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arXiv:cond-mat/9709271 · Journal of the Physical Society of Japan

Three-Leg Antiferromagnetic Heisenberg Ladder with Frustrated Boundary Condition; Ground State Properties

Kenro Kawano, Minoru Takahashi

Published Dec 15, 1997• 102 citations
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Abstract

The antiferromagnetic Heisenberg spin systems on the three-leg ladder are investigated. Periodic boundary condition is imposed in the rung direction. The system has an excitation gap for all antiferromagnetic inter-chain coupling ($J_{\perp}>0$). The estimated gap for the strong coupling limit ($J_{\perp}/J_1 \to \infty$) is 0.28$J_1$. Although the interaction is homogeneous and only nearest-neighbor, the ground states of the system are dimerized and break the translational symmetry in the thermodynamic limit. Introducing the next-nearest neighbor coupling ($J_2$), we can see that the system is solved exactly. The ground state wave function is completely dimer-ordered. Using density matrix renomalization group algorithm, we show numerically that the original model ($J_2=0$) has the same nature with the exactly solvable model. The ground state properties of the ladder with a higher odd number of legs are also discussed.

DOI
10.1143/jpsj.66.4001

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The antiferromagnetic Heisenberg spin systems on the three-leg ladder are investigated. Periodic boundary condition is imposed in the rung direction. The system has an excitation gap for all antiferromagnetic inter-chain coupling (J⊥>0J_{\perp}>0J⊥​>0). The estimated gap for the strong coupling limit (J⊥/J1→∞J_{\perp}/J_1 \to \inftyJ⊥​/J1​→∞) is 0.28J1J_1J1​. Although the interaction is homogeneous and only nearest-neighbor, the ground states of the system are dimerized and break the translational symmetry in the thermodynamic limit. Introducing the next-nearest neighbor coupling (J2J_2J2​), we can see that the system is solved exactly. The ground state wave function is completely dimer-ordered. Using density matrix renomalization group algorithm, we show numerically that the original model (J2=0J_2=0J2​=0) has the same nature with the exactly solvable model. The ground state properties of the ladder with a higher odd number of legs are also discussed.
Abstract. We study three-leg antiferromagnetic Heisenberg model with the periodic boundary conditions in the rung direction. Since the rungs form regular triangles, spin frustration is induced. We use the density-matrix renormalization group method to investigate the ground state. We find that the spin excitations are always gapped to remove the spin frustration as long as the rung coupling is nonzero. We also visibly confirm spin-Peierls dimerization order in the leg direction. Both the spin gap and the dimerization order are basically enhanced as the rung coupling increases. 1.
We study three-leg antiferromagnetic Heisenberg model with the periodic boundary conditions in the rung direction. Since the rungs form regular triangles, spin frustration is induced. We use the density-matrix renormalization group method to investigate the ground state. We find that the spin excitations are always gapped to remove the spin frustration as long as the rung coupling is nonzero. We also visibly confirm spin-Peierls dimerization order in the leg direction. Both the spin gap and the dimerization order are basically enhanced as the rung coupling increases.
We present a density matrix renormalization group study of the ground-state properties of spin-1/2 frustrated J1-J3 Heisenberg n(l)-leg ladders (with n(l) up to 8). For strong frustration (J(3)/J(1) approximately 0.5), both even-leg and odd-leg ladders display a finite gap to spin excitations, which we argue remains finite in the two-dimensional limit. In this regime, on odd-leg ladders the ground state is spontaneously dimerized, in agreement with the Lieb-Schultz-Mattis prediction, while on even-leg ladders the dimer correlations decay exponentially. The magnitude of the dimer order parameter decreases as the number of legs increases, consistent with a two-dimensional spin-liquid ground state.
