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arXiv:quant-ph/0009031 · Journal of Optics B Quantum and Semiclassical Optics

Sympathetic ground-state cooling and coherent manipulation with two-ion crystals

H. J. Rohde, S. Gulde, Christian F. Roos, P A Barton, Dietrich G. Leibfried, Jürgen Eschner, Ferdinand Schmidt‐Kaler, R. Blatt

Published Jan 25, 2001• 99 citations
arXivHTMLPDF

Abstract

We have cooled a two-ion crystal to the ground-state of its collective modes of motion. Laser cooling, more specifically resolved sideband cooling, is performed sympathetically by illuminating only one of the two 40 Ca + ions in the crystal. The heating rates of the motional modes of the crystal in our linear trap have been measured, and we found them considerably smaller than those previously reported by Turchette et al (2000 Phys.Rev. A 61 063418) in the case of trapped 9 Be + ions. After the ground state is prepared, coherent quantum state manipulation of the atomic population can be performed. Up to 12 Rabi oscillations are observed, showing that many coherent manipulations can be achieved. Coherent excitation of each ion individually and ground state cooling are important tools for the realization of quantum information processing in ion traps.

DOI
10.1088/1464-4266/3/1/357

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This thesis extends the recently reported ground state sideband cooling of the axial motion of a single ion to a broader frequency range of the axial motion, the radial motion and ion crystals. Once cold, coherent control of these different configurations is demonstrated. The experimental work in this thesis uses 40Ca+ ions that can be coherently addressed on a narrow linewidth optical transition at 729 nm. The technique of axialization that resonantly couples the two radial modes of motion is used to enhance laser Doppler cooling leading to mean phonon occupation numbers in the low hundreds for both modes. The sideband cooling technique is then used to simultaneously cool both the motional modes to within one phonon of the ground state for the first time evers. Sideband cooling is then also employed to cool the axial modes of many ion Coulomb crystals in two different configurations. For two ions in a 1D chain, motional occupation numbers of nbar_COM=0.30(4) and nbar_B=0.07(3) are achieved. For two ions in a planar 2D configuration the result for the two modes are nbar_T=nbar_COM<0.1. This technique is scaled up to demonstrate ground state occupation of up to 10 ions in the planar configuration. The axial mode of motion of a single motion is used to characterise the coherent addressing capabilities in our system through optical and motional Ramsey spectroscopy. We observe optical coherence times of 1.78(4) ms and motional coherence times of 590(12) ms. Dynamical decoupling techniques are shown to extend these coherence times. Furthermore, basic decoherence models are validated in high-lying non-thermal motional states that are prepared by a sideband heating technique. Progress towards entangling gates is demonstrated using a bichromatic laser beam to prepare non-classical states of motion.

