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arXiv:quant-ph/0109037

From Spectral Relaxation to Quantified Decoherence

Chr. Balzer, Th. Hannemann, Dirk Reiß, Werner Neuhauser, P. E. Toschek, C. Wunderlich

Published Sep 7, 2001• 0 citations
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Abstract

Quantum information processing (QIP) requires thorough assessment of decoherence. Atoms or ions prepared for QIP often become addressed by radiation within schemes of alternating microwave-optical double resonance. A well-defined amount of decoherence may be applied to the system when spurious resonance light is admitted simultaneously with the driving radiation. This decoherence is quantified in terms of longitudinal and transversal relaxation. It may serve for calibrating observed decoherence as well as for testing error-correcting quantum codes.

DOI
10.48550/arxiv.quant-ph/0109037

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Quantum information processing (QIP) requires thorough assessment of decoherence. Atoms or ions prepared for QIP often become addressed by radiation within schemes of alternating microwave-optical double resonance. A well-defined amount of decoherence may be applied to the system when spurious resonance light is admitted simultaneously with the driving radiation. This decoherence is quantified in terms of longitudinal and transversal relaxation. It may serve for calibrating observed decoherence as well as for testing error-correcting quantum codes.
Atoms or ions prepared in traps for applications in quantum information processing (QIP) often become addressed by radiation within schemes of alternating microwave-optical double resonance. QIP requires thorough assessment of decoherence. A well-defined amount of decoherence may be applied to the system when spurious resonance light is admitted simultaneously with the driving radiation. This decoherence is quantified in terms of longitudinal and transversal relaxation. It may serve for calibrating observed decoherence as well as for testing error-correcting quantum codes.
The development of quantum error correcting techniques is of paramount importance to the ultimate goal of implementing practical quantum computers. The simultaneous transmission of quantum and classical information over a quantum channel was initially investigated by Shor and since been continued by others. It was shown that there is an advantage to transmitting both quantum and classical information simultaneously, compared to independent transmissions. The characterization and construction of codes that allow to transmit both quantum and classical information, which we refer to as hybrid codes, was done from a coding theory perspective and by using the operator algebra quantum error correction (OAQEC) perspective. In this work we unify these two perspectives, showing that the coding theory formulation is a specific case of the OAQEC perspective. As a result we generalized the quantum hamming bound to the hybrid case. To date no such hybrid codes have been physically implemented. Nuclear magnetic resonance (NMR) quantum information processors (QIP) have been an excellent test bed for quantum computing. The techniques of NMR had been refined for many years and can now be applied to quantum computing. NMR techniques provides a high degree of qubit control and long decoherence times compared to other QIP. These two properties of NMR QIP make it a prime candidate for implementing hybrid codes. In this work we developed a hybrid code and designed the circuit for encoding it. We used Matlab to simulate the pulse sequence which would be used in an NMR QIP to carry out the encoding of the hybrid circuit. According to those simulations the full encoding, a single qubit Pauli error and a full decoding can be carried out without the effects of decoherence destroying the quantum information beyond retrieval.
The success of the emerging field of solid-state optical quantum information processing (QIP) critically depends on the access to resonant optical materials. Rare-earth ions (REIs) are suitable candidates for QIP protocols due to their extraordinary photo-physical and magnetic quantum properties such as long optical and spin coherence lifetimes (T2T_2T2​). However, molecules incorporating REIs, despite having advantageous properties such as atomically exact quantum tunability, inherent scalability, and large portability, have not yet been studied for QIP applications. As a first testimony of the usefulness of REI molecules for optical QIP applications, we demonstrate in this study that narrow spectral holes can be burned in the inhomogeneously broadened 5^55D0→7_0\to^70​→7F0_00​ optical transition of a binuclear Eu(III) complex, rendering a homogeneous linewidth (ΓhΓ_hΓh​) = 22 ±\pm± 1 MHz, which translates as T2=14.5T_2 = 14.5T2​=14.5 ±\pm± 0.7 ns at 1.4 K. Moreover, long-lived spectral holes are observed, demonstrating efficient polarization of Eu(III) ground state nuclear spins, a fundamental requirement for all-optical spin initialization and addressing. These results elucidate the usefulness of REI-based molecular complexes as versatile coherent light-spin interfaces for applications in quantum communications and processing.
From the early days of quantum theory, it is felt that the classical ideas about information may need reorientation under a quantum theoretical framework. In quantum theory, where Heisenberg uncertainty principle is the guiding philosophy, a non-commuting observable cannot simultaneously have precisely defined values. In fact, if two observations do not commute, performing a measurement of one observable will necessarily influence the outcome of a subsequent measurement of the other observable. Hence, the act of acquiring information about a physical system inevitably disturbs the state of the system. This is because of the fact that the outcome of a measurement has some random elements due to uncertainty of the initial state of the system. Moreover, acquiring information causes a disturbance, and due to this disturbance the information cannot be copied with perfect fidelity. The information under this framework is termed as quantum information [1].
Abstract The success of the emerging field of solid-state optical quantum information processing (QIP) critically depends on the access to resonant optical materials. Rare-earth ion (REI)- based molecular systems, whose quantum properties could be tuned taking advantage of molecular engineering strategies, are one of the systems actively pursued for the implementation of QIP schemes. Herein, we demonstrate the efficient polarization of 2 ground-state nuclear spins—a fundamental requirement for all-optical spin initialization and addressing—in a binuclear Eu(III) complex, featuring inhomogeneously broadened 5D0→7 F0 optical transition. At 1.4 K, long-lived spectral holes have been burnt in the transition: homogeneous linewidth (Γh) = 22 +/- 1 MHz, which translates as optical coherence lifetime (T2opt) = 14.5 +/- 0.7 ns, and ground-state spin population lifetime (T1spin) = 1.6 +/- 0.4 s have been obtained. The results presented in this study are a progressive step towards the realization of molecule-based coherent light-spin QIP interfaces.