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arXiv:cond-mat/9906313 · Physical Review Letters

Exact Eigenstates and Magnetic Response of Spin-1 and Spin-2 Bose-Einstein Condensates

Masato Koashi, Masahito Ueda

Published Feb 7, 2000• 269 citations
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Abstract

The exact eigenspectra and eigenstates of spin-1 and spin-2 Bose-Einstein condensates (BECs) are found, and their response to a weak magnetic field is studied and compared with their mean-field counterparts. Whereas mean-field theory predicts the vanishing population of the zero magnetic-quantum-number component of a spin-1 antiferromagnetic BEC, the component is found to become populated as the magnetic field decreases. The spin-2 BEC exhibits an even richer magnetic response due to quantum correlations among three bosons.

DOI
10.1103/physrevlett.84.1066

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The exact eigenspectra and eigenstates of spin-1 and spin-2 Bose-Einstein condensates (BECs) are found, and their response to a weak magnetic field is studied and compared with their mean-field counterparts. Whereas mean-field theory predicts the vanishing population of the zero magnetic-quantum-number component of a spin-1 antiferromagnetic BEC, the component is found to become populated as the magnetic field decreases. The spin-2 BEC exhibits an even richer magnetic response due to quantum correlations among three bosons.
The ground states of Bose-Einstein condensates (BECs) of spin-2 bosons are classified into three distinct phases (ferromagnetic, ``antiferromagnetic,'' and cyclic) depending on the s-wave scattering lengths of binary collisions for total-spin 0, 2, and 4 channels. Many-body spin correlations and magnetic response of the condensate in each of these phases are studied in a mesoscopic regime, while low-lying excitation spectra are investigated in the thermodynamic regime. In the mesoscopic regime, where the system is so tightly confined that the spatial degrees of freedom are frozen, the exact, many-body ground state for each phase is found to be expressed in terms of the creation operators of pair or trio bosons having spin correlations. These pairwise and trio-wise units are shown to bring about some unique features of spin-2 BECs such as a huge jump in magnetization from minimum to maximum possible values and the robustness of the minimum-magnetization state against an applied magnetic field. In the thermodynamic regime, where the system is spatially uniform, low-lying excitation spectra in the presence of magnetic field are obtained analytically using the Bogoliubov approximation. In the ferromagnetic phase, the excitation spectrum consists of one Goldstone mode and four single-particle modes. In the antiferromagnetic phase, where spin-singlet ``pairs'' undergo Bose-Einstein condensation, the spectrum consists of two Goldstone modes and three massive ones, all of which become massless when magnetic field vanishes. In the cyclic phase, where boson ``trios'' condense into a spin-singlet state, the spectrum is characterized by two Goldstone modes, one single-particle mode having a magnetic-field-independent energy gap, and a gapless single-particle mode that becomes massless in the absence of magnetic field.
We study experimentally the equilibrium phase diagram of a spin-1 Bose-Einstein condensate with antiferromagnetic interactions, in a regime where spin and spatial degrees of freedom are decoupled. For a given total magnetization mz{m}_{z}mz​, we observe for low magnetic fields an ``antiferromagnetic'' phase where atoms condense in the $m=\ifmmode\pm\else\textpm\fi{}1$ Zeeman states, and occupation of the m=0m=0m=0 state is suppressed. Conversely, for large enough magnetic fields, a phase transition to a ``broken-axisymmetry'' phase takes place: The m=0m=0m=0 component becomes populated and rises sharply above a critical field Bc(mz){B}_{c}({m}_{z})Bc​(mz​). This behavior results from the competition between antiferromagnetic spin-dependent interactions (dominant at low fields) and the quadratic Zeeman energy (dominant at large fields). We compare the measured Bc{B}_{c}Bc​ as well as the global shape of the phase diagram with mean-field theory, and find good quantitative agreement.
We demonstrate that dynamical symmetry plays a crucial role in determining the structure of the eigenspectra of spinor Bose-Einstein condensates (BECs). In particular, the eigenspectra of spin-1 and spin-2 BECs in the single-mode approximation are shown to be completely determined by dynamical symmetries, where a spin-2 BEC corresponds to the U(5) limit of the interacting boson model in nuclear physics. The eigenspectrum of a spin-3 BEC is solved analytically for a specific class of coupling constants, while it is shown that dynamical symmetry alone is not sufficient to determine the spectrum for arbitrary coupling constants. We also study the low-lying eigenspectra of spin-1 and spin-2 BECs in the absence of external magnetic field, and find, in particular, that the quasidegenerate spectra emerge for antiferromagnetic and cyclic phases. This implies that these systems are highly susceptible to external perturbations and may undergo symmetry-breaking transitions to other states upon increasing the system's size.
We investigate Bose-Einstein condensation of trapped spin-1 atoms with ferromagnetic or antiferromagnetic two-body contact interactions. We adopt the mean field theory and develop a Hartree-Fock-Popov type approximation in terms of a semiclassical two-fluid model. For antiferromagnetic interactions, our study reveals double condensations as atoms in the $\ensuremath{\mid}{m}_{F}=0⟩$ state never seem to condense under the constraints of both the conservation of total atom number NNN and magnetization MMM. For ferromagnetic interactions, however, triple condensations can occur. Our results can be conveniently understood in terms of the interplay of three factors: (anti)ferromagnetic atom-atom interactions, MMM conservation, and the miscibilities between and among different condensed components.