Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:quant-ph/0008001 · Physical Review Letters

Manipulation of Cold Atomic Collisions by Cavity QED Effects

J. I. Kim, R.B.B. Santos, P. Nussenzveig

Published Feb 19, 2001• 7 citations
arXivHTMLPDF

Abstract

We show how the dynamics of collisions between cold atoms can be manipulated by a modification of spontaneous emission times. This is achieved by placing the atomic sample in a resonant optical cavity. Spontaneous emission is enhanced by a combination of multiparticle entanglement together with a higher density of modes of the modified vacuum field, in a situation akin to superradiance. A specific situation is considered and we show that this effect can be experimentally observed as a large suppression in trap-loss rates.

DOI
10.1103/physrevlett.86.1474

Related papers

Manipulating molecules with quantum light

Markus Kowalewski, Shaul Mukamel

It was first realized by Purcell (1) that the spontaneous emission rate of a quantum system can be enhanced or suppressed by placing it in a resonant radiofrequency cavity. Spontaneous emission as it was first theoretically described by Einstein (2) is not a pure property of matter. It is described by matter coupled to quantized radiation field modes, which can be manipulated in an artificial structure such as a cavity. Cavity quantum electrodynamics (QED) is used to describe such effects that intimately depend on the fact that light is made of photons. Cavity QED has been extensively studied in atoms and the experimental proof was awarded with the Nobel Prize in 2012 (3). It has been applied to cooling of single atoms and for the detection of single atoms and creating and studying states with few photons and few atoms (4). In more recent developments these ideas have been extended to manipulate electronic states (5) and vibrations in molecules (6, 7). In PNAS, Flick et al. (8) introduce recent theoretical developments for the application of cavity QED to molecules and suggest possible novel applications to photochemistry. These include nonadiabatic dynamics of molecules in cavities, the modification of molecular properties, and the integration of QED with density functional theory. A quantized electromagnetic field mode can be described as a harmonic oscillator whose coordinate is the electric field displacement (Fig. 1 A ). The zero point energy translates into a nonvanishing field intensity ⟨ e 2 ⟩ in the ground state | 0 ⟩ (vacuum fluctuations). The electric vacuum field increases for a small cavity volume e c = ℏ ω c V ϵ 0 , [1] Fig. 1. ( A ) Illustration of the standing wave cavity mode and the resulting field quantization (Fock states). ( B ) Combined matter-field states (dressed states, | ± , n ⟩ … [↵][1]1To whom correspondence should be addressed. Email: smukamel{at}uci.edu. [1]: #xref-corresp-1-1

Proceedings of the National Academy of Sciences•Mar 16, 2017•63 citations

Cavity quantum electrodynamics

Partha Ghose

Introduction Ever since 1916/17 when Einstein argued [45] [46] that spontaneous emission must occur if matter and radiation are to achieve thermal equilibrium, physicists have believed that spontaneous emission is an inherent quantum mechanical property of atoms and that excited atoms inevitably radiate. This view, however, overlooks the fact that spontaneous emission is a consequence of the coupling of quantized energy states of atoms with the quantized radiation field, and is a manifestation of quantum noise or of emission ‘stimulated’ by ‘vacuum fluctuations’. An infinity of vacuum states is available to the photon radiated by an excited atom placed in free space, leading to the effective irreversibility of such emissions. If these vacuum states are modified, as for example by placing an excited atom between closely spaced mirrors or in a small cavity (essentially the Casimir effect), spontaneous emission can be greatly inhibited or enhanced or even made reversible. Recent advances in atomic and optical techniques have made it possible to control and manipulate spontaneous emission. A whole new branch of quantum optics called ‘cavity QED’ has developed since 1987 utilizing these dramatic changes in spontaneous emission rates in cavities to construct new kinds of microscopic masers or micromasers that operate with a single atom and a few photons or with photons emitted in pairs in a two-photon transition.

Cambridge University Press eBooks•Apr 29, 1999•0 citations

Spontaneous Emission Manipulation

Marlan O. Scully, Shi-Yao Zhu, Muhammad Suhail Zubairy

The earliest studies on the subject of spontaneous emission from an excited atom via interaction with the vacuum modes of the radiation field go back to the early days of quantum mechanics. In view of the fundamental nature of the vacuum fluctuations, it was long thought that spontaneous emission could not be controlled. However, in 1946 Purcell noted that the spontaneous emission rate of the atom inside a resonant cavity can be substantially enhanced (or suppressed) over its free-space value. This is due to the dramatic change of the density of modes of the vacuum field in a cavity. The enhancement and suppression of spontaneous emission in resonant and off-resonant cavities were observed experimentally in the 1980s. It was also realized in the 1950s and 1960s that coherent driving fields can dramatically change the characteristics of the spontaneous emission. The Autler-Townes doublet and Mollow three-peak spectrum are the examples of such behavior. A dramatic narrowing of the spectral peaks were discovered in driven multilevel atomic systems in the early 1990s. The role of atomic coherence in quenching spontaneous emission fluctuations in the context of laser physics was studied in the 1980s, via the correlated spontaneous emission laser (CEL). In this case atomic coherence results in the correlation of two spontaneous emission noise events so that the spontaneous emission quantum noise is eliminated in the relative linewidth. Later, it was “discovered” that the spontaneous emission can be suppressed through quantum interference between decay channels. Properly stated, this was rediscovered since it was first discovered and explained by Lamb in the 1940s. If the dipoles of two transitions from one upper level to two lower levels are parallel, the spontaneous emission in an ordinary vacuum can be cancelled. In a nonuniform vacuum, e.g., a cavity, the quenching of spontaneous emission can be achieved, even for the orthogonal dipoles.

