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arXiv:cond-mat/0603270 · Physical Review A

Dressed molecules in resonantly interacting ultracold atomic Fermi gases

G. M. Falco, Henk T. C. Stoof

Published Feb 12, 2007• 12 citations
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Abstract

We present a detailed analysis of the two-channel atom-molecule effective Hamiltonian for an ultracold two-component homogeneous Fermi gas interacting near a Feshbach resonance. We particularly focus on the two-body and many-body properties of the dressed molecules in such a gas. An exact result for the many-body T matrix of the two-channel theory is derived by both considering coupled vertex equations and functional-integral methods. Making use of this result allows us to incorporate exactly into the many-body theory the two-body physics of the Feshbach scattering by means of simple analytical formulas without any fitting parameters. New interesting many-body effects are discussed in the case of narrow resonances. We give also a description of the BEC-BCS crossover above and below ${T}_{C}$. The effects of different approximations for the self-energy of the dressed molecules are discussed. The single-channel results are derived as a special limit for broad resonances. Moreover, through an analytic analysis of the BEC limit, the relation between the composite boson of the single-channel model and the dressed-molecule of the two-channel model is established.

DOI
10.1103/physreva.75.023612

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The use of Feshbach resonances in the field of ultracold gases has received a lot of attention recently. In first instance it was realized that these resonances can be used to alter the interaction strength in an atomic gas, by means of tuning an external magnetic field. Furthermore, by sweeping the magnetic field from one side of the resonance to the other, a degenerate gas of bosonic molecules can be created, a significant accomplishment. By making the interactions between fermionic atoms strongly attractive, a fermionic superfluid was recently made, a feat that has drawn a lot of attention in the physics community and from the media. We present work that describes these many-particle systems near a Feshbach resonance in a comprehensive way by using the concept of dressed molecules. These dressed molecules are essentially two-particle states that are a superposition of a tightly bound bare molecule, and two unbound bare atoms. This description reduces to the correct paired wave-function in the two-body limit. Moreover it gives a physically correct description of all the phenomena mentioned above: the Bose-condensation of a gas near a Feshbach resonance, that contains molecules, is more correctly interpreted as a Bose-condensation of dressed molecules. The fermionic superfluid contains a condensate of bosonic pairs, normally called Cooper pairs, that can be understood as the dressed molecules. For the latter case, the dressed-molecule picture also gives an elegant characterization of the crossover between a Bose condensate of pure molecules on one side of the resonance, to a fermionic Bardeen-Cooper-Schrieffer superfluid on the other side. Then, the dressed molecules change continuously from being mostly a bare molecule, to being mostly a loose pair of two atoms. It is clear that the nature of the dressed molecules is much determined by the probability for it to be in the bare-molecular state. This probability we denote with a single parameter Z. We present various ways of calculating it, and study how it affects the macroscopic physics.

