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arXiv:cond-mat/0611196 · Physical Review B

Many-body interaction in semiconductors probed with two-dimensional Fourier spectroscopy

Mikhail Erementchouk, Michael Niklaus Leuenberger, Lu Jeu Sham

Published Sep 10, 2007• 13 citations
arXivHTMLPDF

Abstract

A particular difficulty in studying many-body interactions in a solid is the absence of an experimental technique that can directly probe their key characteristics. We show that two-dimensional (2D) Fourier spectroscopy provides an efficient tool for the measurement of critical parameters describing the effect of many-body interactions on the optical response of semiconductors. We develop the basic microscopic theory of 2D Fourier spectroscopy of semiconductors in the framework of the three-band model (heavy holes, light holes, and electrons). The theory includes many-body correlations nonperturbatively and can be generalized straightforwardly in order to describe 2D Fourier spectra obtained in atomic physics. We establish a relation between the 2D Fourier spectrum and the many-body correlations. It is shown, in particular, that 2D Fourier spectroscopy provides a principal possibility to establish experimentally the origin of the fast decay of the memory term describing the Coulomb interaction between heavy- and light-hole excitons. The theory is applied to an analysis of the available experimental data. Experiments providing more detailed information are suggested.

DOI
10.1103/physrevb.76.115307

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A microscopic many-body theory for the optical and electronic properties of semiconductors is reviewed with an emphasis on the role of correlation effects. At the semiclassical level, the semiconductor Bloch equations include many-body effects via bandgap and field renormalization as well as correlation contributions representing two electron-hole pair amplitudes, excitonic populations, and coupled interband and intraband coherences. These Coulomb interaction induced carrier correlations lead to characteristic signatures in nonlinear semiconductor spectroscopy. At the fully quantum mechanical level the dominant light-matter correlations are described by coupled semiconductor Bloch and luminescence equations. Excitonic emission properties of quantum well and microcavity systems are discussed, including effects such as coherent signatures in the secondary emission and coherent control of the emitted light.
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