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arXiv:cond-mat/0702586 · Physical Review B

Spin-gapped incoherent metal with preformed pairing in the doped antiferromagnetic Mott insulator

Ki‐Seok Kim, Mun Dae Kim

Published Mar 7, 2008• 6 citations
arXivHTMLPDF

Abstract

We investigate how the antiferromagnetic Mott insulator evolves into the $d$-wave BCS superconductor through hole doping. Allowing spin fluctuations in the strong-coupling approach, we find a spin-gapped incoherent metal with preformed pairing as an intermediate phase between the antiferromagnetic Mott insulator and $d$-wave superconductor. This non-Fermi-liquid metal is identified with an infrared stable fixed point in the spin-decomposition gauge theory, analogous to the spin liquid insulator in the slave-boson gauge theory. We consider the single particle spectrum and dynamical spin susceptibility in the anomalous metallic phase, and discuss physical implications.

DOI
10.1103/physrevb.77.125103

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We investigate how the antiferromagnetic Mott insulator evolves into the ddd-wave BCS superconductor through hole doping. Allowing spin fluctuations in the strong-coupling approach, we find a spin-gapped incoherent metal with preformed pairing as an intermediate phase between the antiferromagnetic Mott insulator and ddd-wave superconductor. This non-Fermi-liquid metal is identified with an infrared stable fixed point in the spin-decomposition gauge theory, analogous to the spin liquid insulator in the slave-boson gauge theory. We consider the single particle spectrum and dynamical spin susceptibility in the anomalous metallic phase, and discuss physical implications.
A slave-fermion gauge-theory approach of the t-J model: Doping-induced complex magnetic structure and Z2_{2}2​ spin-gapped anomalous metal in an antiferromagnetic doped Mott insulator
We reinvestigate a doped antiferromagnetic Mott insulator based on the slave-fermion approach of the t-J model, where antiferromagnetic spin fluctuations and doped holes are described by bosonic spinons and fermionic holons, respectively. Earlier studies have shown that an effective field theory for the doped antiferromagnetic Mott insulator is given by a non-relativistic fermion (holon) U(1) gauge theory for charge dynamics and a relativistic boson (spinon) U(1) gauge theory for spin dynamics, thus allowing an anomalous metallic phase where bosonic spinons are gapped away from an antiferromagnetic state, analogous to the U(1) spin liquid phase in the slave-boson approach of the t-J model. We argue that the emergent U(1) gauge structure in this approach is based on a simplified picture for antiferromagnetic correlations. Considering that dynamics of doped holes frustrates a collinear antiferromagnetic spin configuration, we show that doped holes enhance ferromagnetic spin correlations and result in a complex magnetic structure. The presence of such a complex spin texture reduces the U(1) gauge structure down to Z2_{2}2​, thus a different effective field theory results for the spin-gapped non-Fermi liquid metal at low temperatures because there are no gapless U(1) gauge fluctuations.
Using a simple variational ansatz, we estimate the pair wave function of a superconductor obtained by doping a Mott insulator with short-range antiferromagnetic spin correlations. The pairing symmetry is generically d wave. The so-called ``anyon superconductors'' are related to traditional BCS states with d-wave order parameters that break parity and time-reversal invariance. The transition between a tetragonal normal metal and a superconductor of this type generically proceeds through an intermediate phase with either superconducting order or broken time reversal, but not both.
Proximity to a Mott insulating phase is likely to be an important physical ingredient of a theory that aims to describe high-temperature superconductivity in the cuprates. Quantum cluster methods are well suited to describe the Mott phase. Hence, as a step toward a quantitative theory of the competition between antiferromagnetism and ddd-wave superconductivity in the cuprates, we use cellular dynamical mean-field theory to compute zero-temperature properties of the two-dimensional square lattice Hubbard model. The ddd-wave order parameter is found to scale like the superexchange coupling JJJ for on-site interaction UUU comparable to or larger than the bandwidth. The order parameter also assumes a dome shape as a function of