•Mar 25, 2017•1 citation

Single-photon superradiance in cold atoms

Rafael Alves De Oliveira, Milrian S. Mendes, Weliton Soares Martins +3 more

The interaction of an ensemble of atoms with common vacuum modes may lead to an enhanced emission into these modes. This phenomenon, known as superradiance, highlights the coherent nature of spontaneous emission, resulting in macroscopic entangled states in mundane situations. The complexity of the typical observations of superradiance, however, masks its quantum nature, allowing alternative classical interpretations. Here we stress how this picture changed with the implementation ten years ago of a new process for single-photon generation from atomic ensembles. We present then the last piece of evidence for the superradiant nature of such a process, reporting the observation of an accelerated emission of the photon with a rate that may be tuned by controllably changing the number of atoms in the ensemble. We hope such an investigation will help open up a new bottom-up approach to the study of superradiance.

arXiv:1408.0825•Physical Review A•Aug 26, 2014•61 citations

Atomic physics experiments in micron-sized cavities: suppressing spontaneous decay at optical frequency

A. Anderson, S. Haroche, E. A. Hinds +3 more

Spontaneous emission from an excited atomic state reflects the properties of the surrounding vacuum field. By placing the atom near a metallic surface or in a cavity, one can modify the spectral density of the vacuum modes coupled to it and either enhance1 or inhibit2 spontaneous emission. Large enhancement3 or inhibition effects have been obtained recently in microwave experiments involving either Rydberg atoms4 or a trapped electron5 radiating in cavities whose sizes were of the order of one-tenth of a millimeter to a centimeter.

•Apr 26, 1987•1 citation

Spontaneous emission by moving atoms

Pierre Meystre, Martin Wilkens

It is well known that spontaneous emission is not an intrinsic atomic property, but rather results from the coupling of the atom to the vacuum modes of the electromagnetic field. As such, it can be modified by tailoring the electromagnetic environment into which the atom can radiate. This was already realized by Purcell, who noted that the spontaneous emission rate can be enhanced if the atom placed inside a cavity is resonant with one of the cavity is resonant with one of the cavity modes, and by Kleppner, who discussed the opposite case of inhibited spontaneous emission. It has also been recognized that spontaneous emission need not be an irreversible process. Indeed, a system consisting of a single atom coupled to a single mode of the electromagnetic field undergoes a periodic exchange of excitation between the atom and the field. This periodic exchange remains dominant as long as the strength of the coupling between the atom and a cavity mode is itself dominant. 23 refs., 6 figs.

