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arXiv:physics/0509181 · Optics and Spectroscopy

A saturable absorber, coherent population oscillations, and slow light

Valerii S Zapasskii, G. G. Kozlov

Published Mar 1, 2006• 46 citations
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Abstract

The paper presents a critical analysis of publications on one of the methods of creating so-called slow light (light with an anomalously low group velocity) arising due to a high steepness of the refractive index dispersion curve. The method employs, for this purpose, the effect of coherent population oscillations accompanied by burning of a narrow spectral hole in the homogeneously broadened absorption spectrum. The interpretation of the experimental data in the studies under consideration is based on the analysis of the response of a nonlinear medium to a low-frequency intensity modulation of the propagating light beam. We show that all the observations of these papers can be easily interpreted in the framework of the simplest model of a saturable absorber and have nothing to do with the hole burning effect or group velocity reduction.

DOI
10.1134/s0030400x06030192

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The paper presents a critical analysis of publications on one of the methods of creating so-called slow light (light with an anomalously low group velocity) arising due to a high steepness of the refractive index dispersion curve. The method employs, for this purpose, the effect of coherent population oscillations accompanied by burning of a narrow spectral hole in the homogeneously broadened absorption spectrum. The interpretation of the experimental data in the studies under consideration is based on the analysis of the response of a nonlinear medium to a low-frequency intensity modulation of the propagating light beam. We show that all the observations of these papers can be easily interpreted in the framework of the simplest model of a saturable absorber and have nothing to do with the hole burning effect or group velocity reduction.
A critical review of experimental studies of the so-called 'slow light' arising due to anomalously high steepness of the refractive index dispersion under conditions of electromagnetically induced transparency or coherent population oscillations is presented. It is shown that a considerable amount of experimental evidence for observation of the 'slow light' is not related to the low group velocity of light and can be easily interpreted in terms of a standard model of interaction of light with a saturable absorber.
A critical review of experimental studies of the so-called 'slow light' arising due to anomalously high steepness of the refractive index dispersion under conditions of electromagnetically induced transparency or coherent population oscillations is presented. It is shown that a considerable amount of experimental evidence for observation of the 'slow light' is not related to the low group velocity of light and can be easily interpreted in terms of a standard model of interaction of light with a saturable absorber.
A comparative analysis of two approaches to the description of the light modulation pulse in a saturable absorber is presented. According to the simplest model, the delay of the optical pulse is a result of the distortion of its shape due to the self-modulation of absorption in the nonlinear medium. The second model of the effect, arisen at the beginning of our century, relates the pulse delay to the so-called “slow light,” attributing this delay to the group velocity reduction under the condition of coherent oscillations of the population. It is shown that the data of all known experiments on the light pulse delay in saturable absorbers can be comprehensively described in terms of the simplest model of saturable absorber and do not require invoking the effect of population coherent oscillations with spectral hole-burning and anomalous modifications of the light group velocity. It is concluded that the effect of the group velocity reduction under the condition of population coherent oscillations has not received so far any experimental confirmation, and the assertions about real observation of the slow light based on this mechanism are unfounded.
It is shown that the effect of hole-burning under conditions of coherent population oscillations as well as the light pulse delay in a saturable absorber (a modification of the so-called slow light effect) can be interpreted, in a comprehensive way, in terms of the intensity spectrum of the light and intensity-related susceptibility of the medium. The physical content of these effects is illustrated by a simple electric circuit with a non-linear resistor which realizes a full analog of the saturable absorber. In this case the effect of hole-burning in the absorption spectrum of the medium is converted into the effect of hole-burning in the frequency dependence of resistance of the resistor and the effect of slow light into the effect of slow current.
Quantitative analysis of slow light experiments utilising coherent population oscillation (CPO) in a range of saturably absorbing media, including ruby and alexandrite, Er 3+ :Y 2 SiO 5 , bacteriorhodopsin, semiconductor quantum devices and erbium-doped optical fibres, shows that the observations may be more simply interpreted as saturable absorption phenomena. A basic two-level model of a saturable absorber displays all the effects normally associated with slow light, namely phase shift and modulation gain of the transmitted signal, hole burning in the modulation frequency spectrum and power broadening of the spectral hole, each arising from the finite response time of the non-linear absorption. Only where hole-burning in the optical spectrum is observed (using independent pump and probe beams), or pulse delays exceeding the limits set by saturable absorption are obtained, can reasonable confidence be placed in the observation of slow light in such experiments. Superluminal (“fast light”) phenomena in media with reverse saturable absorption (RSA) may be similarly explained.
Quantitative analysis of slow light experiments utilising coherent population oscillation (CPO) in a range of saturably absorbing media, including ruby and alexandrite, Er3+:Y2SiO5, bacteriorhodopsin, semi-conductor quantum devices and erbium doped optical fibres, shows that the observations may be more simply interpreted as saturable absorption phenomena. A basic two-level model of a saturable absorber displays all the effects normally associated with slow light, namely phase shift and modulation gain of the transmitted signal, hole burning in the modulation frequency spectrum and power broadening of the spectral hole, arising from the finite response time of the non-linear absorption. Only where hole-burning in the optical spectrum is observed (using independent pump and probe beams), or pulse delays exceeding the limits set by saturable absorption are obtained, can reasonable confidence be placed in the observation of slow light in such experiments. Superluminal ('fast light') phenomena in media with reverse saturable absorption (RSA) may be similarly explained.