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arXiv:cond-mat/9908404 · Physical Review Letters

Real-Time Renormalization Group and Charge Fluctuations in Quantum Dots

Herbert Schoeller, Jürgen König

Published Apr 17, 2000• 115 citations
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Abstract

We develop a perturbative renormalization-group method in real time to describe nonequilibrium properties of discrete quantum systems coupled linearly to an environment. We include energy broadening and dissipation and develop a cutoff-independent formalism. We present quantitatively reliable results for the linear and nonlinear conductance in the mixed-valence and empty-orbital regime of the nonequilibrium Anderson impurity model with finite on-site Coulomb repulsion.

DOI
10.1103/physrevlett.84.3686

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We apply the real-time renormalization group (RG) in nonequilibrium to an arbitrary quantum dot in the Coulomb blockade regime. Within one-loop RG equations, we include self-consistently the kernel governing the dynamics of the reduced density matrix of the dot. As a result, we find that relaxation and dephasing rates generically cut off the RG flow. In addition, we include all other cutoff scales defined by temperature, energy excitations, frequency, and voltage. We apply the formalism to transport through single molecular magnets, realized by the fully anisotropic Kondo model (with three different exchange couplings Jx{J}_{x}Jx​, Jy{J}_{y}Jy​, and Jz{J}_{z}Jz​) in a magnetic field hz{h}_{z}hz​. We calculate the differential conductance as function of bias voltage VVV and discuss a quantum phase transition which can be tuned by changing the sign of JxJyJz{J}_{x}{J}_{y}{J}_{z}Jx​Jy​Jz​ via the anisotropy parameters. Finally, we calculate the noise $S(\ensuremath{\Omega})$ at finite frequency $\ensuremath{\Omega}$ for the isotropic Kondo model and find that the dephasing rate determines the height of the shoulders in $dS(\ensuremath{\Omega})∕d\ensuremath{\Omega}$ near $\ensuremath{\Omega}=V$.
One of the main open problems in the field of transport in strongly interacting nanostructures is the understanding of currents beyond the linear response regime. In this work, we consider the single-impurity Anderson model and use the adaptive time-dependent density matrix renormalization group method to compute real-time currents out of equilibrium. We first focus on the particle-hole symmetric point where Kondo correlations are the strongest and then extend the study of the nonequilibrium transport to the mixed-valence regime. As a main result, we present accurate data for the current-voltage characteristics of this model.
We apply the recently developed real-time renormalization-group (RTRG) method to different quantum dissipative systems. In contrast to other renormalization-group techniques the RTRG approach is formulated on the Keldysh contour and therefore allows for the description of nonequilibrium situations. The method is based on an exact kinetic equation which determines the time-dependent reduced density matrix. The kinetic equation involves an integral kernel which describes the phenomenon of dissipation. We calculate this quantity using the RTRG method: After applying Wick's theorem the arising diagrams are accounted for successively with respect to their time scale. During that process the theory is left invariant by renormalizing the operators describing the theory. As a starting point we discuss the polaron problem. We calculate the renormalized ground-state energy and the effective mass. We compare our results of the RTRG with those obtained from the flow equation formalism, which is based on infinitesimal transformations. In the central part of this thesis we consider the spin-boson model which is applicable to various physical and chemical systems. It models a particle in a double-well potential which is coupled to a bosonic environment. We determine static properties such as the static susceptibility. We also present results for the time evolution of the reduced density matrix starting from an arbitrary nonequilibrium state. The asymptotic behaviour of the reduced density matrix can be characterized by an oscillation frequency and two decay constants, all of which are determined. Finally, we calculate equilibrium correlation functions. We find consistency of our results with quantum Monte Carlo simulations and with the Shiba-relation. Additionally, our results show the correct scaling behaviour. Comparisons are also drawn to results of the noninteracting blip approximation and to results obtained for the anisotropic Kondo model. Our approach is very accurate for not too large couplings to the environment. Furthermore, the stationary tunnel current through a double quantum dot coupled to a phonon bath is calculated and compared to experimental data. Eventually, the running couplings of the two-lead Kondo model are discussed.
We develop a general approach to the nonequilibrium dynamics of quantum-impurity systems for arbitrary coupling strength. The numerical renormalization group is used to generate a complete basis set necessary for the correct description of the time evolution. We benchmark our method with the exact analytical solution for the resonant-level model. As a first application, we investigate the equilibration of an ultrasmall quantum dot subject to a sudden change of gate voltage and external magnetic field. Two distinct relaxation times are identified for the spin and charge dynamics.
We study transport properties of quantum impurity systems using the functional renormalization group. The latter is an RG-based diagrammatic tool to treat Coulomb interactions in a fast and flexible way. Prior applications, which employed a simple first-order (Hartree-Fock-like) scheme to truncate the FRG flow equations within the Matsubara formalism, succeeded in accurately describing linear transport of various quantum dot geometries at zero temperature T=0. In a nutshell, advance in this Thesis is three-fold. First, we introduce a frequency-dependent second-order approximation in order to eventually compute finite-energy properties such as the conductance at T>0 (mainly focusing on the single impurity Anderson model). Second, a generalisation of the Hartree-Fock-like approach to Keldysh space allows for addressing the non-equilibrium steady-state dynamics of the interacting resonant level model. Third, we investigate the physics of a quantum dot Josephson junction as well as the charging of a single narrow level using the first-order scheme.