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arXiv:cond-mat/0511230

Quantum oscillations in a two-mode atom-molecule Bose-Einstein condensate -- the discrete WKB approach

Jérôme Dorignac, Yu. B. Gaĭdideĭ, J. Chris Eilbeck, Peter Leth Christiansen, C. Katerji

Published Nov 9, 2005• 0 citations
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Abstract

Quantum effects in a system of coupled atomic and molecular Bose-Einstein condensates in the framework of a two-mode model are studied numerically and analytically, using the discrete WKB approach. In contrast to the mean-field approximation, the WKB analytical results are in a very good agreement with numerical results. The quantum fluctuations of the atomic and molecular populations are calculated, and found to be of the same order of magnitude as their mean values.

DOI
10.48550/arxiv.cond-mat/0511230

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Quantum effects in a system of coupled atomic and molecular Bose-Einstein condensates in the framework of a two-mode model are studied numerically and analytically, using the discrete WKB approach. In contrast to the mean-field approximation, the WKB analytical results are in a very good agreement with numerical results. The quantum fluctuations of the atomic and molecular populations are calculated, and found to be of the same order of magnitude as their mean values.
We study the system of coupled atomic and molecular condensates within the two-mode model and beyond mean-field theory. Large-amplitude atom-molecule coherent oscillations are shown to be damped by the rapid growth of fluctuations near the dynamically unstable molecular mode. This result contradicts earlier predictions about the recovery of atom-molecule oscillations in the two-mode limit. The frequency of the damped oscillation is also shown to scale as N/lnN\sqrt{N}/\mathrm{ln}NN​/lnN with the total number of atoms N, rather than the expected pure N\sqrt{N}N​ scaling. Using a linearized model, we obtain analytical expressions for the initial depletion of the molecular condensate in the vicinity of the instability, and show that the important effect neglected by mean-field theory is an initially nonexponential ``spontaneous'' dissociation into the atomic vacuum. Starting with a small population in the atomic mode, the initial dissociation rate is sensitive to the exact atomic amplitudes, with the fastest (superexponential) rate observed for the entangled state formed by spontaneous dissociation.
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A study of coherent photoassociation is presented for the case of an atomic Bose-Einstein condensate. It is shown that the phenomenon is analogous to coherent optical transient in a few-level system, with a difference that the participating levels have Bose enhanced populations. A second-quantized Hamiltonian in momentum and position representation is developed to describe photoassociation. A classical version of the field theory for atoms and molecules is used to demonstrate that in the presence of photoassociating light, a joint atom-molecule condensate is unstable against the growth of the density fluctuations. ^ A simple mean-field model of atom-molecule Bose-Einstein condensate is constructed and it is shown that in the model there is no collapse, irrespective of the sign of the effective atom-atom scattering length. The properties of the two most important eigenstates, the ground state and the twin state, are determined for different values of the system parameters δ and K, the detuning and the atom-molecule coupling, respectively. It is shown that in a coupled atom-molecule system a collapse is replaced by a dynamical instability. The lines in the parameter space where these instabilities occur are in fact fractures where the underlying eigenstates discontinuously change. The features of instability are in good qualitative agreement with the experimental observations of collapse. ^
We analyze the coherent multimode dynamics of a system of coupled atomic and molecular Bose gases. Starting from an atomic Bose-Einstein condensate with a small thermal component, we observe a complete depletion of the atomic and molecular condensate modes on a short time scale due to a significant population of excited states. Giant coherent oscillations between the two condensates for typical parameters are almost completely suppressed. Our results cast serious doubts on the common use of the 2-mode model for the description of coupled ultracold atomic-molecular systems and should be considered when planning future experiments with ultracold molecules.
Abstract We investigate the chaotic dynamics of a coupled three-level atom–molecular Bose–Einstein condensate system composed by one molecular mode and two atomic modes. With the increase of atom–molecular coupling strength, we reveal the emergence of chaotic oscillations of the relative population difference between two atomic modes, which can be proven by the broad windows with a huge number of frequencies in spectral density and the chaotic trajectories in phase space diagrams. The different effects of initial states on atomic population oscillations are revealed, where for more particles in the initial state of the molecular model, chaos appears in the larger parameter region of system dynamics. Furthermore, we find that strong intermolecular interaction strength can suppress chaos resulting from strong atom–molecule coupling. This is due to the difficult transformation between atomic and molecular modes, as well as the relatively independent dynamic evolution of atoms and molecules.
Bose-Einstein condensate (BEC) is considered under conditions of Feshbach resonance in two-atom collisions due to a coupling of atomic pair and resonant molecular states. The association of condensate atoms can form a molecular BEC, and the molecules can dissociate to pairs of entangled atoms in two-mode squeezed states. Both entanglement and squeezing can be applied to quantum measurements and information processing. The processes in the atom-molecule quantum gas are analyzed using two theoretical approaches. The mean-field one takes into account deactivating collisions of resonant molecules with other atoms and molecules, neglecting quantum fluctuations. This method allows analysis of inhomogeneous systems, such as expanding BEC. The non-mean-field approach -- the parametric approximation -- takes into account both deactivation and quantum fluctuations. This method allows determination of optimal conditions for formation of molecular BEC and describes Bose-enhanced dissociation of molecular BEC, as well as entanglement and squeezing of the non-condensate atoms.