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arXiv:hep-th/9501040 · Talk given at

Correlations, Decoherence, Dissipation, and Noise in Quantum Field Theory

Esteban Calzetta, B. L. Hu

Published Jan 12, 1995• 24 citations
arXivHTMLPDF

Abstract

The statistical mechanical properties of interacting quantum fields in terms of the dynamics of the correlation functions are investigated. We show how the Dyson - Schwinger equations may be derived from a formal action functional, the n-particle irreducible ($nPI, n \to \infty$) or the `master' effective action. It is related to the decoherence functional between histories defined in terms of correlations. Upon truncation of the Dyson - Schwinger hierarchy at a certain order, the master effective action becomes complex, its imaginary part arising from the higher order correlation functions, the fluctuations of which we define as the correlation noises of that order. Decoherence of correlation histories via these noises gives rise to classical stochastic histories %driven by the flucutations of these higher correlation functions. Ordinary quantum field theory corresponds to taking the lowest order functions, usually the mean field and the 2-point functions. As such, our reasoning shows that it is an effective theory which can be intrinsically dissipative. The relation of loop expansion and correlation order as well as the introduction of an arrow of time from the choice of boundary conditions are expounded with regard to the origin of dissipation in quantum fields. Relation with critical phenomena, quantum transport, molecular hydrodynamics and potential applications to quantum gravity, early universe processes and black hole physics are mentioned.

DOI
10.48550/arxiv.hep-th/9501040

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The thesis comprises two major themes of quantum statistical dynamics. One is the development of quantum dissipation theory (QDT). It covers the establishment of some basic relations of quantum statistical dynamics, the construction of several nonequivalent complete second-order formulations, and the development of exact QDT. Another is related to the applications of quantum statistical dynamics to a variety of research fields. In particular, unconventional but novel theories of the electron transfer in Debye solvents, quantum transport, and quantum measurement are developed on the basis of QDT formulations. The thesis is organized as follows. In Chapter 1, we present some background knowledge in relation to the afore-mentioned two themes of this thesis. The key quantity in QDT is the reduced density operator ρ(t) ≡ trBρT(t); i.e., the partial trace of the total system and bath composite ρT(t) over the bath degrees of freedom. 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The interplay between system-bath interaction strength, non-Markovian property, and the required level of hierarchy is also studied with the aid of simple spin-boson systems, together with the three proposed schemes to truncate the infinite hierarchy. In Chapter 5, we develop a nonperturbative theory of electron transfer (ET) in Debye solvents. The resulting exact and analytical rate expression is constructed on the basis of the aforementioned continued fraction Liouville-space Green's func-tion formalism, together with the Dyson equation technique. Not only does it re-cover the celebrated Marcus' inversion and Kramers' turnover behaviors, the new theory also shows some distinct quantum solvation effects that can alter the ET mechanism. Moreover, the present theory predicts further for the ET reaction ther-modynamics, such as equilibrium Gibbs free-energy and entropy, some interesting solvent-dependent features that are calling for experimental verification. 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This will be carried out by reducing the many-particle (Fermion or Boson) QDT to a single-particle one by exploring, e.g. the Wick's contraction theorem. It also results in a time-dependent density func-tional theory (TDDFT) for transport through complex large-scale (e.g. molecules) systems. Primary results of the TDDFT-QDT are reported. In Chapter 10, we summary the thesis, and comment and remark on the future work on both the theoretical and application aspects of QDT.

