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arXiv:cond-mat/0604495 · Physical Review B

Magnetic phase diagram of a frustrated ferrimagnetic ladder: Relation to the one-dimensional boson Hubbard model

Nedko B. Ivanov, Johannes Richter

Published Apr 19, 2006• 3 citations
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Abstract

We study the magnetic phase diagram of two coupled mixed-spin $(1,\frac{1}{2})$ Heisenberg chains as a function of the frustration parameter related to diagonal exchange couplings. The analysis is performed by using spin-wave series and exact numerical diagonalization techniques. The obtained phase diagram---containing the Luttinger liquid phase, the plateau phase with a magnetization per rung $M=1∕2$, and the fully polarized phase---is closely related to the generic $(J∕U,\ensuremath{\mu}∕U)$ phase diagram of the one-dimensional boson Hubbard model.

DOI
10.1103/physrevb.73.132407

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Using exact numerical diagonalization and the conformal field theory approach, we study the effect of magnetic frustrations due to diagonal exchange bonds in a system of two coupled mixed-spin (1,12)(1,\frac{1}{2})(1,21​) Heisenberg chains. It is established that relatively moderate frustrations are able to destroy the ferrimagnetic state and to stabilize the critical spin-liquid phase typical for half-integer-spin antiferromagnetic Heisenberg chains. Both phases are separated by a narrow but finite region occupied by a critical partially polarized ferromagnetic phase.
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We study the impact of the diagonal frustrating couplings on the quantum phase diagram of a two-leg ladder composed of alternating spin-1 and spin-12\frac{1}{2}21​ rungs. As the coupling strength is increased the system successively exhibits two gapped paramagnetic phases (a rung-singlet and a Haldane-type nondegenerate states) and two ferrimagnetic phases with different ferromagnetic moments per rung. The first two states are similar to the phases studied in the frustrated spin-12\frac{1}{2}21​ ladder, whereas the magnetic phases appear as a result of the mixed-spin structure of the model. A detailed characterization of these phases is presented using density-matrix renormalization-group calculations, exact diagonalizations of periodic clusters, and an effective Hamiltonian approach inspired by the analysis of numerical data. The present theoretical study was motivated by the recent synthesis of the quasi-one-dimensional ferrimagnetic material FeIIFeIII{\text{Fe}}^{\text{II}}{\text{Fe}}^{\text{III}}FeIIFeIII (trans-1,4-cyclohexanedicarboxylate) exhibiting a similar ladder structure.
We use bosonization and renormalization group methods to determine the ground-state phase diagram of a one-dimensional frustrated Kondo-Heisenberg system consisting of a one-dimensional spin-12\frac{1}{2}21​ Luttinger liquid coupled by a Kondo exchange interaction JK{J}_{K}JK​ to a frustrated quantum antiferromagnetic Heisenberg chain, with a nearest-neighbor exchange coupling J1{J}_{1}J1​ and a next-nearest-neighbor (frustrating) exchange interaction J2{J}_{2}J2​. We analyze the interplay of quantum frustration in the antiferromagnetic chain with the Kondo exchange coupling JK{J}_{K}JK​ with the Luttinger liquid. We discuss the structure of the phase diagram of this system as a function of the ratios JK/J1{J}_{K}/{J}_{1}JK​/J1​, J2/J1{J}_{2}/{J}_{1}J2​/J1​, and of the parameters of the Luttinger liquid. In particular, we discuss in detail the regimes in which a pair-density-wave state may be realized and its relation with the spin correlations in the frustrated antiferromagnetic chain.
We present a brief survey of the recent theoretical work related to generic Heisenberg spin models describing quasi-one-dimensional quantum ferrimagnets.The emphasis is on quantum chains and ladders with strong competing interactions, such as the frustrated J 1 -J 2 chain with alternating (1, 1/2) spins, the spin-1/2 diamond chain with four-spin cyclic couplings, and some generic types of mixed-spin ladders with geometric frustration.As a rule, the discussed models exhibit rich quantum phase diagrams and provide some interesting examples of one-dimensional magnetic-paramagnetic quantum phase transitions.A number of open problems in the reviewed research area are discussed.
Ground states of the frustrated spin-1 Ising-Heisenberg two-leg ladder with Heisenberg intra-rung coupling and only Ising interaction along legs and diagonals are rigorously found by taking advantage of local conservation of the total spin on each rung.The constructed ground-state phase diagram of the frustrated spin-1 Ising-Heisenberg ladder is then compared with the analogous phase diagram of the fully quantum spin-1 Heisenberg two-leg ladder obtained by density matrix renormalization group (DMRG) calculations.Both investigated spin models exhibit quite similar magnetization scenarios, which involve intermediate plateaux at one-quarter, one-half and threequarters of the saturation magnetization.