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arXiv:cond-mat/9807150 · Physical Review Letters

Semiclassical Eigenstates of Four-Sublattice Antiferromagnets

Christopher L. Henley, Nai-Gong Zhang

Published Dec 7, 1998• 16 citations
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Abstract

Applying Bohr-Sommerfeld quantization and the topological phase of spin path integrals, one can determine the multiplicities, lattice symmetries, and eigenvalue clustering pattern of the low-lying singlet eigenstates of the triangular and fcc antiferromagnets with four-sublattice classical ground states. In the triangular case, the clustering pattern agrees with numerical results of Lecheminant et al. [Phys. Rev. B 52, 6647 (1995)].

DOI
10.1103/physrevlett.81.5221

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Applying Bohr-Sommerfeld quantization and the topological phase of spin path integrals, one can determine the multiplicities, lattice symmetries, and eigenvalue clustering pattern of the low-lying singlet eigenstates of the triangular and fcc antiferromagnets with four-sublattice classical ground states. In the triangular case, the clustering pattern agrees with numerical results of Lecheminant et al. [Phys. Rev. B 52, 6647 (1995)].
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We study the low-lying eigenenergy clustering patterns of quantum antiferromagnets with p sublattices (in particular p=4).p=4).p=4). We treat each sublattice as a large spin, and using second-order degenerate perturbation theory, we derive the effective (biquadratic) Hamiltonian coupling the p large spins. In order to compare with exact diagonalizations, the Hamiltonian is explicitly written for a finite-size lattice, and it contains information on energies of excited states as well as the ground state. The result is applied to the face-centered-cubic Type-I antiferromagnet of spin 1/2, including second-neighbor interactions. A 32-site system is exactly diagonalized, and the energy spectrum of the low-lying singlets follows the analytically predicted clustering pattern.
Quantum magnetic phases near the magnetic saturation of triangular-lattice antiferromagnets with XXZ anisotropy have been attracting renewed interest since it has been suggested that a nontrivial coplanar phase, called the $\ensuremath{\pi}$-coplanar or $\mathrm{\ensuremath{\Psi}}$ phase, could be stabilized by quantum effects in a certain range of anisotropy parameter J/JzJ/{J}_{z}J/Jz​ besides the well-known 0-coplanar (known also as V)V)V) and umbrella phases. Recently, Sellmann et al. [Phys. Rev. B 91, 081104(R) (2015)] claimed that the $\ensuremath{\pi}$-coplanar phase is absent for S=1/2S=1/2S=1/2 from an exact-diagonalization analysis in the sector of the Hilbert space with only three down-spins (three magnons). We first reconsider and improve this analysis by taking into account several low-lying eigenvalues and the associated eigenstates as a function of J/JzJ/{J}_{z}J/Jz​ and by sensibly increasing the system sizes (up to 1296 spins). A careful identification analysis shows that the lowest eigenstate is a chirally antisymmetric combination of finite-size umbrella states for $J/{J}_{z}\ensuremath{\gtrsim}2.218$ while it corresponds to a coplanar phase for $J/{J}_{z}\ensuremath{\lesssim}2.218$. However, we demonstrate that the distinction between 0-coplanar and $\ensuremath{\pi}$-coplanar phases in the latter region is fundamentally impossible from the symmetry-preserving finite-size calculations with fixed magnon number. Therefore, we also perform a cluster mean-field plus scaling analysis for small spins $S\ensuremath{\le}3/2$. The obtained results, together with the previous large-SSS analysis, indicate that the $\ensuremath{\pi}$-coplanar phase exists for any SSS except for the classical limit $(S\ensuremath{\rightarrow}\ensuremath{\infty})$ and the existence range in J/JzJ/{J}_{z}J/Jz​ is largest in the most quantum case of S=1/2S=1/2S=1/2.