•Jan 1, 2006•0 citations
The statistical mechanical properties of interacting quantum fields in terms of the dynamics of the correlation functions are investigated. We show how the Dyson - Schwinger equations may be derived from a formal action functional, the n-particle irreducible (nPI,n→∞nPI, n \to \inftynPI,n→∞) or the `master' effective action. It is related to the decoherence functional between histories defined in terms of correlations. Upon truncation of the Dyson - Schwinger hierarchy at a certain order, the master effective action becomes complex, its imaginary part arising from the higher order correlation functions, the fluctuations of which we define as the correlation noises of that order. Decoherence of correlation histories via these noises gives rise to classical stochastic histories %driven by the flucutations of these higher correlation functions. Ordinary quantum field theory corresponds to taking the lowest order functions, usually the mean field and the 2-point functions. As such, our reasoning shows that it is an effective theory which can be intrinsically dissipative. The relation of loop expansion and correlation order as well as the introduction of an arrow of time from the choice of boundary conditions are expounded with regard to the origin of dissipation in quantum fields. Relation with critical phenomena, quantum transport, molecular hydrodynamics and potential applications to quantum gravity, early universe processes and black hole physics are mentioned.
The aim of this paper is twofold: to probe the statistical mechanical properties of interacting quantum fields, and to provide a field theoretical justification for a stochastic source term in the Boltzmann equation. We start with the formulation of quantum field theory in terms of the set of Schwinger-Dyson equations for the correlation functions, which we describe by a closed-time-path master $(n=\ensuremath{\infty}\mathrm{PI})$ effective action. When the hierarchy is simply truncated to a certain order, one obtains the usual closed system of correlation functions up to that order, and from the nPIn\mathrm{PI}nPI effective action, a set of time-reversal invariant equations of motion. (This is the Dyson equation, the quantum field theoretical parallel of the collisionless Boltzmann equation.) But when the effect of the higher order correlation functions is included through a causal factorization condition (such as the molecular chaos assumption in Boltzmann's theory) called slaving, the dynamics of the lower order correlations shows dissipative features, as familiar in the usual (dissipative yet noiseless) Boltzmann equation, the field-theoretical version of which being the dissipative Dyson equations. We show that a fluctuation-dissipation relation should exist for such effectively open systems, and use this fact to show that a stochastic term, which explicitly introduces quantum fluctuations in the lower order correlation functions, necessarily accompanies the dissipative term. This leads to a stochastic Dyson equation, which is the quantum field theoretic parallel of the classical Boltzmann-Langevin equation, encompassing both the dissipative and stochastic dynamics of correlation functions.
We use a λΦ 4 scalar quantum field theory to illustrate a new approach to the study of quantum to classical transition. In this approach, the decoherence functional is employed to assign probabilities to consistent histories defined in terms of correlations among the fields at separate points, rather than the field itself. We present expressions for the quantum amplitudes associated with such histories, as well as for the decoherence functional between two of them. The dynamics of an individual consistent history may be described by a Langevintype equation, which we derive. Dedicated to Professor Brill on the occasion of his sixtieth birthday, August 1993 Introduction Interpretations of Quantum Mechanics and Paradigms of Statistical Mechanics This paper attempts to bring together two basic concepts, one from the foundations of statistical mechanics and the other from the foundations of quantum mechanics, for the purpose of addressing two basic issues in physics: the quantum to classical transition, and the quantum origin of stochastic dynamics. Both issues draw in the interlaced effects of dissipation, decoherence, noise, and fluctuation. A central concern is the role played by coarse-graining —the naturalness of its choice, the effectiveness of its implementation and the relevance of its consequences.
