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arXiv:cond-mat/9909043 · Physical review. B, Condensed matter

BCS to Bose crossover in anisotropic superconductors

J. P. Wallington, James F. Annett

Published Jan 1, 2000• 26 citations
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Abstract

In this work we use functional integral techniques to examine the nearest-neighbor attractive Hubbard model on a quasi-two-dimensional lattice. It is a simple phenomenological model for the high-${T}_{c}$ cuprates that allows both extended (nonlocal) s- and d-wave singlet superconductivity as well as mixed symmetry states. The Hartree-Gor'kov mean-field theory of the model has a finite-temperature phase diagram which shows a transition from pure s-wave to pure d-wave superconductivity, via a mixed symmetry $s+id$ state, as a function of doping. Including Gaussian fluctuations we examine the crossover from weak-coupling BCS superconductivity to the strong-coupling Bose-Einstein condensation of composite s- or d-wave bosons and comment on the origin and symmetry of the pseudogap.

DOI
10.1103/physrevb.61.1433

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In this work we use functional integral techniques to examine the nearest-neighbor attractive Hubbard model on a quasi-two-dimensional lattice. It is a simple phenomenological model for the high-Tc{T}_{c}Tc​ cuprates that allows both extended (nonlocal) s- and d-wave singlet superconductivity as well as mixed symmetry states. The Hartree-Gor'kov mean-field theory of the model has a finite-temperature phase diagram which shows a transition from pure s-wave to pure d-wave superconductivity, via a mixed symmetry s+ids+ids+id state, as a function of doping. Including Gaussian fluctuations we examine the crossover from weak-coupling BCS superconductivity to the strong-coupling Bose-Einstein condensation of composite s- or d-wave bosons and comment on the origin and symmetry of the pseudogap.
We consider a lattice version of the ``negative-U′′U''U′′ Hubbard model in three dimensions, to study the crossover from a superconducting phase transition (dominated by phase fluctuation) to a regime where the amplitude of the superconducting order parameter controls the critical temperature. Starting from a fermionic Hamiltonian, we give a microscopic derivation of the effective action in terms of the relevant physical fields: the modulus and phase of the superconducting order parameter. Furthermore, by employing to the resulting coarse--grained quantum XY\mathrm{XY}XY model the phase fluctuation algebra between number and phase operators (given by the Euclidean group E2),{E}_{2}),E2​), we map the ``phase-only'' action onto a solvable quantum spherical model. We establish the self--consistent theory (involving both fermionic and bosonic degrees of freedom), and calculate the superconducting phase coherence transition temperature Tc{T}_{c}Tc​ as a function of the coupling strength ∣U∣,|U|,∣U∣, exhibiting a maximum where the behavior crosses over from BCS to Bose-Einstein (BE) condensation. We examine a pseudogap in the normal state which emerges naturally as a precursor of superconductivity at the second characteristic temperature Tg{T}_{g}Tg​ due to a state with bound pairs but without long--range phase coherence. Furthermore, we demonstrate that the reduced gaps of the model $2{\ensuremath{\Delta}}_{0}{/k}_{B}{T}_{g}\ensuremath{\sim}4$ is almost independent on the pairing strength ∣U∣/t,|U|/t,∣U∣/t, whereas $2{\ensuremath{\Delta}}_{0}{/k}_{B}{T}_{c}$ increases with increasing ∣U∣|U|∣U∣---in striking analogy with the phenomenology of the high--temperature cuprate superconductors when interpreted in terms of the BCS-BC crossover scenario.
In this paper we address the behavior of the superfluid transition temperature Tc{T}_{c}Tc​ in the attractive Hubbard model. The attractive Hubbard model can be regarded as the generalization of the BCS to Bose-Einstein condensation (BEC) crossover to a lattice and, as such, may have implications for future optical lattice studies. Nevertheless, the BEC limit of the Hubbard model is very different from that of the better-studied Fermi gases, owing to the strong intersite repulsion between pairs. Here we address systematically the effects of pairing fluctuations for all filling fractions over the entire range of attractive interaction strength. A central conclusion of our work is that in a lattice, around half filling, the smooth evolution from the BCS to the BEC limits is interrupted: Tc{T}_{c}Tc​ vanishes when the system approaches the bosonic regime with increasing interaction strength. We suggest that this interruption of crossover may signal a quantum critical transition to another form of superfluid not continuously connected to a BCS-like phase. A simple variational ansatz for an alternate ground state in this more strongly coupled superfluid is presented. A generalization of the (sss-wave) Hubbard model to ddd-wave pairing allows us to address issues of relevance to high-Tc{T}_{c}Tc​ superconductivity. The phase diagram (representing the pairing or pseudogap onset temperature T∗{T}^{*}T∗ and Tc{T}_{c}Tc​) shows that here too one observes a vanishing of Tc{T}_{c}Tc​ when T∗{T}^{*}T∗ becomes sufficiently large. Given this predicted breakdown of the crossover, and given the striking similarity to features of the cuprate phase diagram, we suggest that future experiments on ultracold fermions in optical lattices should not be exclusively limited to the repulsive Hubbard model, but should address the attractive model in order to elucidate features of high-temperature superconductivity.
