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arXiv:cond-mat/0609022

New polarization effect and collective excitation in S=1/2 quasi 1D antiferromagnetic quantum spin chain

S. V. Demishev, A. V. Semeno, Hitoshi Ohta, S. Okubo, I. E. Tarasenko, Ishchenko, T. V., Nikolay E. Sluchanko

Published Sep 1, 2006• 0 citations
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Abstract

Anomalous polarization characteristics of magnetic resonance in CuGeO3 doped with 2% of Co impurity are reported. For the Faraday geometry this mode is damped for the microwave field Bw aligned along a certain crystallographic direction showing that the character of magnetic oscillation differs from the standard spin precession. The observed resonance coexists with the ESR on Cu2+ chains and argued not to be caused by "impurity" EPR, as previously claimed, but to correspond to a previously unknown collective mode of magnetic oscillations in S=1/2 AF quantum spin chain.

DOI
10.48550/arxiv.cond-mat/0609022

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Anomalous polarization characteristics of magnetic resonance in CuGeO3 doped with 2% of Co impurity are reported. For the Faraday geometry this mode is damped for the microwave field Bw aligned along a certain crystallographic direction showing that the character of magnetic oscillation differs from the standard spin precession. The observed resonance coexists with the ESR on Cu2+ chains and argued not to be caused by "impurity" EPR, as previously claimed, but to correspond to a previously unknown collective mode of magnetic oscillations in S=1/2 AF quantum spin chain.
Anomalous polarization characteristics of magnetic resonance in CuGeO3 doped with 2% Co impurity are reported. For the Faraday geometry, this mode is damped for the microwave field B ω aligned along a certain crystallographic direction, showing that the character of magnetic oscillation differs from the standard spin precession. The observed resonance coexists with the ESR on Cu2+ chains; it is argued not to be caused by “impurity” EPR, as previously claimed, but to correspond to a previously unknown collective mode of magnetic oscillations in an S = 1/2 AF quantum spin chain.
Magnetic excitations of the exchange-dipole quasi-one-dimensional XXZ antiferromagnet are studied in the ordered phase. We observe a transformation of the electron spin resonance (ESR) spectrum when crossing the N\'eel temperature near 0.2 K. The single-mode ESR of a correlated XXZ chain transforms in the multimode spectrum in the ordered phase. The multimode spectrum consists mainly of the intensive mode of a single correlated chain, which is surrounded and/or indented by numerous weak satellites. The number of securely fixed modes is eight at $\mathbf{H}\ensuremath{\parallel}b$ and twelve at $\mathbf{H}\ensuremath{\parallel}a$. In addition to the multimode resonance observed at the transverse polarization of the microwave and static magnetic fields, we reveal a wide band of absorption by (kkk,--kkk) pairs of quasiparticles at the longitudinal polarization. This kind of absorption of microwaves occurs both in the ordered and specific spin-liquid phases, revealing the presence of quasiparticles in the specific spin-liquid phase.
We report on an electron spin resonance (ESR) study of a nearly one-dimensional (1D) spin-12\frac{1}{2}21​ chain antiferromagnet, Sr2CuO3{\mathrm{Sr}}_{2}{\mathrm{CuO}}_{3}Sr2​CuO3​, with extremely weak magnetic ordering. The ESR spectra at T>TNT>{T}_{N}T>TN​, in the disordered Luttinger-spin-liquid phase, reveal nearly ideal Heisenberg-chain behavior with only a very small, field-independent linewidth, $\ensuremath{\sim}1/T$. In the ordered state, below TN{T}_{N}TN​, we identify field-dependent antiferromagnetic resonance modes, which are well described by pseudo-Goldstone magnons in the model of a collinear biaxial antiferromagnet. Additionally, we observe a major resonant mode with unusual and strongly anisotropic properties, which is not anticipated by the conventional theory of Goldstone spin waves. We propose that this unexpected magnetic excitation can be attributed to a field-independent magnon mode renormalized due to its interaction with the high-energy amplitude (Higgs) mode in the regime of weak spontaneous symmetry breaking.
High-field electron spin resonance (ESR) measurements were performed on the S = 1/2 Ising-like antiferromagnetic chain CsCoCl3 in the frequency range up to 4.4 THz and magnetic fields for H || c up to 53 T. We observed softening of the spinon excitation, which drives the spin chain into the quantum critical state at the critical field Hc = 33.0 T. Above Hc, we observed the string excitation at the wave number q = π, which is characteristic of the S = 1/2 spin chain in the quantum critical state in the magnetic fields. We also observed a crossover of the string excitation to the magnon bound state above the saturation field Hs = 43.9 T upon increasing the magnetic fields. Finally, we discuss how the string excitation and magnon bound state can be excited by the electric dipole transition due to spin quadrupolar resonance.
This article is a review of the recent achievements in experimental studies of magnetic excitations in the copper pyrimidine dinitrate [PM–Cu(NO3)2(H2O)2]n (PM = pyrimidine), an S = 1/2 antiferromagnetic chain material with an alternating g-tensor and the Dzyaloshinskii–Moriya interaction, by means of high-field electron spin resonance (ESR). Due to this alternation, in the 1D critical regime this material exhibits a field-induced gap. The excitation spectrum is formed by solitons and their bound states, breathers, and can be effectively described using the sine-Gordon model. With increasing temperature, the soliton-breather regime can be suppressed, resulting in a substantial evolution of ESR parameters. These changes can be described using a new theoretical concept recently proposed for S = 1/2 AF chains with a staggered transverse field. High magnetic field induces a transition into the spin-polarized state with the excitation spectrum formed by magnons. Nonmonotonous behavior of the field-induced gap is observed in vicinity of the saturation field. Experimental data are compared with results of existing theoretical approaches, revealing excellent agreement with predictions.
We discuss the universal theory of localized impurities in the paramagnetic state of 2D antiferromagnets where the spin gap is assumed to be significantly smaller than a typical exchange energy. We study the impurity spin susceptibility near the host quantum transition from a gapped paramagnet to a Néel state, and we compute the impurity-induced damping of the spin-1 mode of the gapped antiferromagnet. Under suitable conditions our results apply also to d-wave superconductors. Doped antiferromagnets (AF) have been the subject of intense studies in the context of the cuprate high-temperature superconductors and other layered transition metal compounds. We present a quantum theory of a particular class of doped AF where it is possible to neglect the coupling between the spin and charge degrees of freedom and consider a theory of the spin excitations alone. Such a theory will apply to (i) quasi-2D ‘spin gap ’ insulators like SrCu2O3 or NaV2O5 in