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arXiv:physics/9805037 · Physical Review A

Atom cooling and trapping by disorder

Péter Horák, Jean-Yves Courtois, G. Grynberg

Published Nov 1, 1998• 80 citations
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Abstract

We demonstrate the possibility of three-dimensional cooling of neutral atoms by illuminating them with two counterpropagating laser beams of mutually orthogonal linear polarization, where one of the lasers is a speckle field, i.e., a highly disordered but stationary coherent light field. This configuration gives rise to atom cooling in the transverse plane via a Sisyphus cooling mechanism similar to the one known in standard two-dimensional optical lattices formed by several plane laser waves. However, striking differences occur in the spatial diffusion coefficients as well as in local properties of the trapped atoms.

DOI
10.1103/physreva.58.3953

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We demonstrate the possibility of three-dimensional cooling of neutral atoms by illuminating them with two counterpropagating laser beams of mutually orthogonal linear polarization, where one of the lasers is a speckle field, i.e., a highly disordered but stationary coherent light field. This configuration gives rise to atom cooling in the transverse plane via a Sisyphus cooling mechanism similar to the one known in standard two-dimensional optical lattices formed by several plane laser waves. However, striking differences occur in the spatial diffusion coefficients as well as in local properties of the trapped atoms.
We demonstrate the possibility of three-dimensional cooling of neutral atoms by illuminating them with two counterpropagating laser beams of mutually orthogonal linear polarization, where one of the lasers is a speckle field, i.e., a highly disordered but stationary coherent light field. This configuration gives rise to atom cooling in the transverse plane via a Sisyphus cooling mechanism similar to the one known in standard two-dimensional optical lattices formed by several plane laser waves. However, striking differences occur in the spatial diffusion coefficients as well as in local properties of the trapped atoms.
We present a general theoretical description of laser cooling of three-level atoms in a Λ configuration in two standing waves. Detunings, intensity, and spatial phase difference of the two waves are arbitrary. We demonstrate that, for a zero spatial phase shift, sub-Doppler cooling requires equal detunings. The basic mechanism is then coherent population trapping. For different detunings sub-Doppler cooling occurs only when the spatial phases of the two standing waves are different. This effect can be traced back to a mechanism of the Sisyphus type. These schemes of sub-Doppler cooling require neither polarization gradients nor magnetic fields.
A theoretical analysis is given for 1-D laser cooling below the Doppler limit of J = 1/2 ground- state atoms. The laser field consists of a pair of counterpropagating, linearly polarized low- power beams, whose polarization directions differ by an angle θ (0 ≤ θ ≤ π/2). For θ ≪ 1, the effective optical pumping time is shown to increase strongly near the nodes of the standing wave and the cooling force can be much larger than that for θ ~1. Moreover, for θ ≪ 1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for θ ~ 1. As a consequence it is possible to achieve an equilibrium atomic distribution that, for θ ≪ 1, is characterized by a mean kinetic energy lower than that predicted to occur for θ = π/2. The equilibrium velocity distribution is not necessarily Maxwellian and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms are trapped in the vicinity of the laser field nodes. An explanation for these effects is given in terms of Sisyphus cooling.
We propose a scheme for three-dimensional trapping and cooling of atoms in a bichromatic standing wave formed by two different longitudinal modes of an optical cavity. The atoms are cooled through an efficient Sisyphus mechanism and trapped at those anti-nodes (maxima) of the stronger field where the second weaker field has a node, this leading to a large effective atom-field coupling. Contrary to the case of a single strong standing wave, the final width of the momentum distribution is considerably less than the depth of the optical potential implying long storage times. The scheme offers the possibility of capturing atoms out of the background and achieving high local densities modulated with the beat frequency of the two involved modes. The results from a three-dimensional semi-classical calculation are confirmed by a full QMCWF simulation as well as by a quantum rate equation model in the one-dimensional case in the proper limits.
In sub-Doppler laser cooling of atoms, the lowest temperatures are known to occur at low (but not too low) excitation, and the temperature increases roughly linearly with laser intensity. However, under conditions for which the lowest temperatures are obtained, the small velocity capture range and low optical pumping rate limit the number of atoms that can be collected into the cold sample. In this study, we present measurements for laser cooling of Rb and metastable He atoms for two counterpropagating laser beams with orthogonal linear polarization (lin\ensuremath{\perp}lin) over a wide range of saturation parameters and laser detunings, together with results of semiclassical (Fokker-Planck) and quantum density matrix calculations. We find that at higher laser intensity, a larger number of atoms can be collected into a final velocity distribution that is significantly narrower than that given by a linear extrapolation vs the square root of laser intensity. Two cooling mechanisms are at work: the sub-Doppler Sisyphus mechanism and also Doppler cooling. Under certain conditions that we discuss, Doppler cooling aids Sisyphus cooling by collecting high-velocity atoms beyond the Sisyphus capture range. He∗{\mathrm{He}}^{*}He∗ presents a rather unusual situation in that the minimum average kinetic energy (Eav){(E}_{\mathrm{av}})(Eav​) for purely Sisyphus cooling is comparable to the minimum value of Eav{E}_{\mathrm{av}}Eav​ with Doppler cooling alone.
We describe a numerical implementation of our semiclassical laser-cooling theory [J. Javanainen, Phys. Rev. A 44, 5857 (1991)] for an arbitrary multilevel atom and light field. There is satisfactory agreement between experiments and temperatures obtained from Langevin-equation simulations of the motion of an atom subject to light-pressure force and the accompanying diffusion in three-dimensional (3D) optical molasses in which there are three orthogonal pairs of counterpropagating waves with a common linear polarization for the two beams in a pair, but orthogonal polarizations between the pairs. However, the velocity distribution of the atoms is anisotropic and may deviate strongly from a Gaussian, heterodyne spectra may have a sideband, and the atomic density may be a maximum at the maximum of the potential of the dipole forces of the molasses beams. Subsequent velocity-linearized analysis of atomic damping and diffusion shows that the damping tensor may have a negative eigenvalue corresponding to heating in large regions of space, even though the light is red tuned for cooling. It is also found that the position-averaged damping and diffusion tensors make a poor predictor of the temperature obtained in Langevin-equation simulations and real experiments. Based on additional simulations of a simple 1D model, we formulate a hypothesis that connects our findings. The key idea is that an atom trapped in a minimum of the potential of the dipole forces is subject to a weaker-than-average damping, and therefore tends to boil out of the trap.