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arXiv:quant-ph/0107008 · Physical Review Letters

Observation of Nonclassical Photon Statistics due to Quantum Interference

Y. J. Lu, Z. Y. Ou

Published Dec 20, 2001• 62 citations
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Abstract

Phase-dependent photon statistics is observed in the mixed field of a narrow band two-photon source and a coherent field. At a certain phase, the nonclassical effect of photon antibunching occurs while at another the photon bunching effect appears. Furthermore, we observed a novel nonclassical phenomenon that exhibits more complex structure. The different features in photon statistics are attributed to a two-photon interference effect.

DOI
10.1103/physrevlett.88.023601

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Phase-dependent photon statistics is observed in the mixed field of a narrow band two-photon source and a coherent field. At a certain phase, the nonclassical effect of photon antibunching occurs while at another the photon bunching effect appears. Furthermore, we observed a novel nonclassical phenomenon that exhibits more complex structure. The different features in photon statistics are attributed to a two-photon interference effect.
The concept of photon antibunching as a manifestation of nonclassical character in single-mode radiation is extended to two-mode radiation. A simple criterion for the existence of nonclassical effects in two-mode radiation is established. It implies that the intermode photon bunching, rather than antibunching, can play a key role in rendering two-mode radiation nonclassical. The two-mode squeezed vacuum states are used as simple examples to illustrate the essential point of the criterion. The criterion is then used to study the nonclassical properties of two types of two-mode squeezed states. A state generated by applying the squeeze operator to the two-mode vacuum first, followed by the displacement operator, is called a two-mode coherent squeezed state. If the order of the two operators is reversed, a two-mode squeezed coherent state is obtained. It is found that the latter has a much stronger tendency to become a nonclassical state than the former, assuming that the parameters involved are all the same. A measure of nonclassical depth of radiation is adopted. It is found that, according to this measure, the effect of squeezing in making two-mode coherent squeezed states nonclassical is not monotonic. Such phenomena do not occur in squeezed coherent states.
We demonstrate the existence of nonclassical correlations in the radiation of two atoms, that are coherently driven by a continuous laser source. The photon-photon correlations of the fluorescence light show a spatial interference pattern not present in a classical treatment. A feature of this phenomenon is that bunched and antibunched light is emitted in different spatial directions. The calculations are performed analytically. It is pointed out that the correlations are induced by state reduction due to the measurement process when the detection of the photons does not distinguish between the atoms. It is interesting to note that the phenomena show up even without any interatomic interaction.
The statistical fluctuations of light can, under certain circumstances, exhibit a number of interesting nonclassical features. These include photon antibunching, sub-Poissonian statistics, and squeezing, all of which exist only in a quantum field. The three effects are distinct, and do not necessarily go together, although the first two are sometimes mistakenly treated as interchangeable. Both photon antibunching and sub-Poissonian statistics have been observed in experiments on resonance fluorescence from single atoms, which is described. Squeezing has not yet been seen experimentally, although many nonlinear processes are expected to give rise to it. The squeezed state can be recognized in heterodyne or homodyne experiments, where the squeezing becomes manifest as sub-Poissonian photon fluctuations.
Controlling the photon statistics of light is paramount for quantum science and technologies. Recently, we demonstrated that transmitting resonant laser light past an ensemble of two-level emitters can result in a stream of single photons or excess photon pairs. This transformation is due to quantum interference between the transmitted laser light and the incoherently scattered photon pairs [Prasad et al., Nat. Photonics 14, 719 (2020)NPAHBY1749-488510.1038/s41566-020-0692-z]. Here, using the dispersion of the atomic medium, we actively control the relative quantum phase between these two components. We thereby realize a tunable two-photon interferometer and observe interference fringes in the normalized photon coincidence rate. When tuning the relative phase, the coincidence rate varies periodically, giving rise to a continuous modification of the photon statistics from antibunching to bunching. Beyond the fundamental insight that there exists a tunable quantum phase between incoherent and coherent light that dictates the photon statistics, our results lend themselves to the development of novel quantum light sources.
Dirac has written "Each photon then interferes only with itself. Interference between two different photons never occurs." Indeed, a practical definition is that "classical" optics consists of phenomena due to the interference of photons only with themselves. However, photons obey Bose statistics which implies a ``nonclassical'' tendency for them to ``bunch''. For a simple example of nonclassical optical behavior, we consider two pulses of photons of a single frequency that are simultaneously incident on two sides of a lossless, 50:50 beam splitter.
Interference of light fields, first postulated by Young, is one of the fundamental pillars of physics. Dirac extended this observation to the quantum world by stating that each photon interferes only with itself. A precondition for interference to occur is that no welcher-weg information labels the paths the photon takes; otherwise, the interference vanishes. This remains true, even if two-photon interference is considered, e.g., in the Hong-Ou-Mandel-experiment. Here, the two photons interfere only if they are indistinguishable, e.g., in frequency, momentum, polarization, and time. Less known is the fact that two-photon interference and photon indistinguishability also determine the photon statistics in the overlapping light fields of two independent sources. As a consequence, measuring the photon statistics in the far field of two independent sources reveals the degree of indistinguishability of the emitted photons. In this Letter, we prove this statement in theory using a quantum mechanical treatment. We also demonstrate the outcome experimentally with a simple setup consisting of two statistically independent thermal light sources with adjustable polarizations. We find that the photon statistics vary indeed as a function of the polarization settings, the latter determining the degree of welcher-weg information of the photons emanating from the two sources.