In this sequel paper we explore how macroscopic quantum phenomena can be measured or understood from the behavior of quantum correlations which exist in a quantum system of many particles or components and how the interaction strengths change with energy or scale, under ordinary situations and when the system is near its critical point. We use the nPI (master) effective action related to the Boltzmann-BBGKY / Schwinger-Dyson hierarchy of equations as a tool for systemizing the contributions of higher order correlation functions to the dynamics of lower order correlation functions. Together with the large N expansion discussed in our first paper(MQP1) we explore 1) the conditions whereby an H-theorem is obtained, which can be viewed as a signifier of the emergence of macroscopic behavior in the system. We give two more examples from past work: 2) the nonequilibrium dynamics of N atoms in an optical lattice under the large N\cal NN (field components), 2PI and second order perturbative expansions, illustrating how N and N\cal NN enter in these three aspects of quantum correlations, coherence and coupling strength. 3) the behavior of an interacting quantum system near its critical point, the effects of quantum and thermal fluctuations and the conditions under which the system manifests infrared dimensional reduction. We also discuss how the effective field theory concept bears on macroscopic quantum phenomena: the running of the coupling parameters with energy or scale imparts a dynamical-dependent and an interaction-sensitive definition of `macroscopia'.
In this paper we are interested in studying coarse graining in field theories using the language of quantum open systems. Motivated by the ideas of Hu and Calzetta on correlation histories we employ the Zwanzig projection technique to obtain evolution equations for relevant observables in self-interacting scalar field theories. Our coarse-graining operation consists in concentrating solely on the evolution of the correlation functions of degree less than n,n,n, a treatment which corresponds to the familiar truncation of the BBKGY hierarchy at the nnnth level. We derive the equations governing the evolution of mean-field and two-point functions thus identifying the terms corresponding to dissipation and noise. We discuss possible applications of our formalism, the emergence of classical behavior, and the connection to the decoherent histories framework.
It is well known that some quantum and statistical fluctuations of a quantum field may be recovered by adding suitable stochastic sources to the mean field equations derived from the Schwinger–Keldysh (closed-time path) effective action. In this paper we show that this method can be extended to higher correlations and higher ( n -particle irreducible) effective actions. As an example, we investigate third- and fourth-order correlations by adding stochastic sources to the Schwinger–Dyson equations derived from the 2-particle irreducible effective action. This method is a simple way to investigate the nonlinear dynamics of quantum fluctuations.
The thesis comprises two major themes of quantum statistical dynamics. One is the development of quantum dissipation theory (QDT). It covers the establishment of some basic relations of quantum statistical dynamics, the construction of several nonequivalent complete second-order formulations, and the development of exact QDT. Another is related to the applications of quantum statistical dynamics to a variety of research fields. In particular, unconventional but novel theories of the electron transfer in Debye solvents, quantum transport, and quantum measurement are developed on the basis of QDT formulations. The thesis is organized as follows. In Chapter 1, we present some background knowledge in relation to the afore-mentioned two themes of this thesis. The key quantity in QDT is the reduced density operator ρ(t) ≡ trBρT(t); i.e., the partial trace of the total system and bath composite ρT(t) over the bath degrees of freedom. QDT governs the evolu-tion of reduced density operator, where the effects of bath are treated in a quantum statistical manner. In principle, the reduced density operator contains all dynam-ics information of interest. However, the conventional quantum transport theory is formulated in terms of nonequilibrium Green's function. The newly emerging field of quantum measurement in relation to quantum information and quantum computing does exploit a sort of QDT formalism. Besides the background of the relevant theoretical development, some representative experiments on molecular nanojunctions are also briefly discussed. In Chapter 2, we outline some basic (including new) relations that highlight several important issues on QDT. The content includes the background of nonequi-librium quantum statistical mechanics, the general description of the total compos-ite Hamiltonian with stochastic system-bath interaction, a novel parameterization scheme for bath correlation functions, a newly developed exact theory of driven Brownian oscillator (DBO) systems, and its closely related solvation mode trans-formation of system-bath coupling Hamiltonian in general. The exact QDT of DBO systems is also used to clarify the validity of conventional QDT formulations that involve Markovian approximation. In Chapter 3, we develop three nonequivalent but all complete second-order QDT (CS-QDT) formulations. Two of them are of the conventional prescriptions in terms of time-local dissipation and memory kernel, respectively. The third one is called the correlated driving-dissipation equations of motion (CODDE). This novel CS-QDT combines the merits of the former two for its advantages in both the application and numerical implementation aspects. Also highlighted is the importance of correlated driving-dissipation effects on the dynamics of the reduced system. In Chapter 4, we construct an exact QDT formalism via the calculus on path integrals. The new theory aims at the efficient evaluation of non-Markovian dis-sipation beyond the weak system-bath interaction regime in the presence of time-dependent external field. By adopting exponential-like expansions for bath corre-lation function, hierarchical equations of motion formalism and continued fraction Liouville-space Green's function formalism are established. The latter will soon be used together with the Dyson equation technique for an efficient evaluation of non-perturbative reduced density matrix dynamics. The interplay between system-bath interaction strength, non-Markovian property, and the required level of hierarchy is also studied with the aid of simple spin-boson systems, together with the three proposed schemes to truncate the infinite hierarchy. In Chapter 5, we develop a nonperturbative theory of electron transfer (ET) in Debye solvents. The resulting exact and analytical rate expression is constructed on the basis of the aforementioned continued fraction Liouville-space Green's func-tion formalism, together with the Dyson equation technique. Not only does it re-cover the celebrated Marcus' inversion and Kramers' turnover behaviors, the new theory also shows some distinct quantum solvation effects that can alter the ET mechanism. Moreover, the present theory predicts further for the ET reaction ther-modynamics, such as equilibrium Gibbs free-energy and entropy, some interesting solvent-dependent features that are calling for experimental verification. In Chapter 6, we discuss the constructed QDTs, in terms of their unified math-ematical structure that supports a linear dynamics space, and thus facilitates their applications to various physical problems. The involving details are exemplified with the CODDE form of QDT. As the linear space is concerned, we identify the Schrödinger versus Heisenberg picture and the forward versus backward propaga-tion of the reduced, dissipative Liouville dynamics. For applications we discuss the reduced linear response theory and the optimal control problems, in which the correlated effects of non-Markovian dissipation and field driving are shown to be important. In Chapter 7, we turn to quantum transport, i.e. electric current through molecular or mesoscopic systems under finite applied voltage. By viewing the nonequilibrium transport setup as a quantum open system, we develop a reduced-density-matrix approach to quantum transport. The resulting current is explicitly expressed in terms of the molecular reduced density matrix by tracing out the degrees of freedom of the electrodes at finite bias and temperature. We propose a conditional quantum master equation theory, which is an extension of the conven-tional (or unconditional) QDT by tracing out the well-defined bath subsets indi-vidually, instead of the entire bath degrees of freedom. Both the current and the noise spectrum can be conveniently analyzed in terms of the conditional reduced density matrix dynamics. By far, the QDT (including the conditional one) has only been exploited in a second-order form. A self-consistent Born approximation for the system-electrode coupling is further proposed to recover all existing nonlinear current-voltage behaviors including the nonequilibrium Kondo effect. Transport theory based on the exact QDT formalism will be developed in future. In Chapter 8, we study the quantum measurement of a qubit with a quantum-point-contact detector. On the basis of a unified quantum master equation (a form of QDT), we study the measurement-induced relaxation and dephasing of the qubit . Our treatment pays particular attention on the detailed-balance relation, which is a consequence of properly accounting for the energy exchange between the qubit and detector during the measurement process. We also derive a conditional quantum master equation for quantum measurement in general, and study the readout characteristics of the qubit measurement. Our theory is applicable to the quantum measurement at arbitrary voltage and temperature. A number of remarkable new features are found and highlighted in concern with their possible relevance to future experiments. In Chapter 9, we discuss the further development of QDT, aiming at an effi-cient evaluation of many-electron systems. This will be carried out by reducing the many-particle (Fermion or Boson) QDT to a single-particle one by exploring, e.g. the Wick's contraction theorem. It also results in a time-dependent density func-tional theory (TDDFT) for transport through complex large-scale (e.g. molecules) systems. Primary results of the TDDFT-QDT are reported. In Chapter 10, we summary the thesis, and comment and remark on the future work on both the theoretical and application aspects of QDT.