With the pseudogap in cuprate superconductors in mind, we study an attractive Hubbard model on the square lattice, in which the mechanism of superconductivity undergoes a crossover at |Uco|/t from a BCS type to a Bose-Einstein condensation type, as the interaction strength |U|/t increases. Correspondingly, for |U|>|Uco|, a normatate, realized for T>Tc, is considered to exhibit gapped behavior. We try to construct such a state and study its properties using a variational Monte Carlo method, which treats the local correlation accurately and can connect the weak-and strong-correlation limits continuously. We introduce an intersite correlation factor between antiparallel spins in nearest-neighbor sites, in addition to the onsite (Gutzwiller) projection. This factor brings about a first-order transition from a metal to a spin-gapped phase at |U=|Uc|=W (bandwidth). For |U|>|Uc|, a gap opens in the spin degree of freedom, whereas the charge sector remains gapless. In this phase, conductivity is caused by a hopping of doublons.
We model fermions with an attractive interaction in an optical lattice with a single-band Hubbard model away from half-filling with on-site attraction UUU and nearest neighbor hopping ttt. Our goal is to understand the crossover from BCS superfluidity in the weak attraction limit to the BEC of molecules in the strong attraction limit, with particular emphasis on how this crossover in an optical lattice differs from the much better studied continuum problem. We use a large-NNN theory with Sp(2N) symmetry to study the fluctuations beyond mean field theory. At T=0, we calculate across the crossover various observables, including chemical potential, gap, ground state energy, speed of sound and compressibility. The superfluid density nsn_sns​ is found to have non-trivial U/tU/tU/t dependence in this lattice system. We show that the transition temperature TcT_cTc​ scales with the energy gap in the weak coupling limit but crosses over to a t2/Ut^2/Ut2/U scaling in the BEC limit, where phase fluctuations controlled by nsn_sns​ determine TcT_cTc​. We also find, quite contrary to our expectations, that in the strong coupling limit, the large-NNN theory gives qualitatively wrong trends for compressibility. A comparison with a simple Hartree shifted BCS theory, which takes into account both pairing and Hartree shifts, and correctly recovers the atomic limit and the right qualitative trend for compressibility, reveals that the large-NNN theory on the lattice, although considers a larger number of diagrams, is in fact inferior to the simpler Hartree shifted BCS theory. The failure of the large-NNN approach is explained by noting (i) the importance of Hartree shift in lattice problems, and (ii) inability of the large-NNN approach to treat particle-particle and particle-hole channels at equal footing at the saddle point level.
We investigate the zero-temperature BCS to Bose-Einstein crossover at the mean-field level, by driving it with the attractive potential and the particle density. We emphasize specifically the role played by the particle density in this crossover. Three different interparticle potentials are considered for the continuum model in three spatial dimensions, while both s- and d-wave solutions are analyzed for the attractive (extended) Hubbard model on a two-dimensional square lattice. For this model the peculiar behavior of the crossover for the d-wave solution is discussed. In particular, in the strong-coupling limit when approaching half-filling we evidence the occurrence of strong correlations among antiparallel-spin fermions belonging to different composite bosons, which give rise to a quasi-long-range antiferromagnetic order in this limit.
The problem of the evolution from BCS theory with cooperative Cooper pairing to the formation and condensation of composite bosons has attracted considerable attention for the past several decades. It has gained renewed impetus in the mid-eighties with the discovery of the high-Tc superconductors, which have a coherence length comparable to the interparticle spacing. More recently, this subject has spurred a great deal of research activity in connection with experiments involving dilute atomic gases of fermionic atoms. The initial objective of this work will be to use functional integral techniques to analyze the low-temperature BCS-to-BEC evolution of d-wave superconductors within the saddle point (mean field) approximation for a continuum model. Then, the same mathematical formalism will be applied to the problem of the BCS-to-BEC evolution of fully spin-polarized p-wave Fermi gases in two dimensions. We find that a quantum phase transition occurs for both systems as they are driven from the BCS-like regime of weakly interacting fermionic pairs to the opposite BEC-like regime of strongly interacting bosonic molecules. This is in contrast to the smooth crossover predicted and observed in systems that exhibit s-wave pairing symmetry. We calculate several spectroscopic and thermodynamic properties that signal the occurrence of this phase transition, and suggest some possible experimental realizations. Finally, fluctuations about the saddle point solution are included in the calculations, and the effects of such correction are analyzed in the low (T~0) and high (T~Tc) temperature limits. We conclude that, at high temperatures, the bosonic degrees of freedom that arise from two-particle bound states become essential to describe the strong coupling limit,\nas the saddle point approximation alone becomes unreliable.