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arXiv:cond-mat/0508637 · Physical Review B

Ordering of geometrically frustrated classical and quantum triangular Ising magnets

Ying Yan Jiang, Thorsten Emig A

Published Mar 31, 2006• 23 citations
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Abstract

A systematic study of both classical and quantum geometric frustrated Ising models with a competing ordering mechanism is reported in this paper. The ordering comes in the classical case from a coupling of two-dimensional (2D) layers and in the quantum model from the quantum dynamics induced by a transverse field. By mapping the Ising models on a triangular lattice to elastic lattices of noncrossing strings, we derive an exact relation between the spin variables and the displacement field of the strings. Using this map for both the classical $(2+1)\mathrm{D}$ stacked model and the quantum frustrated 2D system, we obtain a microscopic derivation of an effective Hamiltonian which was proposed before on phenomenological grounds within a Landau-Ginzburg-Wilson approach. In contrast to the latter approach, our derivation provides the coupling constants and hence the entire transverse field-versus-temperature phase diagram can be deduced, including the universality classes of both the quantum and the finite-temperature transitions. The structure of the ordered phase is obtained from a detailed entropy argument. We compare our predictions to recent simulations of the quantum system and find good agreement. We also analyze the connections to a dimer model on the hexagonal lattice and its height profile representation, providing a simple derivation of the continuum free energy and a physical explanation for the universality of the stiffness of the height profile for anisotropic couplings.

