We show that the ground state of disordered rotor models with quadrupolar interactions can exhibit biaxial nematic ordering in the disorder-averaged sense. We present a mean-field analysis of the model and demonstrate that the biaxial phase is stable against small quantum fluctuations. We point out the possibility of experimental realization of such rotor models using ultracold spin-1 Bose atoms in a spin-dependent and disordered optical lattice in the limit of a large number of atoms per site and also suggest an imaging experiment to detect the biaxial nematicity in such systems.
We show that the ground state of disordered rotor models with quadrupolar interactions can exhibit biaxial nematic ordering in the disorder-averaged sense. We present a mean-field analysis of the model and demonstrate that the biaxial phase is stable against small quantum fluctuations. We point out the possibility of experimental realization of such rotor models using ultracold spin-1 Bose atoms in a spin-dependent and disordered optical lattice in the limit of a large number of atoms per site and also suggest an imaging experiment to detect the biaxial nematicity in such systems.
In this thesis, we investigate strongly correlated phenomena in quantum spin systems. In the first part of this work, we study geometrically frustrated antiferromagnets (AFMs). Generalizing the SU(2) Heisenberg Hamiltonian to Sp(N) symmetry, we obtain, in the large-N limit, the mean-field phase diagrams for the planar pyrochlore and cubic AFMs. We then use gauge theories to consider fluctuation effects about their respective mean-field configurations. We find, in addition to conventional Neel states, a plethora of novel magnetically disordered phases: two kinds of spin liquids, Z2 in 2+1D and U(1)in 3+1D, and several valence bond solids such as two and three-dimensional plaquette and columnar singlet states. We use the same approach to study the diamond lattice AFM which possesses extended classical ground state degeneracy. We demonstrate that quantum and entropic fluctuations lift this degeneracy in different ways. In the second part of the thesis, we study ultracold spinor atoms confined in optical lattices. We first demonstrate the feasibility of experimental realization of rotor models using ultracold spin-one Bose atoms in a spin-dependent and disordered optical lattice. We show that the ground state of such disordered rotor models with quadrupolar interactions can exhibit biaxial nematic ordering in the disorder-averaged sense, and suggest an imaging experiment to detect the biaxial nematicity in such systems. Finally, using variational wavefunction methods, we study the Mott phases and superfluid-insulator transition of spin-three bosons in an optical lattice with an anisotropic two dimensional optical trap. We chart out the phase diagrams for Mott states with n = 1 and n = 2 atoms per lattice site. We show that the long-range dipolar interaction stabilizes a state characterized by antiferromagnetic chains made of ferromagnetically aligned spins. We also obtain the mean-field phase boundary for the superfluid-insulator transition, and show that inside the superfluid phase and near the superfluid-insulator phase boundary, the system undergoes a first order antiferromagnetic-ferromagnetic spin ordering transition.
We consider quantum phases of tightly confined spin-2 bosons in an external field under the presence of rotationally invariant interactions. Generalizing previous treatments, we show how this system can be mapped onto a quantum rotor model. Within the rotor framework, low-energy excitations about fragmented states, which cannot be accessed within standard Bogoliubov theory, can be obtained. In the spatially extended system in the thermodynamic limit there exists a mean field ground-state degeneracy between a family of nematic states for appropriate interaction parameters. It has been established that quantum fluctuations lift this degeneracy through the mechanism of order by disorder and select either a uniaxial or square-biaxial ground state. On the other hand, in the full quantum treatment of the analogous single-spatial-mode problem with finite-particle number, it is known that, due to symmetry-restoring fluctuations, there is a unique ground state across the entire nematic region of the phase diagram. Within the established rotor framework, we investigate the possible quantum phases under the presence of a quadratic Zeeman field, a problem which has previously received little attention. By investigating wave-function overlaps, we do not find any signatures of the order-by-disorder phenomenon which is present in the continuum case. Motivated by this, we consider an alternative external potential which breaks less symmetry than the quadratic Zeeman field. For this case, we do find the phenomenon of order by disorder in the fully quantum system. This is established within the rotor framework and with exact diagonalization.
We show that quantum and thermal fluctuations in spin-2 Bose-Einstein condensates lift the accidental degeneracy of the mean-field phase diagram. Fluctuations select the uniaxial (square biaxial) nematic state for scattering lengths a4>a2 (a4<a2). Paradoxically, the order is stronger at higher temperatures. For spin-2 87Rb and 23Na, a continuous Ising-type transition is predicted on raising the magnetic field, from a fluctuation stabilized uniaxial state to a field stabilized square biaxial order state. This is a promising experimental system to realize the "order-by-disorder" phenomenon.
We present a theory of the anisotropy-tuned quantum phase transition between spin-nematic and spin-Peierls phases in S=1 systems with significant biquadratic exchange interactions. Based on quantum Monte Carlo studies on finite-size systems, it has been proposed that this phase transition is second order with new deconfined fractional excitations that are absent in either of the two phases. The possibility of a weak first-order transition, however, cannot be ruled out. To elucidate the nature of the transition, we construct a large-NSO(3N) model for this phase transition and find in the $N\ensuremath{\rightarrow}\ensuremath{\infty}$ limit that the transition is generically of first-order. Furthermore, we find a critical point in the one-dimensional (1D) limit, where two transition lines, separating spin-nematic, ferromagnetic, and spin-Peierls phases, meet. Our study indicates that the spin-nematic phase is absent in 1D, while its correlation length diverges at the critical point. Predictions for 23Na atoms trapped in an optical lattice, where the nematic to spin-Peierls quantum phase transition naturally arises are discussed.
We explore several classes of quadrupolar ordering in a system of antiferromagnetically coupled quantum spin-1 dimers, which are stacked in the triangular lattice geometry forming a bilayer. Low-energy properties of this model are described by an S=1 hard-core bosonic degrees of freedom defined on each dimer bond, where the singlet and triplet states of the dimerized spins are interpreted as the vacuum and the occupancy of boson, respectively. The number of bosons per dimer and the magnetic and density fluctuations of bosons are controlled by the interdimer Heisenberg interactions. In a solid phase where each dimer hosts one boson and the interdimer interaction is weak, a conventional spin nematic phase is realized by the pair fluctuation of bosons. Larger interdimer interaction favors Bose-Einstein condensates (BEC) carrying quadrupolar moments. Among them, we find one exotic phase where the quadrupoles develop a spatially modulated structure on the top of a uniform BEC, interpreted in the original dimerized spin-1 model as coexistent p-type nematic and ${120}^{\ensuremath{\circ}}$ magnetic correlations. This may explain an intriguing nonmagnetic phase found in Ba3ZnRu2O9.
We study magnetically stabilized nematic order for spin-one bosons in optical lattices. We show that the Zeeman field-driven quantum phase transitions between non-nematic Mott states and quantum spin nematic Mott states in the weak hopping limit are in the universality class of the ferromagnetic XXZ(S=1∕2) spin model. We further discuss these transitions as condensation of interacting magnons. The development of O(2) nematic order when external fields are applied corresponds to condensation of magnons, which breaks a U(1) symmetry. Microscopically, this results from a coherent superposition of two non-nematic states at each individual site. Nematic order and spin-wave excitations around critical points are studied and critical behaviors are obtained in a dilute gas approximation. We also find that spin-singlet states are unstable with respect to quadratic Zeeman effects and Ising nematic order appears in the presence of any finite quadratic Zeeman coupling. All discussions are carried out for states in three-dimensional bipartite lattices.