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arXiv:physics/0512033 · Physical Review Letters

One-Dimensional Bose Chemistry: Effects of Nonintegrability

Vladimir Yurovsky, A. Ben‐Reuven, Maxim Olshanii

Published Apr 28, 2006• 21 citations
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Abstract

Three-body collisions of ultracold identical Bose atoms under tight cylindrical confinement are analyzed. A Feshbach resonance in two-body collisions is described by a two-channel zero-range interaction. Elimination of the closed channel in the three-body problem reduces the interaction to a one-channel zero-range one with an energy-dependent strength. The related integrable Lieb-Liniger-McGuire (LLMG) model, with an energy-independent strength, forbids all chemical processes, such as three-atom association and diatom dissociation, as well as reflection in atom-diatom collisions. The resonant case is analyzed by a numerical solution of the Faddeev equations. The results demonstrate that as the internal symmetry of the LLMG model is lifted, reflection and chemical reactions become allowed and may be observed in experiments.

DOI
10.1103/physrevlett.96.163201

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1. Highlight “short-ranged,” “dilute,” and “low-energy” as three main features of interactions between ultracold atoms. 2. Introduce the important concept of the phase shift. 3. Introduce the $s$-wave scattering length as a universal parameter describing the low-energy interaction between ultracold atoms. 4. Discuss the relation between divergent scattering length, low-energy bound state, and jump of phase shift. 5. Discuss the relation between the scattering length and the scattering amplitude. 6. Discuss under what condition a positive scattering length describes repulsive interaction. 7. Discuss the condition when an algebraically decayed potential can be treated as a finite range one. 8. Introduce two types of zero-range single-channel potentials to capture the universal low-energy $s$-wave interaction between ultracold atoms. 9. Introduce the concept of renormalization condition and renormalizable theory. 10. Discuss how the spin rotational symmetry imposes constraints on interaction form for both alkali-metal and alkaline-earth-metal atoms. 11. Introduce Feshbach resonance as an important tool to tune scattering length. 12. Compare the two-channel Feshbach resonance with the single-channel shape resonance and compare the wide and the narrow resonances. 13. Introduce a zero-range two-channel model. 14. Introduce the confinement-induced resonance to tune interaction strength by an external potential. 15. Summarize three key conditions for a Feshbach resonance, and unify the optical Feshbach resonance, the orbital Feshbach resonance, and the confinement-induced resonance all in terms of these three conditions. 16. Introduce the Efimov effect as an important three-body effect at the vicinity of the two-body scattering resonance. 17. Highlight the symmetry aspect of the Efimov effect. 18. Discuss various connections between few-body and many-body physics. 19. Illustrate that few-body calculation can be used to determine properties of many-body systems by using high-temperature expansion as an example.