•Feb 7, 2007•1 citation
We present a detailed analysis of the two-channel atom-molecule effective Hamiltonian for an ultracold two-component homogeneous Fermi gas interacting near a Feshbach resonance. We particularly focus on the two-body and many-body properties of the dressed molecules in such a gas. An exact result for the many-body T matrix of the two-channel theory is derived by both considering coupled vertex equations and functional-integral methods. Making use of this result allows us to incorporate exactly into the many-body theory the two-body physics of the Feshbach scattering by means of simple analytical formulas without any fitting parameters. New interesting many-body effects are discussed in the case of narrow resonances. We give also a description of the BEC-BCS crossover above and below TC{T}_{C}TC​. The effects of different approximations for the self-energy of the dressed molecules are discussed. The single-channel results are derived as a special limit for broad resonances. Moreover, through an analytic analysis of the BEC limit, the relation between the composite boson of the single-channel model and the dressed-molecule of the two-channel model is established.
A self-consistent theory is derived to describe the BCS--Bose-Einstein-condensate crossover for a strongly interacting Fermi gas with a Feshbach resonance. In the theory the fluctuation of the dressed molecules, consisting of both preformed Cooper pairs and ``bare'' Feshbach molecules, has been included within a self-consistent TTT-matrix approximation, beyond the Nozi\`eres and Schmitt-Rink strategy considered by Ohashi and Griffin. The resulting self-consistent equations are solved numerically to investigate the normal-state properties of the crossover at various resonance widths. It is found that the superfluid transition temperature Tc{T}_{c}Tc​ increases monotonically at all widths as the effective interaction between atoms becomes more attractive. Furthermore, a residue factor Zm{Z}_{m}Zm​ of the molecule's Green function and a complex effective mass have been determined to characterize the fraction and lifetime of Feshbach molecules at Tc{T}_{c}Tc​. Our many-body calculations of Zm{Z}_{m}Zm​ agree qualitatively well with recent measurments of the gas of 6Li^{6}\mathrm{Li}6Li atoms near the broad resonance at 834G834\phantom{\rule{0.3em}{0ex}}\mathrm{G}834G. The crossover from narrow to broad resonances has also been studied.
A Feshbach resonance in the s-wave scattering length occurs if the energy of the two atoms in the incoming open channel is close to the energy of a bound state in a coupled closed channel. Starting from the microscopic Hamiltonian that describes this situation, we derive the effective atom–molecule theory for a Bose gas near a Feshbach resonance. In order to take into account all two-body processes, we have to dress the bare couplings of the atom–molecule model with ladder diagrams. This results in a quantum field theory that exactly reproduces the scattering amplitude of the atoms and the bound-state energy of the molecules. Since these properties are incorporated at the quantum level, the theory can be applied both above and below the critical temperature of the gas. Moreover, making use of the true interatomic potentials ensures that no divergences are encountered at any stage of the calculation. We also present the mean-field theory for the Bose–Einstein condensed phase of the gas.
We analyze a system of two-component fermions, which interact via a Feshbach resonance in the presence of a three-dimensional lattice potential. By expressing a two-channel model of the resonance in the basis of Bloch states appropriate for the lattice, we derive an eigenvalue equation for the two-particle bound states, which is nonlinear in the energy eigenvalue. Compact expressions for the interchannel matrix elements, numerical methods for the solution of the nonlinear eigenvalue problem, and a renormalization procedure to remove ultraviolet divergences are presented. From the structure of the two-body solutions we identify the relevant degrees of freedom, which describe the resonance behavior in the lowest Bloch band. These degrees of freedom, which we call dressed molecules, form an effective closed channel in a many-body model of the resonance, the Fermi resonance Hamiltonian (FRH). It is shown how the properties of the FRH can be determined numerically by solving a projected lattice two-channel model at the two-particle level. As opposed to single-channel lattice models such as the Hubbard model, the FRH is valid for general sss-wave scattering length and resonance width. Hence, the FRH provides an accurate description of the BEC-BCS crossover for ultracold fermions on an optical lattice.
We investigate the non-universal behavior of the BCS-BEC crossover model at the normal to superfluid transition. By using a finite temperature quantum field theoretical approach due to Nozieres and Schmitt-Rink and by making the effective range expansion of the effective two-body interaction we numerically calculate the crossover transition temperature as a function of the scattering length, aF,a_{F},aF​, and the effective range parameter, re.r_{\mathrm{e}}.re​. In an ultracold two-component atomic Fermi gas BCS-BEC crossover physics is expected to appear near magnetic-field-induced Feshbach resonances. By matching two-body scattering properties near a Feshbach resonance to a simple renormalized model potential, a broad resonance is characterized by a small effective range and the gas displays a universal BCS-BEC crossover behavior. On the other hand, for a narrow resonance thermodynamic quantities depend the effective range which may be large and negative at resonance. For increasing values of −re-r_{\mathrm{e}}−re​ we find the transition temperature to be suppressed in the crossover region. We furthermore argue for existence of a lower bound of TcT_{c}Tc​ at fixed coupling for increasing −re-r_{\mathrm{e}}−re​ in the crossover region.
Fermionic superfluidity in atomic Fermi gases across a Feshbach resonance is normally described by the atom-molecule theory, which treats the closed channel as a noninteracting point boson. In this work we present a theoretical description of the resonant superfluidity in analogy to the two-band superconductors. We employ the underlying two-channel scattering model of Feshbach resonance where the closed channel is treated as a composite boson with binding energy ${\ensuremath{\varepsilon}}_{0}$ and the resonance is triggered by the microscopic interchannel coupling U12{U}_{12}U12​. The binding energy ${\ensuremath{\varepsilon}}_{0}$ naturally serves as an energy scale of the system, which has been sent to infinity in the atom-molecule theory. We show that the atom-molecule theory can be viewed as a leading-order low-energy effective theory of the underlying fermionic theory in the limit ${\ensuremath{\varepsilon}}_{0}\ensuremath{\rightarrow}\ensuremath{\infty}$ and ${U}_{12}\ensuremath{\rightarrow}0$, while keeping the phenomenological atom-molecule coupling finite. The resulting two-band description of the superfluid state is in analogy to the BCS theory of two-band superconductors. In the dilute limit ${\ensuremath{\varepsilon}}_{0}\ensuremath{\rightarrow}\ensuremath{\infty}$, the two-band description recovers precisely the atom-molecule theory. The two-band theory provides a natural approach to study the corrections because of a finite binding energy ${\ensuremath{\varepsilon}}_{0}$ in realistic experimental systems. For broad and moderate resonances, the correction is not important for current experimental densities. However, for extremely narrow resonance, we find that the correction becomes significant. The finite binding energy correction could be important for the stability of homogeneous polarized superfluid against phase separation in imbalanced Fermi gases across a narrow Feshbach resonance.
The use of Feshbach resonances in the field of ultracold gases has received a lot of attention recently. In first instance it was realized that these resonances can be used to alter the interaction strength in an atomic gas, by means of tuning an external magnetic field. Furthermore, by sweeping the magnetic field from one side of the resonance to the other, a degenerate gas of bosonic molecules can be created, a significant accomplishment. By making the interactions between fermionic atoms strongly attractive, a fermionic superfluid was recently made, a feat that has drawn a lot of attention in the physics community and from the media. We present work that describes these many-particle systems near a Feshbach resonance in a comprehensive way by using the concept of dressed molecules. These dressed molecules are essentially two-particle states that are a superposition of a tightly bound bare molecule, and two unbound bare atoms. This description reduces to the correct paired wave-function in the two-body limit. Moreover it gives a physically correct description of all the phenomena mentioned above: the Bose-condensation of a gas near a Feshbach resonance, that contains molecules, is more correctly interpreted as a Bose-condensation of dressed molecules. The fermionic superfluid contains a condensate of bosonic pairs, normally called Cooper pairs, that can be understood as the dressed molecules. For the latter case, the dressed-molecule picture also gives an elegant characterization of the crossover between a Bose condensate of pure molecules on one side of the resonance, to a fermionic Bardeen-Cooper-Schrieffer superfluid on the other side. Then, the dressed molecules change continuously from being mostly a bare molecule, to being mostly a loose pair of two atoms. It is clear that the nature of the dressed molecules is much determined by the probability for it to be in the bare-molecular state. This probability we denote with a single parameter Z. We present various ways of calculating it, and study how it affects the macroscopic physics.