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arXiv:physics/0202059 · Physical Review Letters

Specular Reflection of Matter Waves from a Rough Mirror

V. Savalli, D. Stevens, Jérôme Estève, P. D. Featonby, Vincent Josse, Nathalie Westbrook, Christoph Ira Westbrook, Alain Aspect

Published Jun 10, 2002• 26 citations
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Abstract

We present a high resolution study of the specularity of the atomic reflection from an evanescent wave mirror using velocity selective Raman transitions. We observed a double structure in the velocity distribution after reflection: a peak consistent with specular reflection and a diffuse reflection pedestal whose contribution decreases rapidly with increasing detuning. The diffuse reflection is due to two distinct effects: spontaneous emission in the evanescent wave and roughness in the evanescent wave potential whose amplitude is smaller than the de Broglie wavelength of the reflected atoms.

DOI
10.1103/physrevlett.88.250404

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AIP conference proceedings•Jan 1, 2008•0 citations
We present a high resolution study of the specularity of the atomic reflection from an evanescent wave mirror using velocity selective Raman transitions. We observed a double structure in the velocity distribution after reflection: a peak consistent with specular reflection and a diffuse reflection pedestal whose contribution decreases rapidly with increasing detuning. The diffuse reflection is due to two distinct effects: spontaneous emission in the evanescent wave and roughness in the evanescent wave potential whose amplitude is smaller than the de Broglie wavelength of the reflected atoms.
We present a theoretical analysis of the influence of surface roughness on the atomic reflection from an evanescent wave mirror. In our calculations we assume that light scattered at the rough dielectric surface interferes with the evanescent wave, creating a rough potential that scatters the atoms. We calculate the probability of diffuse reflection and the momentum distribution of the scattered atoms with a statistical model for the rough surface. The atomic reflection is diffuse rather than specular if the surface roughness is comparable to the wavelength of the incident atoms. We discuss the spatial coherence of the reflected matter waves. We indicate how to generalize our treatment to the case of multilevel atoms.
Summary form only given. Evanescent wave atomic mirrors have been shown to be very sensitive to the surface roughness of the glass substrate on which the evanescent wave is formed. Non-specular reflection of slow atoms at normal incidence has been observed for surface roughness as low as 0.1 nm. We interpret this behaviour in terms of diffraction of the atomic De Broglie wave on the modulated potential created by the interference of the evanescent wave with light scattered by the rough surface. However these experiments could not separate the specular peak of reflected atoms from the diffuse part. We have developed a new method to measure the velocity distribution of the atoms after the bounce with a much better resolution, using Raman transitions. Two phase locked counterpropagating laser beams induce a Raman transition between the ground state hyperfine levels of the /sup 85/Rb atoms falling from a magneto-optical trap. The resonance condition is only fulfilled for atoms with a transverse velocity controlled by the interaction time between the atoms and the beams. These velocity selected atoms bounce on the mirror and their velocity distribution after reflection can be measured using the same Raman beams, by scanning their difference in frequency.
We tested the specularity of the ref lection of slow atoms from an evanescent-wave mirror at normal incidence. In two of the three prisms that we tested the atoms were ref lected diffusely. This nonspecular ref lection appears to be correlated with the rms roughness of the surface supporting the evanescent wave. Only the highest quality surface (rms roughness of the order of 0.1 nm) leads to specular ref lection. This discovery imposes stringent limits on the use of these mirrors in atomic-optics experiments.
The reflection of metastable argon atoms from evanescent waves produced by total internal reflection and surface-plasmon excitation is investigated. We study the departure from ideal specular reflection by comparing our experimental results with a Monte Carlo simulation of the reflection process. The observed broadening of the reflection beam was found to be caused predominantly by fluctuations of the diple force. We show that the surface plasmon produces significant enhancement of the evanescent-wave intensity without degrading the quality of reflection. In addition, the number of spontaneous emissions occurring during the reflection process was investigated by comparing the reflectivity of evanescent-wave mirrors based on open and closed transitions in argon. An open-transition mirror selectively reflects atoms which do not undergo spontaneous emission. For a large detuning, the average number of spontaneous emissions for reflected atoms was 0.11.
A research project at the “Laboratoire d’électronique quantique” consists in a theoretical study of the reflection and diffraction phenomena via an atomic mirror. This poster presents the principle of an atomic mirror. Many groups in the world have constructed this type of atom optics experiments such as in Paris‐Orsay‐Villetaneuse (France), Stanford‐Gaithersburg (USA), Munich‐Heidelberg (Germany), etc. A laser beam goes into a prism with an incidence bigger than the critical incidence. It undergoes a total reflection on the plane face of the prism and then exits. The transmitted resulting wave out of the prism is evanescent and repulsive as the frequency detuning of the laser beam compared to the atomic transition δ = ωL−ω0 is positive. The cold atomic sample interacts with this evanescent wave and undergoes one or more elastic bounces by passing into backward points in its trajectory because the atoms’ kinetic energy (of the order of the μeV) is less than the maximum of the dipolar potential barrier ℏΩ2/Δ where Ω is the Rabi frequency [1]. In fact, the atoms are cooled and captured in a magneto‐optical trap placed at a distance of the order of the cm above the prism surface. The dipolar potential with which interact the slow atoms is obtained for a two level atom in a case of a dipolar electric transition (D2 Rubidium transition at a wavelength of 780nm delivered by a Titane‐Saphir laser between a fundamental state Jf = l/2 and an excited state Je = 3/2). This potential is corrected by an attractive Van der Waals term which varies as 1/z3 in the Lennard‐Jones approximation (typical atomic distance of the order of λ0/2π where λ0 is the laser wavelength) and in 1/z4 if the distance between the atom and its image in the dielectric is big in front of λ0/2π. This last case is obtained in a quantum electrodynamic calculation by taking into account an orthornormal base [2]. We’ll examine the role of spontaneous emission for which the rate is inversely proportional to the detuning δ and is responsible of the non specular aspect of the atomic reflection (atomic diffusion). In the contrary, we note that the specularity of the reflection preserve the coherence of the atomic wave packet. The atoms will constitute a probe of the rugosity of the prism surface which can be imperfect or super‐polished.