doping, while, by contrast, the gap in the single-particle density of states decreases monotonically with increasing doping. In the presence of a finite second neighbor hopping ${t}^{\ensuremath{'}}$, the zero-temperature phase diagram displays the electron-hole asymmetric competition between antiferromagnetism and superconductivity that is observed experimentally in the cuprates. Adding realistic third neighbor hopping ${t}^{\ensuremath{''}}$ improves the overall agreement with the experimental phase diagram. Since band parameters can vary depending on the specific cuprate considered, the sensitivity of the theoretical phase diagram to band parameters challenges the commonly held assumption that the doping vs Tc∕Tcmax{T}_{c}∕{T}_{c}^{\mathit{max}}Tc​∕Tcmax​ phase diagram of the cuprates is universal. The calculated angle-resolved photoemission spectrum displays the observed electron-hole asymmetry. The tendency to homogeneous coexistence of the superconducting and antiferromagnetic order parameters is stronger than observed in most experiments but consistent with many theoretical results and with experiments in some layered high-temperature superconductors. Clearly, our calculations reproduce important features of ddd-wave superconductivity in the cuprates that would otherwise be considered anomalous from the point of view of the standard Bardeen--Cooper--Schrieffer approach. At strong coupling, ddd-wave superconductivity and antiferromagnetism naturally appear as two equally important competing instabilities of the normal phase of the same underlying Hamiltonian.
The competition between antiferromagnetism and hole motion in two-dimensional Mott insulators lies at the heart of a doping-dependent transition from an anomalous metal to a conventional Fermi liquid. We observe such a crossover in Fermi-Hubbard systems on a cold-atom quantum simulator and reveal the transformation of multipoint correlations between spins and holes upon increasing doping at temperatures around the superexchange energy. Conventional observables, such as spin susceptibility, are furthermore computed from the microscopic snapshots of the system. Starting from a magnetic polaron regime, we find the system evolves into a Fermi liquid featuring incommensurate magnetic fluctuations and fundamentally altered correlations. The crossover is completed for hole dopings around 30%. Our work benchmarks theoretical approaches and discusses possible connections to lower-temperature phenomena.
The issues of single particle coherence and its interplay with singlet pairing are studied within the slave boson gauge theory of a doped Mott insulator. Prior work by one of us [T. Senthil, Phys. Rev. B 78, 045109 (2008)10.1103/PhysRevB.78.045109] showed that the coherence scale below which Landau quasiparticles emerge is parametrically lower than that identified in the slave boson mean field theory. Here we study the resulting new non-Fermi liquid intermediate temperature regime characterized by a single particle scattering rate that is linear in temperature (T). In the presence of a d-wave pair amplitude, this leads to a pseudogap state with T-dependent Fermi arcs near the nodal direction. Implications for understanding the cuprates are discussed.
Cooper pairing instability in a Fermi liquid is well understood by the BCS theory, but pairing mechanism for doped Mott insulators still remains elusive. Previously it has been shown by density matrix renormalization group (DMRG) method that a single doped hole is always self-localized due to the quantum destructive interference of the phase string signs hidden in the t-J ladders. Here we report a DMRG investigation of hole binding in the same model, where a novel pairing-glue scheme beyond the BCS realm is discovered. Specifically, we show that, in addition to spin pairing due to superexchange interaction, the strong frustration of the phase string signs on the kinetic energy gets effectively removed by pairing the charges, which results in strong binding of two holes. By contrast, if the phase string signs are "switched off" artificially, the pairing strength diminishes significantly even if the superexchange coupling remains the same. In the latter, unpaired holes behave like coherent quasiparticles with pairing drastically weakened, whose sole origin may be attributed to the resonating-valence-bond (RVB) pairing of spins. Such non-BCS pairing mechanism is therefore beyond the RVB picture and may shed important light on the high-T(c) cuprate superconductors.