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arXiv:quant-ph/0107126 · Physical Review Letters

Coherent Population Trapping in Two-Electron Three-Level Systems with Aligned Spins

J. Mompart, R. Corbalán, L. Roso

Published Dec 21, 2001• 16 citations
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Abstract

The possibility of coherent population trapping in two electron states with aligned spins (orthosystem) is evidenced. From the analysis of a three-level atomic system containing two electrons, and driven by the two laser fields needed for coherent population trapping, a conceptually new kind of dark state appears. The properties of this trapping are physically interpreted in terms of a dark hole, instead of a dark two-electron state. This technique, among many other applications, offers the possibility of measuring, with subnatural resolution, some superposition-state matrix elements of the electron-electron correlation that due to their time dependent nature are inaccessible by standard measuring procedures.

DOI
10.1103/physrevlett.88.023603

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Coherent population trapping in two electron three-level systems with aligned spins

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Journal of Experimental and Theoretical Physics•Apr 1, 2006•3 citations
The possibility of coherent population trapping in two electron states with aligned spins (orthosystem) is evidenced. From the analysis of a three-level atomic system containing two electrons, and driven by the two laser fields needed for coherent population trapping, a conceptually new kind of dark state appears. The properties of this trapping are physically interpreted in terms of a dark hole, instead of a dark two-electron state. This technique, among many other applications, offers the possibility of measuring, with subnatural resolution, some superposition-state matrix elements of the electron-electron correlation that due to their time dependent nature are inaccessible by standard measuring procedures.
This work investigates the possibility of realizing coherent population trapping (CPT) in a two-electron three-level system with parallel spins. Making an analogy with solid-state physics, this study demonstrates that a V-type three-level system with two electrons can be described as a /spl Lambda/-type three-level system for one single hole. Cancellation of the probe field absorption is obtained when the hole is placed in the dark state. Alternatively, in terms of the two-electron V-type system, the CPT condition is realized when one electron is placed in the ground state and the other one in the bright combination of the excited states. In addition, when the electron-electron Coulomb repulsion is taken into account, it is shown that this technique offers the possibility of measuring, with subnatural resolution, some superposition-state matrix elements of the electron-electron correlation that due to their time dependent nature are inaccessible by standard measuring procedures.
We observe coherent population trapping (CPT) in a two-electron atom— 174 Yb—using the transition. CPT is not possible for such a transition according to one-electron theory because the magnetic sublevels form a V-type system, but in a two-electron atom like Yb, the interaction of the electrons transforms the level structure into a Λ -type system, which allows the formation of a dark state and hence the observation of CPT. Since the two levels involved are degenerate, we use a magnetic field to lift the degeneracy. The single fluorescence dip then splits into five dips—the central unshifted one corresponds to coherent population oscillation, while the outer four are due to CPT. The linewidth of the CPT resonance is about 300 kHz and is limited by the natural linewidth of the excited state, which is to be expected because the excited state is involved in the formation of the dark state.
We show that an arbitrary system described by two dipole moments exhibits coherent superpositions of internal states that can be completely decoupled from the dissipative interactions (responsible for decoherence) and an external driving laser field. These superpositions, known as dark or trapping states, can be completely stable or can coherently interact with the remaining states. We examine the master equation describing the dissipative evolution of the system and identify conditions for population trapping and also classify processes that can transfer the population to these undriven and nondecaying states. It is shown that coherent transfers are possible only if the two systems are nonidentical, that is the transitions have different frequencies and/or decay rates. In particular, we find that the trapping conditions can involve both coherent and dissipative interactions, and depending on the energy level structure of the system, the population can be trapped in a linear superposition of two or more bare states, a dressed state corresponding to an eigenstate of the system plus external fields or, in some cases, in one of the excited states of the system. A comprehensive analysis is presented of the different processes that are responsible for population trapping, and we illustrate these ideas with three examples of two coupled systems: single V- and $\ensuremath{\Lambda}$-type three-level atoms and two nonidentical two-level atoms, which are known to exhibit dark states. We show that the effect of population trapping does not necessarily require decoupling of the antisymmetric superposition from the dissipative interactions. We also find that the vacuum-induced coherent coupling between the systems could be easily observed in $\ensuremath{\Lambda}$-type atoms. Our analysis of the population trapping in two nonidentical atoms shows that the atoms can be driven into a maximally entangled state which is completely decoupled from the dissipative interaction.
Three-level systems exhibit quantum interference effects absent in two-level systems, making them important for quantum optics. Here, we study the coherent interaction of a Λ-type three-level system with free electrons shaped by optical near fields. By treating the electron train as a quantum drive, we show that the interplay between electron modulation and the three-level system's transition pathways induces tunable interference patterns. This interaction effectively realizes electron-mediated coherent population trapping. We identify a regime that enables complete population transfer between the two lower states and the preparation of a high-coherence superposition, manifested as dark states. In particular, these driven-dissipative steady states are independent of the initial state. Our Letter proposes shaped free electrons as a platform for steady-state coherent control of three-level systems, enabling atomic-scale state engineering.
Three-level systems exhibit quantum interference effects absent in two-level systems, making them important for quantum optics. Here, we study the coherent interaction of a Lambda-type three-level system with free electrons shaped by optical near fields. By treating the electron train as a quantum drive, we show that the interplay between electron modulation and the three-level system's transition pathways induces tunable interference patterns. This interaction effectively realizes electron-mediated coherent population trapping (CPT). We identify a regime that enables complete population transfer between the two lower states and the preparation of a high-coherence superposition, manifested as dark states. In particular, these driven-dissipative steady states are independent of the initial state. Our work proposes shaped free electrons as a platform for steady-state coherent control of three-level systems, enabling atomic-scale state engineering.
Description of states of quantum systems in terms of bivectors (in the general case, polyvectors) is proposed as an alternative to vectors in a Hilbert space. This approach is developed for slow atoms under coherent population trapping conditions (in a dark state). The field of local two-dimensional dark subspaces is naturally associated with a local bivector field. An analysis in terms of bivectors is performed to recover the state of an atom or an atomic ensemble by using the condition for its being in some unknown dark state. This approach exposes natural correlations between atoms. The corresponding many-particle states belong to the class of states with positive partial transpose.