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arXiv:cond-mat/9311008 · Physical Review Letters

Resonant impurity scattering in a strongly correlated electron model

Didier Poilblanc, Douglas J. Scalapino, Werner R. Hanke

Published Feb 7, 1994• 100 citations
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Abstract

Scattering by a single impurity introduced in a strongly correlated electronic system is studied by exact diagonalization of small clusters. It is shown that an inert site which is spinless and unable to accommodate holes can give rise to strong resonant scattering. A calculation of the local density of states reveals that, for increasing antiferromagnetic exchange coupling, d,- s,- and p-wave symmetry bound states in which a mobile hole is trapped by the impurity potential induced by a local distortion of the antiferromagnetic background successively pull out from the continuum.

DOI
10.1103/physrevlett.72.884

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Scattering by a single impurity introduced in a strongly correlated electronic system is studied by exact diagonalization of small clusters. It is shown that an inert site which is spinless and unable to accommodate holes can give rise to strong resonant scattering. A calculation of the local density of states reveals that, for increasing antiferromagnetic exchange coupling, d,- s,- and p-wave symmetry bound states in which a mobile hole is trapped by the impurity potential induced by a local distortion of the antiferromagnetic background successively pull out from the continuum.
The effect of a magnetic (S=1/2) impurity coupled to a two-dimensional system of correlated electrons (described by the t-J model) is studied by exact diagonalizations. It is found that, if the exchange coupling of the impurity with the neighboring spins is ferromagnetic or weakly antiferromagnetic, an extra hole can form bound states of different spatial symmetries with the impurity extending to a few lattice spacings. The binding energy is maximum when the impurity is completely decoupled (vacancy) and vanishes for an antiferromagnetic coupling exceeding \ensuremath{\sim}0.3J. Several peaks appear in the single-hole spectral function below the lower edge of the quasiparticle band as signatures of the d-, s-, and p-wave bound states.
We investigate magnetic properties induced by a spinless impurity in strongly correlated electron systems, i.e., the Hubbard model in spatial dimension D=1,2,D=1,2,D=1,2, and 3.3.3. For the one-dimensional (1D) system exploiting the Bethe ansatz exact solution we find that the spin susceptibility and the local density of states in the vicinity of a spinless impurity show divergent behaviors. The results imply that the induced local moment is not completely quenched at any finite temperatures. On the other hand, the spin lattice relaxation rate obtained by bosonization and boundary conformal field theory satisfies a relation analogous to the Korringa law, ${1/T}_{1}T\ensuremath{\sim}{\ensuremath{\chi}}^{2}.$ In the 2D and 3D systems, the analysis based upon the antiferromagnetically correlated Fermi liquid theory reveals that the antiferromagnetic spin fluctuation developed in the bulk is much suppressed in the vicinity of a spinless impurity, and thus magnetic properties are governed by the induced local moment, which leads to the Korringa law of 1/T1.{1/T}_{1}.1/T1​.
In nearly antiferromagnetic (AF) metals such as high-Tc{T}_{\mathrm{c}}Tc​ superconductors (HTSCs), a single nonmagnetic impurity frequently causes nontrivial widespread change of the electronic states. To elucidate this long-standing issue, we study a Hubbard model with a strong onsite impurity potential based on an improved fluctuation-exchange (FLEX) approximation, which we call the GVIG{V}^{I}GVI-FLEX method. This model corresponds to the HTSC with dilute nonmagnetic impurity concentration. We find that (i) both local and staggered susceptibilities are strongly enhanced around the impurity. By this reason, (ii) the quasiparticle lifetime as well as the local density of states are strongly suppressed in a wide area around the impurity (like a Swiss cheese hole), which causes the ``huge residual resistivity'' beyond the sss-wave unitary scattering limit. We stress that the excess quasiparticle damping rate caused by impurities has strong k\mathbf{k}k-dependence due to non-sss-wave scatterings induced by many-body effects, so the structure of the ``hot spot/cold spot'' in the host system persists against impurity doping. This result could be examined by the ARPES measurements. In addition, (iii) only a few percent of impurities can cause a ``Kondo-like'' upturn of resistivity $(d\ensuremath{\rho}∕dT<0)$ at low TTT when the system is very close to the AF quantum critical point. The results (i)--(iii) obtained in the present study, which cannot be derived by the simple FLEX approximation, naturally explain the main impurity effects in HTSCs. We also discuss the impurity effect in heavy fermion systems and organic superconductors.
We investigate magnetic properties induced by a spinless impurity in strongly correlated electron systems, i.e. the Hubbard model in the spatial dimension D=1,2,D=1,2,D=1,2, and 3. For the 1D system exploiting the Bethe ansatz exact solution we find that the spin susceptibility and the local density of states in the vicinity of a spinless impurity show divergent behaviors. The results imply that the induced local moment is not completely quenched at any finite temperatures. On the other hand, the spin lattice relaxation rate obtained by bosonization and boundary conformal field theory satisfies a relation analogous to the Korringa law, 1/T1T∼χ21/T_1T \sim \chi^21/T1​T∼χ2. In the 2D and 3D systems, the analysis based upon the antiferromagnetically correlated Fermi liquid theory reveals that the antiferromagnetic spin fluctuation developed in the bulk is much suppressed in the vicinity of a spinless impurity, and thus magnetic properties are governed by the induced local moment, which leads to the Korringa law of 1/T11/T_11/T1​.
We consider a strongly correlated ladder with diagonal hopping and exchange interactions described by t−Jt-Jt−J type hamiltonian. We study the dynamics of a single hole in this model in the presence of a static non-magnetic (or magnetic) impurity. In the case of a non-magnetic (NM) impurity we solve the problem analytically both in the triplet (S=1) and singlet (S=0) sectors. In the triplet sector the hole doesn't form any bound state with the impurity. However, in the singlet sector the hole forms bound states of different symmetries with increasing J/tJ/tJ/t values. Binding energies of those impurity-hole bound states are compared with the binding energy of a pair of holes in absence of any impurity. In the case of magnetic impurity the analytical eigenvalue equations are solved for a large (50 X 2) lattice. In this case also, with increasing J/tJ/tJ/t values, impurity-hole bound states of different symmetries are obtained. Binding of the hole with the impurity is favoured for the case of a ferromagnetic (FM) impurity than in the case of antiferromagnetic (AFM) impurity. However binding energy is found to be maximum for the NM impurity. Comparison of binding energies and various impurity-hole correlation functions indicates a pair breaking mechanism by NM impurity.
We study a magnetic impurity embedded in a correlated electron system using the density-matrix renormalization group method. The correlated electron system is described by the one-dimensional Hubbard model. At half filling, we confirm that the binding energy of the singlet bound state increases exponentially in the weak-coupling regime and decreases inversely proportional to the correlation in the strong-coupling regime. The spin-spin correlation shows an exponential decay with distance from the impurity site. The correlation length becomes smaller with increasing the correlation strength. We find discontinuous reduction of the binding energy and of spin-spin correlations with hole doping. The binding energy is reduced by hole doping; however, it remains of the same order of magnitude as for the half-filled case.