The frustrated ladder with alternate ferromagnetic exchange $\ensuremath{-}{J}_{F}$ and antiferromagnetic exchange JA{J}_{A}JA​ to first neighbors and ferromagnetic exchange $\ensuremath{-}{J}_{L}$ to second neighbors is studied by exact diagonalization and density matrix renormalization group calculations in systems of 2N2N2N spins-12\frac{1}{2}21​ with periodic boundary conditions. The ground state is a singlet (S=0)(S=0)(S=0) and the singlet-triplet gap ${\ensuremath{\varepsilon}}_{T}$ is finite for the exchanges considered. Spin-12\frac{1}{2}21​ string correlation functions g1(N){g}_{1}(N)g1​(N) and g2(N){g}_{2}(N)g2​(N) are defined for an even number NNN of consecutive spins in systems with two spins per unit cell; the ladder has string order ${g}_{2}(\ensuremath{\infty})>0$ and ${g}_{1}(\ensuremath{\infty})=0$. The minimum N∗{N}^{*}N∗ of g2(N){g}_{2}(N)g2​(N) is related to the range of ground-state spin correlations. Convergence to ${g}_{2}(\ensuremath{\infty})$ is from below, and g1(N){g}_{1}(N)g1​(N) decreases exponentially for $N\ensuremath{\ge}{N}^{*}$. Singlet valence bond (VB) diagrams account for the size dependencies. The frustrated ladder at special values of JF,JL{J}_{F}, {J}_{L}JF​,JL​, and JA{J}_{A}JA​ reduces to well-known models such as the spin-1 Heisenberg antiferromagnet and the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model, among others. Numerical analysis of ladders matches previous results for spin-1 gaps or string correlation functions and extends them to spin-12\frac{1}{2}21​ systems. The nondegenerate singlet ground state of the ladder is a bond-order wave, a Kekul\'e VB diagram at ${J}_{L}={J}_{F}/2\ensuremath{\le}{J}_{A}$, that is reversed on interchanging $\ensuremath{-}{J}_{F}$ and JA{J}_{A}JA​. Inversion symmetry is spontaneously broken in the dimer phase of the ${J}_{1}\text{\ensuremath{-}}{J}_{2}$ model where the Kekul\'e diagrams are the doubly degenerate ground states at J2/J1=1/2{J}_{2}/{J}_{1}=1/2J2​/J1​=1/2.
The frustrated ladder with alternate ferromagnetic(F) exchange −JF-J_F−JF​ and AF exchange JAJ_AJA​ to first neighbors and F exchange −JL-J_L−JL​ to second neighbors is studied by exact diagonalization (ED) and density matrix renormalization group (DMRG) calculations in systems of 2N2N2N spins-1/2 with periodic boundary conditions. The ground state is a singlet (S=0)(S = 0)(S=0) and the singlet-triplet gap εT\varepsilon_TεT​ is finite for the exchanges considered. Spin-1/2 string correlation functions g1(N)g_1(N)g1​(N) and g2(N)g_2(N)g2​(N) are defined for an even number NNN of consecutive spins in systems with two spins per unit cell; the ladder has string order g2(∞)>0g_2(\infty)> 0g2​(∞)>0 and g1(∞)=0g_1(\infty) = 0g1​(∞)=0. The minimum N∗N^*N∗ of g2(N)g_2(N)g2​(N) is related to the range of ground-state spin correlations. Convergence to g2(∞)g_2(\infty)g2​(∞) is from below, and g1(N)g_1(N)g1​(N) decreases exponentially for N≥N∗N \geq N^*N≥N∗. Singlet valence bond (VB) diagrams account for the size dependencies. The frustrated ladder at special values of JFJ_FJF​, JLJ_LJL​ and JAJ_AJA​ reduces to well-known models such as the spin-1 Heisenberg antiferromagnet and the J1−J2J_1-J_2J1​−J2​ model, among others. Numerical analysis of ladders matches previous results for spin-1 gaps or string correlation functions and extends them to spin-1/2 systems. The nondegenerate singlet ground state of ladder is a bond-order wave, a Kekulé VB diagrams at JL=JF/2≤JAJ_L = J_F/2 \leq J_AJL​=JF​/2≤JA​, that is reversed on interchanging −JF-J_F−JF​ and JAJ_AJA​. Inversion symmetry is spontaneously broken in the dimer phase of the J1−J2J_1-J_2J1​−J2​ model where the Kekulé diagrams are the doubly degenerate ground states at J2/J1=1/2J_2/J_1 = 1/2J2​/J1​=1/2.
We perform a systematic investigation on an asymmetric zigzag spin ladder with interleg exchange J1{J}_{1}J1​ and different exchange integrals ${J}_{2}\ifmmode\pm\else\textpm\fi{}\ensuremath{\delta}$ on both legs. In the weak frustration limit, the spin model can be mapped to a revised double frequency sine-Gordon model by using bosonization. Renormalization-group analysis shows that the Heisenberg critical point flows to an intermediate-coupling fixed point with gapless excitations and a vanishing spin velocity. When the frustration is large, a spin gap opens and a dimer ground state is realized. Fixing J2=J1/2,{J}_{2}{=J}_{1}/2,J2​=J1​/2, we find, as a function of $\ensuremath{\delta},$ a continuous manifold of Hamiltonians with dimer product ground states, interpolating between the Majumdar-Ghosh and sawtooth spin-chain model. While the ground state is independent of the alternating next-nearest-neighbor exchange $\ensuremath{\delta},$ the gap size of excitations is found to decrease with increasing $\ensuremath{\delta}.$ We also extend our study to a two-dimensional double layer model with an exactly known ground state.