DOI
10.1103/physrevb.73.104452

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A systematic study of both classical and quantum geometric frustrated Ising models with a competing ordering mechanism is reported in this paper. The ordering comes in the classical case from a coupling of two-dimensional (2D) layers and in the quantum model from the quantum dynamics induced by a transverse field. By mapping the Ising models on a triangular lattice to elastic lattices of noncrossing strings, we derive an exact relation between the spin variables and the displacement field of the strings. Using this map for both the classical (2+1)D(2+1)\mathrm{D}(2+1)D stacked model and the quantum frustrated 2D system, we obtain a microscopic derivation of an effective Hamiltonian which was proposed before on phenomenological grounds within a Landau-Ginzburg-Wilson approach. In contrast to the latter approach, our derivation provides the coupling constants and hence the entire transverse field-versus-temperature phase diagram can be deduced, including the universality classes of both the quantum and the finite-temperature transitions. The structure of the ordered phase is obtained from a detailed entropy argument. We compare our predictions to recent simulations of the quantum system and find good agreement. We also analyze the connections to a dimer model on the hexagonal lattice and its height profile representation, providing a simple derivation of the continuum free energy and a physical explanation for the universality of the stiffness of the height profile for anisotropic couplings.
We report on a systematic study of two-dimensional, periodic, frustrated Ising models with quantum dynamics introduced via a transverse magnetic field. The systems studied are the triangular and kagom\'e lattice antiferromagnets, fully frustrated models on the square and hexagonal (honeycomb) lattices, a planar analog of the pyrochlore antiferromagnet, a pentagonal lattice antiferromagnet, as well as two quasi-one-dimensional lattices that have considerable pedagogical value. All of these exhibit a macroscopic degeneracy at T=0T=0T=0 in the absence of the transverse field, which enters as a singular perturbation. We analyze these systems with a combination of a variational method at weak fields, a perturbative Landau-Ginzburg-Wilson approach from large fields, as well as quantum Monte Carlo simulations utilizing a cluster algorithm. Our results include instances of quantum order arising from classical criticality (triangular lattice) or classical disorder (pentagonal and probably hexagonal) as well as notable instances of quantum disorder arising from classical disorder (kagom\'e). We also discuss the effect of finite temperature, as well as the interplay between longitudinal and transverse fields---in the kagom\'e problem the latter gives rise to a nontrivial phase diagram with bond-ordered and bond-critical phases in addition to the disordered phase. We also note connections to quantum-dimer models and thereby to the physics of Heisenberg antiferromagnets in short-ranged resonating valence-bond phases that have been invoked in discussions of high-temperature superconductivity.
We study the effect of quantum dynamics on geometrically frustrated magnets for a transverse field Ising model at finite temperatures. We develop a microscopic derivation of the Landau-Ginzburg-Wilson action for this model and show that it can be interpreted as the free energy of a 3D elastic lattice of noncrossing strings. As a first application, we quantitatively predict the phase diagram and correlations, confirming excellently a key prediction of recent simulations about the existence of unusual phase transitions and an ordered phase. We discuss the implications of our string picture for the understanding of the effect of quenched disorder in such quantum frustrated systems.
Geometric frustration in two-dimensional Ising models allows for a wealth of exotic universal behavior, both Ising and non-Ising, in the presence of quantum fluctuations. In particular, the triangular antiferromagnet and Villain model in a transverse field can be understood through distinct XY pseudospins, but have qualitatively similar phase diagrams including a quantum phase transition in the (2+1)-dimensional XY universality class. While the quantum dynamics of modestly-sized systems can be simulated classically using tensor-based methods, these methods become infeasible for larger lattices. Here we perform both classical and quantum simulations of these dynamics, where our quantum simulator is a superconducting quantum annealer. Our observations on the triangular lattice suggest that the dominant quench dynamics are not described by the quantum Kibble-Zurek scaling of the quantum phase transition, but rather a faster coarsening dynamics in an effective two-dimensional XY model in the ordered phase. Similarly, on the Villain model, the scaling exponent does not match the Kibble-Zurek expectation. These results demonstrate the ability of quantum annealers to perform coherent quantum dynamics simulations that are hard to classically scale beyond small systems, and open the avenue to predictive simulations of the dynamics of Ising magnetic materials on quantum simulators.
We investigate the interplay of classical degeneracy and quantum dynamics in a range of periodic frustrated transverse field Ising systems at zero temperature. We find that such dynamics can lead to unusual ordered phases and phase transitions or to a quantum spin liquid (cooperative paramagnetic) phase as in the triangular and kagome lattice antiferromagnets, respectively. For the latter, we further predict passage to a bond-ordered phase followed by a critical phase as the field is tilted. These systems also provide exact realizations of quantum dimer models introduced in studies of high temperature superconductivity.
In this work the ordering processes in classical frustrated Ising models and the ground-state behavior of frustrated quantum spin models are investigated. In the first part the phase transition from a high-temperature paramagnetic phase to a antiferromagnetic ground state is analyzed for the square-lattice Ising model with competing antiferromagnetic interactions between nearest- and next-nearest-neighbor spins. In the case of spatially isotropic interactions the phase transition to a collinear state is of special interest. Using Monte-Carlo simulations on finite lattices as well as field-theoretical methods for the continuous model it is shown that depending on the frustration three different sectors can be distinguished that show (i) Ising-universal behavior (ii) Ashkin-Teller-like non-universal behavior (varying critical exponents) and (iii) non-critical first-order behavior. For spatially anisotropic interactions the emergence of an intermediate incommensurate phase is verified by means of Monte-Carlo simulations which has been predicted by earlier mean-field calculations. The nature of this phase is studied analyzing spin-spin correlation functions and its ordering wave-vector reveals a strong temperature and size dependence. In the second part the influence of quantum fluctuations on classical antiferromagnetic ground states are investigated in anisotropic quantum spin-1/2 Heisenberg models with competing interactions. Using quantum Monte-Carlo simulations, exact diagonalization and perturbation theory the ground-state phase diagrams are calculated for a square lattice with nearest- and next-nearest-neighbor interactions and a honeycomb lattice with up to third-nearest-neighbor interactions whereby the fluctuations are chosen to be non-frustrating. For both cases the stability regions of classical magnetic states are identified and an intermediate phase is detected that shows no sign of long-range magnetic order. Further calculations also rule out valence-bond-crystal or topological order for this state, thus a quantum disordered ground state is stabilized in these models.
The quantum antiferromagnetic spin-1/2 Ising model on a triangular lattice and analogous fully frustrated Ising model on a square lattice with quantum fluctuation induced by the application of the transverse magnetic field are studied at finite temperatures by constructing an exact mapping onto a purely classical model with a more complex interaction. It is shown that in weak fields the temperatures of the phase transitions separating the critical phase from the ordered and disordered phases in both models are proportional to the magnitude of the field.