•Dec 31, 1994•0 citations
We show how the dynamics of collisions between cold atoms can be manipulated by a modification of spontaneous emission times. This is achieved by placing the atomic sample in a resonant optical cavity. Spontaneous emission is enhanced by a combination of multiparticle entanglement together with a higher density of modes of the modified vacuum field, in a situation akin to superradiance. A specific situation is considered and we show that this effect can be experimentally observed as a large suppression in trap-loss rates.
It was first realized by Purcell (1) that the spontaneous emission rate of a quantum system can be enhanced or suppressed by placing it in a resonant radiofrequency cavity. Spontaneous emission as it was first theoretically described by Einstein (2) is not a pure property of matter. It is described by matter coupled to quantized radiation field modes, which can be manipulated in an artificial structure such as a cavity. Cavity quantum electrodynamics (QED) is used to describe such effects that intimately depend on the fact that light is made of photons. Cavity QED has been extensively studied in atoms and the experimental proof was awarded with the Nobel Prize in 2012 (3). It has been applied to cooling of single atoms and for the detection of single atoms and creating and studying states with few photons and few atoms (4). In more recent developments these ideas have been extended to manipulate electronic states (5) and vibrations in molecules (6, 7). In PNAS, Flick et al. (8) introduce recent theoretical developments for the application of cavity QED to molecules and suggest possible novel applications to photochemistry. These include nonadiabatic dynamics of molecules in cavities, the modification of molecular properties, and the integration of QED with density functional theory. A quantized electromagnetic field mode can be described as a harmonic oscillator whose coordinate is the electric field displacement (Fig. 1 A ). The zero point energy translates into a nonvanishing field intensity ⟨ e 2 ⟩ in the ground state | 0 ⟩ (vacuum fluctuations). The electric vacuum field increases for a small cavity volume e c = ℏ ω c V ϵ 0 , [1] Fig. 1. ( A ) Illustration of the standing wave cavity mode and the resulting field quantization (Fock states). ( B ) Combined matter-field states (dressed states, | ± , n ⟩ … [↵][1]1To whom correspondence should be addressed. Email: smukamel{at}uci.edu. [1]: #xref-corresp-1-1
Introduction Ever since 1916/17 when Einstein argued [45] [46] that spontaneous emission must occur if matter and radiation are to achieve thermal equilibrium, physicists have believed that spontaneous emission is an inherent quantum mechanical property of atoms and that excited atoms inevitably radiate. This view, however, overlooks the fact that spontaneous emission is a consequence of the coupling of quantized energy states of atoms with the quantized radiation field, and is a manifestation of quantum noise or of emission ‘stimulated’ by ‘vacuum fluctuations’. An infinity of vacuum states is available to the photon radiated by an excited atom placed in free space, leading to the effective irreversibility of such emissions. If these vacuum states are modified, as for example by placing an excited atom between closely spaced mirrors or in a small cavity (essentially the Casimir effect), spontaneous emission can be greatly inhibited or enhanced or even made reversible. Recent advances in atomic and optical techniques have made it possible to control and manipulate spontaneous emission. A whole new branch of quantum optics called ‘cavity QED’ has developed since 1987 utilizing these dramatic changes in spontaneous emission rates in cavities to construct new kinds of microscopic masers or micromasers that operate with a single atom and a few photons or with photons emitted in pairs in a two-photon transition.
The earliest studies on the subject of spontaneous emission from an excited atom via interaction with the vacuum modes of the radiation field go back to the early days of quantum mechanics. In view of the fundamental nature of the vacuum fluctuations, it was long thought that spontaneous emission could not be controlled. However, in 1946 Purcell noted that the spontaneous emission rate of the atom inside a resonant cavity can be substantially enhanced (or suppressed) over its free-space value. This is due to the dramatic change of the density of modes of the vacuum field in a cavity. The enhancement and suppression of spontaneous emission in resonant and off-resonant cavities were observed experimentally in the 1980s. It was also realized in the 1950s and 1960s that coherent driving fields can dramatically change the characteristics of the spontaneous emission. The Autler-Townes doublet and Mollow three-peak spectrum are the examples of such behavior. A dramatic narrowing of the spectral peaks were discovered in driven multilevel atomic systems in the early 1990s. The role of atomic coherence in quenching spontaneous emission fluctuations in the context of laser physics was studied in the 1980s, via the correlated spontaneous emission laser (CEL). In this case atomic coherence results in the correlation of two spontaneous emission noise events so that the spontaneous emission quantum noise is eliminated in the relative linewidth. Later, it was “discovered” that the spontaneous emission can be suppressed through quantum interference between decay channels. Properly stated, this was rediscovered since it was first discovered and explained by Lamb in the 1940s. If the dipoles of two transitions from one upper level to two lower levels are parallel, the spontaneous emission in an ordinary vacuum can be cancelled. In a nonuniform vacuum, e.g., a cavity, the quenching of spontaneous emission can be achieved, even for the orthogonal dipoles.
The interaction of an ensemble of atoms with common vacuum modes may lead to an enhanced emission into these modes. This phenomenon, known as superradiance, highlights the coherent nature of spontaneous emission, resulting in macroscopic entangled states in mundane situations. The complexity of the typical observations of superradiance, however, masks its quantum nature, allowing alternative classical interpretations. Here we stress how this picture changed with the implementation ten years ago of a new process for single-photon generation from atomic ensembles. We present then the last piece of evidence for the superradiant nature of such a process, reporting the observation of an accelerated emission of the photon with a rate that may be tuned by controllably changing the number of atoms in the ensemble. We hope such an investigation will help open up a new bottom-up approach to the study of superradiance.
Spontaneous emission from an excited atomic state reflects the properties of the surrounding vacuum field. By placing the atom near a metallic surface or in a cavity, one can modify the spectral density of the vacuum modes coupled to it and either enhance1 or inhibit2 spontaneous emission. Large enhancement3 or inhibition effects have been obtained recently in microwave experiments involving either Rydberg atoms4 or a trapped electron5 radiating in cavities whose sizes were of the order of one-tenth of a millimeter to a centimeter.
It is well known that spontaneous emission is not an intrinsic atomic property, but rather results from the coupling of the atom to the vacuum modes of the electromagnetic field. As such, it can be modified by tailoring the electromagnetic environment into which the atom can radiate. This was already realized by Purcell, who noted that the spontaneous emission rate can be enhanced if the atom placed inside a cavity is resonant with one of the cavity is resonant with one of the cavity modes, and by Kleppner, who discussed the opposite case of inhibited spontaneous emission. It has also been recognized that spontaneous emission need not be an irreversible process. Indeed, a system consisting of a single atom coupled to a single mode of the electromagnetic field undergoes a periodic exchange of excitation between the atom and the field. This periodic exchange remains dominant as long as the strength of the coupling between the atom and a cavity mode is itself dominant. 23 refs., 6 figs.