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arXiv:cond-mat/9802147 · Journal of Physics Condensed Matter

The antiferromagnetic spin- chain with competing dimers and plaquettes: numerical versus exact results

Johannes Richter, Nedko B. Ivanov, J. Schulenburg

Published Apr 27, 1998• 47 citations
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Abstract

We examine the ground state and the excitations of an one-dimensional Heisenberg spin 1/2 antiferromagnet with alternating dimers and four-spin plaquettes (dimer-plaquette chain). The properties of the system depend on the competing dimer and plaquette bonds. Several exact, exact-numerical and perturbational results are presented. We find that the system is gapped for all parameter values. For the latter one we find an effective S=1 Haldane like behaviour in the limit of dominating dimer bonds. The model considered is related to the recently found 1/5-depleted square-lattice Heisenberg system $CaV_4O_9$.

DOI
10.1088/0953-8984/10/16/015

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We examine the ground state and the excitations of an one-dimensional Heisenberg spin 1/2 antiferromagnet with alternating dimers and four-spin plaquettes (dimer-plaquette chain). The properties of the system depend on the competing dimer and plaquette bonds. Several exact, exact-numerical and perturbational results are presented. We find that the system is gapped for all parameter values. For the latter one we find an effective S=1 Haldane like behaviour in the limit of dominating dimer bonds. The model considered is related to the recently found 1/5-depleted square-lattice Heisenberg system CaV4O9CaV_4O_9CaV4​O9​.
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One dimensional S =1 antiferromagnetic Heisenberg chains with bond alternation and uniaxial single-ion-type anisotropy are studied by numerical exact diagonalization of finite size systems. We calculate the ground state phase diagram using the twisted boundary condition method for D ≥0. The ground states of this model contain the Haldane state, large- D state and the dimer state. Using conformal field theory and the level spectroscopy method, we calculate the D and δ-dependence of the Luttinger liquid paraments K and the critical exponent ν of the energy gap.
One dimensional S = 1 antiferromagnetic Heisenberg chains with bond alternation and uniaxial single-ion-type anisotropy are studied by numerical exact diagonalization of finite size systems. We calculate the ground state phase diagram using the twisted boundary condition method for D≥0. The ground states of this model contain the Haldane state, large-D state and the dimer state. Using conformal field theory and the level spectroscopy method, we calculate the D and δ-dependence of the Luttinger liquid paraments K and the critical exponent ν of the energy gap.
Abstract The spin- S Heisenberg antiferromagnet on the two-dimensional lattice is investigated for S = 1/2 and S = 1. We consider interaction at isolated dimers ( J d ) and interaction bonds that form the bounce lattice ( J b ). For J d = J b , the system is reduced to the maple-leaf-lattice antiferromagnet. We primarily conduct highly parallelized numerical diagonalization to examine the spin excitation gap above the ground state for various J b / J d cases. For S = 1/2, we report calculations for a 42-site cluster that has not been previously treated. The S = 1 case is examined for the first time for clusters up to 24 sites. Regardless of whether S = 1/2 or 1, we find that the system has a gapped nature for small J d / J b and becomes gapless at J d / J b ∼ 1.4. For S = 1, we also find that another gapped region appears between the gapless case at J d / J b ∼ 1.4 and the boundary of the exact-dimer phase.
The experimental observation of a spin gap in the antiferromagnetic spin-12\frac{1}{2}21​ compound CaV4{}_{4}4​O9{}_{9}9​ has been attributed to the formation of a plaquette-resonating-valence-bond (PRVB) state in the underlying 1/5-depleted square lattice. We construct a spin-12\frac{1}{2}21​ model on the 1/5-depleted lattice for which the PRVB state can be shown to be the exact ground state in a particular parameter regime. In a subspace of this parameter regime, the first excited state can be calculated exactly. In a different parameter regime, the dimer state is shown to be the exact ground state.
The ground-state phase diagram of a spin-12\frac{1}{2}21​ XXZ chain with competing ferromagnetic nearest-neighbor (J1<0{J}_{1}<0J1​<0) and antiferromagnetic second-neighbor (J2>0{J}_{2}>0J2​>0) exchange couplings is studied by means of the infinite time evolving block decimation algorithm and effective field theories. For the SU(2)-symmetric (Heisenberg) case, we show that the nonmagnetic phase in the range $\ensuremath{-}4<{J}_{1}/{J}_{2}<0$ has a small but finite ferromagnetic dimer order. We argue that this spontaneous dimer order is associated with effective spin-1 degrees of freedom on dimerized bonds, which collectively form a valence bond solid state as in the spin-1 antiferromagnetic Heisenberg chain (the Haldane spin chain). We thus call this phase the Haldane dimer phase. With easy-plane anisotropy, the model exhibits a variety of phases including the vector chiral phase with gapless excitations and the even-parity dimer and N\'eel phases with gapped excitations, in addition to the Haldane dimer phase. Furthermore, we show the existence of gapped phases with coexisting orders in narrow regions that intervene between the gapless chiral phase and any one of Haldane dimer, even-parity dimer, and N\'eel phases. Possible implications for quasi-one-dimensional edge-sharing cuprates are discussed.