Cambridge University Press eBooks•Jan 30, 2021•0 citations
Three-body collisions of ultracold identical Bose atoms under tight cylindrical confinement are analyzed. A Feshbach resonance in two-body collisions is described by a two-channel zero-range interaction. Elimination of the closed channel in the three-body problem reduces the interaction to a one-channel zero-range one with an energy-dependent strength. The related integrable Lieb-Liniger-McGuire (LLMG) model, with an energy-independent strength, forbids all chemical processes, such as three-atom association and diatom dissociation, as well as reflection in atom-diatom collisions. The resonant case is analyzed by a numerical solution of the Faddeev equations. The results demonstrate that as the internal symmetry of the LLMG model is lifted, reflection and chemical reactions become allowed and may be observed in experiments.
Bound states and collisions of atoms with two-channel two-body interactions in harmonic waveguides are analyzed. The closed-channel contributions to two-atom bound states become dominant in the case of a weak resonance. At low energies and values of the nonresonant scattering length the problem can be approximated by a one-dimensional resonant model. The three-body problem becomes nonintegrable and the properties of triatomic molecules become different from those predicted by the integrable Lieb-Liniger-McGuire model.
Inelastic collisions of ultracold atoms or molecules are analyzed using very general arguments. In free space, the deactivation rate can be enhanced or suppressed together with the scattering length of the corresponding elastic collision via a Feshbach resonance, and by interference of deactivation of the closed and open channels. In reduced dimensional geometries, the deactivation rate decreases with decreasing collision energy and does not increase with resonant elastic scattering length. This has broad implications; e.g., stabilization of molecules in a strongly confining two-dimensional optical lattice, since collisional decay of excited states due to inelastic collisions is suppressed. The relation of our results to the Lieb-Liniger model for bosonic atoms is addressed.
In this thesis, we investigated the physics of two- and three-dimensional ultra cold Bose gases in the strongly interacting regime at zero temperature. This regime can be experimentally accessed using a Feshbach resonance. We applied a self-consistent diagrammatic approach to determine the chemical potential of three-dimensional Bose gases for a wide range of interaction values. We showed that such strongly interacting Bose gases become unstable towards the formation of molecules at a finite positive scattering length. In fact, the interaction between atoms becomes effectively attractive and the system looses its metastability before reaching the unitary limit. We also found that such systems are nearly fermionized close to the instability point. Near this critical point, the chemical potential reaches a maximum and the contribution to the system energy due to three-body forces is estimated to be only a few percent. We also studied the same system using a self-consistent renormalization group method. This approach confirms the existence of an instability point towards the formation of molecules as well as fermionization. We showed that the instability and accompanying maximum are precursors of the sign change of the effective two-body interaction strength from repulsive to attractive near resonance. In addition, we examined the physics of two-dimensional Bose gases near resonance using a similar self-consistent diagrammatic approach as the one introduced for three-dimensional Bose gases. We demonstrated that a competition between three-body attractive interactions and two-body repulsive forces results in the chemical potential of two-dimensional Bose gases to exhibit a maximum at a critical scattering length beyond which these quantum gases possess a negative compressibility. For larger scattering lengths, the increasingly prominent role played by three-body attractive interactions leads to an onset instability at a second critical value. The three-body effects studied for these systems are universal, fully characterized by the effective two-dimensional scattering length and are, in comparison to the three-dimensional case, independent of three-body ultraviolet physics.
1. Highlight “short-ranged,” “dilute,” and “low-energy” as three main features of interactions between ultracold atoms. 2. Introduce the important concept of the phase shift. 3. Introduce the sss-wave scattering length as a universal parameter describing the low-energy interaction between ultracold atoms. 4. Discuss the relation between divergent scattering length, low-energy bound state, and jump of phase shift. 5. Discuss the relation between the scattering length and the scattering amplitude. 6. Discuss under what condition a positive scattering length describes repulsive interaction. 7. Discuss the condition when an algebraically decayed potential can be treated as a finite range one. 8. Introduce two types of zero-range single-channel potentials to capture the universal low-energy sss-wave interaction between ultracold atoms. 9. Introduce the concept of renormalization condition and renormalizable theory. 10. Discuss how the spin rotational symmetry imposes constraints on interaction form for both alkali-metal and alkaline-earth-metal atoms. 11. Introduce Feshbach resonance as an important tool to tune scattering length. 12. Compare the two-channel Feshbach resonance with the single-channel shape resonance and compare the wide and the narrow resonances. 13. Introduce a zero-range two-channel model. 14. Introduce the confinement-induced resonance to tune interaction strength by an external potential. 15. Summarize three key conditions for a Feshbach resonance, and unify the optical Feshbach resonance, the orbital Feshbach resonance, and the confinement-induced resonance all in terms of these three conditions. 16. Introduce the Efimov effect as an important three-body effect at the vicinity of the two-body scattering resonance. 17. Highlight the symmetry aspect of the Efimov effect. 18. Discuss various connections between few-body and many-body physics. 19. Illustrate that few-body calculation can be used to determine properties of many-body systems by using high-temperature expansion as an example.