. The results are demonstrated experimentally in NMR, but also in simulations of ultracold molecules and superconducting qubits. Beyond GRAPE, this thesis also considers methods for designing spin-echo sequences for implementing any arbitrary network of controlled-Z gates in a system of qubits with zz-couplings. First, a method based on linear-programming provides near time-optimal sequences in fully-coupled systems having up to a few hundred qubits. Further, an analytic method based on graph colouring finds near time-optimal spin echo sequences in engineered systems with any number of qubits having only nearest and next-nearest neighbour-couplings.
Experiments in coherent nuclear and electron magnetic resonance and quantum computing in general correspond to control of quantum-mechanical systems, guiding them from initial to final target states by unitary transformations. The control inputs (pulse sequences) that accomplish these unitary transformations should take as little time as possible so as to minimize the effects of relaxation and decoherence and to optimize the sensitivity of the experiments. Here, we derive a time-optimal sequences as fundamental building blocks to synthesize unitary transformations. Such sequences can be widely implemented on various physical systems, including the simulation of effective Hamiltonians for topological quantum computing on spin lattices. Experimental demonstrations are provided for a system consisting of three nuclear spins.
In creating a large-scale quantum information processor, the ability to construct control pulses for implementing an arbitrary quantum circuit in a scalable manner is an important requirement. For liquid-state nuclear-magnetic-resonance quantum computing, a circuit is generally realized through a sequence of selective soft pulses, in which various control imperfections exist and are to be corrected. In this work, we present a comprehensive analysis of the errors arisen in a selective pulse network by using the zeroth- and first-order average Hamiltonian theory. Effective correction rules are derived for adjusting important pulse parameters such as irradiation frequencies, rotational angles, and transmission phases of the selective pulses to increase the control fidelity. Simulations show that applying our compilation procedure for a given circuit is efficient and can greatly reduce the error accumulation.
The most significant achievements of this project were: (1) Development and validation of the hardware and software needed to implement "strongly modulating pulses", by which high precision quantum gates can be obtain in realistic systems of up to 12 qubits; (2) A detailed analysis and evaluation of a 3-qubit quantum Fourier transform via full quantum process tomography; (3) An extensive set of mathematical and computational techniques to accomplish these goals, including Hadamard products, the real density matrix, and methods of fitting superoperators to experimental data; (4) Creation of a 3-qubit "noiseless subsystem", of a Bell state on two 2-qubit decoherence-free subspaces (DFS), and the invention of "partial" pseudopure states which will enable us to demonstrate robust methods for controlling multi-DFS-qubit systems by NMR; (5) Implementation of several quantum chaotic maps, and the discovery that these provide a scalable approach to determining the magnitude and kind of errors present in complex quantum computations; (6) The invention of a "spin amplifier", by which entanglement can be used to enable single spin measurement, and a small-scale demonstration by NMR; (7) Experiments demonstrating that the foregoing advances enable implementation of complex entangling unitary and decoherent operations, culminating in creation of a 12-qubit CAT state.
We demonstrate the implementation of an entanglement swapping operation on a four-qubit liquid-state nuclear-magnetic-resonance (NMR) quantum-information processor. We use this experiment as a benchmark to illustrate the progress made in the field of quantum control using strongly modulating pulses and a correction scheme for removing distortions introduced by the nonlinearities in the transmitter and probe circuits. The advances include compensating for incoherent errors caused by the spatial variation of the system Hamiltonian in the NMR sample. The goal of these control sequences is to cause the collapse of the Kraus operator-sum representation of the superoperator into one unitary operator so that the ensemble appears to evolve as one coherent whole.