•May 1, 2018•2 citations
We have cooled a two-ion crystal to the ground-state of its collective modes of motion. Laser cooling, more specifically resolved sideband cooling, is performed sympathetically by illuminating only one of the two 40 Ca + ions in the crystal. The heating rates of the motional modes of the crystal in our linear trap have been measured, and we found them considerably smaller than those previously reported by Turchette et al (2000 Phys.Rev. A 61 063418) in the case of trapped 9 Be + ions. After the ground state is prepared, coherent quantum state manipulation of the atomic population can be performed. Up to 12 Rabi oscillations are observed, showing that many coherent manipulations can be achieved. Coherent excitation of each ion individually and ground state cooling are important tools for the realization of quantum information processing in ion traps.
Ground state cooling and coherent manipulation of ions in an rf-(Paul) trap is the prerequisite for quantum information experiments with trapped ions. With resolved sideband cooling on the optical S1/2−D5/2 quadrupole transition we have cooled one and two 40Ca+ ions to the ground state of vibration with up to 99.9% probability. With a novel cooling scheme utilizing electromagnetically induced transparency on the S1/2−P1/2 manifold we have achieved simultaneous ground state cooling of two motional sidebands 1.7 MHz apart. Starting from the motional ground state we have demonstrated coherent quantum state manipulation on the S1/2−D5/2 quadrupole transition at 729 nm. Up to 30 Rabi oscillations within 1.4 ms have been observed in the motional ground state and in the n=1 Fock state. In the linear quadrupole rf-trap with 700 kHz trap frequency along the symmetry axis (2 MHz in radial direction) the minimum ion spacing is more than 5 μm for up to 4 ions. We are able to cool two ions to the ground state in the trap and individually address the ions with laser pulses through a special optical addressing channel.
For quantum information experiments we have cooled one and two 40 Ca + ions to the ground state of vibration with up to 99.9% probability, using resolved sideband cooling on the optical S 1/2 -D 5/2 quadrupole transition. Implementing a novel cooling scheme based on electromagnetically induced transparency on the S ↓/2 -P ↓/2 manifold we have achieved simultaneous ground state cooling of two motional sidebands 1.7 MHz apart. Coherent quantum state manipulation on the S 1/2 -D 5/2 quadrupole transition at 729 nm was demonstrated and up to 30 Rabi oscillations within 1.4 ms have been observed starting from the motional ground state and from the n=1 Fock state. In a linear rf-trap two ions were cooled to the ground state of motion and individual addressing of the ions with laser pulses is achieved.
We investigate single ions of 40Ca+ in Paul traps for quantum information processing. Superpositions of the S½ electronic ground state and the metastable D5/2; state are used to implement a qubit. Laser light on the S½ ↔ D5/2 transition is used for the manipulation of the ion's quantum state. We apply sideband cooling to the ion and reach the ground state of vibration with up to 99.9% probability. Starting from this Fock state (n = 0), we demonstrate coherent quantum state manipulation. A large number of Rabi oscillations and a ms-coherence time is observed. Motional heating is measured to be as low as one vibrational quantum in 190ms. We also report on ground state cooling of two ions.
We investigate single ions of 40Ca+ in Paul traps for quantum information processing. Superpositions of the S½ electronic ground state and the metastable D5/2; state are used to implement a qubit. Laser light on the S½ ↔ D5/2 transition is used for the manipulation of the ion's quantum state. We apply sideband cooling to the ion and reach the ground state of vibration with up to 99.9% probability. Starting from this Fock state (n = 0), we demonstrate coherent quantum state manipulation. A large number of Rabi oscillations and a ms-coherence time is observed. Motional heating is measured to be as low as one vibrational quantum in 190ms. We also report on ground state cooling of two ions.
Laser-cooled atomic ions have led to an unprecedented amount of control over the quantum states of matter. The Coulombic interaction allows for information to be transferred between neighboring ions, and this interaction can be used to entangle qubits for logic operations in quantum information processors. The same procedure for logic operations can be used for high resolution atomic spectroscopy, and is the basis for the most accurate atomic optical clocks to date. This thesis describes how laser-cooled atomic ions can impact physical chemistry through the development of molecular ion spectroscopy techniques and the simulation of magnetic systems by ion trap quantum computers. \n\t \n\tA new technique developed for spectroscopy, Sympathetic Heating Spectroscopy (SHS), takes advantage of the Coulombic interaction between two trapped ions: the control ion and a spectroscopy ion. SHS uses the back action of the interrogating laser to map spectroscopy ion information onto the Doppler shift of the control ion for measurement. SHS only requires Doppler cooling of the ions and fluorescence measurement and represents a simplification of quantum logic spectroscopy. This technique is demonstrated on two individual isotopes of calcium: Ca-40(+) for cooling and Ca-44(+) as the spectroscopy ion. \n \n\tHaving demonstrated SHS with atomic ions, the next step was to extend the technique by loading and characterizing molecular ions. The identification of an unknown molecular ion is necessary and can be achieved by monitoring the change in motion of the two ion crystal, which is dependent on the molecular ion mass. The motion of two trapped ions is described by their normal modes, which can be accurately measured by performing resolved sideband spectroscopy of the S(1/2)-D(5/2) transition of calcium. The resolved sidebands can be used to identify unknown ions (atomic and molecular) by calculating the mass based on the observed value in axial normal mode frequencies. Again, the trapped molecular ion is sympathetically cooled via the Coulombic interaction between the Ca-40(+) and the unknown molecular ion. The sensitivity of SHS could be improved by implementing sympathetic sideband cooling and determining the heating by measuring single quanta of motion. \n\t \n\tThe ultimate limit of control would be the development of an ion trap quantum computer. Many theoretical quantum computing researchers have made bold claims of the exponential improvement a quantum computer would have over a classical computer for the simulation of physical systems such as molecules. These claims are true in principle for ideal systems, but given non-ideal components it is necessary to consider the scaling due to error correction. An estimate of the resource requirements, the total number of physical qubits and computational time, required to compute the ground state energy of a 1-D quantum Transverse Ising Model (TIM) of N spin-1/2 particles, as a function of the system size and the numerical precision, is presented. This estimate is based on analyzing the impact of fault-tolerant quantum error correction in the context of the quantum logic array architecture. The results show that a significant amount of error correction is required to implement the TIM problem due to the exponential scaling of the computational time with the desired precision of the energy. Comparison of this result to the resource requirements for a fault-tolerant implementation of Shor's quantum factoring algorithm reveals that the required logical qubit reliability is similar for both the TIM problem and the factoring problem.
This thesis extends the recently reported ground state sideband cooling of the axial motion of a single ion to a broader frequency range of the axial motion, the radial motion and ion crystals. Once cold, coherent control of these different configurations is demonstrated. The experimental work in this thesis uses 40Ca+ ions that can be coherently addressed on a narrow linewidth optical transition at 729 nm. The technique of axialization that resonantly couples the two radial modes of motion is used to enhance laser Doppler cooling leading to mean phonon occupation numbers in the low hundreds for both modes. The sideband cooling technique is then used to simultaneously cool both the motional modes to within one phonon of the ground state for the first time evers. Sideband cooling is then also employed to cool the axial modes of many ion Coulomb crystals in two different configurations. For two ions in a 1D chain, motional occupation numbers of nbar_COM=0.30(4) and nbar_B=0.07(3) are achieved. For two ions in a planar 2D configuration the result for the two modes are nbar_T=nbar_COM<0.1. This technique is scaled up to demonstrate ground state occupation of up to 10 ions in the planar configuration. The axial mode of motion of a single motion is used to characterise the coherent addressing capabilities in our system through optical and motional Ramsey spectroscopy. We observe optical coherence times of 1.78(4) ms and motional coherence times of 590(12) ms. Dynamical decoupling techniques are shown to extend these coherence times. Furthermore, basic decoherence models are validated in high-lying non-thermal motional states that are prepared by a sideband heating technique. Progress towards entangling gates is demonstrated using a bichromatic laser beam to prepare non-classical states of motion.