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arXiv:cond-mat/0507010 · Physical Review Letters

Absence of Single-Particle Bose-Einstein Condensation at Low Densities for Bosons with Correlated Hopping

Rachel Bendjama, Brijesh Kumar, Frédéric Mila

Published Sep 9, 2005• 24 citations
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Abstract

Motivated by the physics of mobile triplets in frustrated quantum magnets, the properties of a two-dimensional model of bosons with correlated hopping are investigated. A mean-field analysis reveals the presence of a pairing phase without single-particle Bose-Einstein condensation (BEC) at low densities for sufficiently strong correlated hopping, and of an Ising quantum phase transition towards a BEC phase at larger density. The physical arguments supporting the mean-field results and their implications for bosonic and quantum spin systems are discussed.

DOI
10.1103/physrevlett.95.110406

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Motivated by the physics of mobile triplets in frustrated quantum magnets, the properties of a two-dimensional model of bosons with correlated hopping are investigated. A mean-field analysis reveals the presence of a pairing phase without single-particle Bose-Einstein condensation (BEC) at low densities for sufficiently strong correlated hopping, and of an Ising quantum phase transition towards a BEC phase at larger density. The physical arguments supporting the mean-field results and their implications for bosonic and quantum spin systems are discussed.
We investigate the consequences of correlated hopping on the ground state properties of hard-core bosons on a square lattice as revealed by extensive exact diagonalizations and quantum Monte Carlo simulations. While for noninteracting hard-core bosons the effective attraction induced by the correlated hopping leads to phase separation at low density, we show that a modest nearest-neighbor repulsion suppresses phase separation, leading to a remarkable low-density pairing phase with no single particle Bose-Einstein condensation but long-range two-particle correlations, signaling a condensation of pairs. We also explain why the unusual properties of the pairing phase are a real challenge for standard one-worm quantum Monte Carlo simulations.
We formulate a bosonic dynamical mean-field theory (B-DMFT) which provides a comprehensive, thermodynamically consistent framework for the theoretical investigation of correlated lattice bosons. The B-DMFT is applicable for arbitrary values of the coupling parameters and temperature and becomes exact in the limit of high spatial dimensions ddd or coordination number ZZZ of the lattice. In contrast to its fermionic counterpart, the construction of the B-DMFT requires different scalings of the hopping amplitudes with ZZZ depending on whether the bosons are in their normal state or in the Bose-Einstein condensate (BEC). A detailed discussion of how this conceptual problem can be overcome by performing the scaling in the action rather than in the Hamiltonian itself is presented. The B-DMFT treats normal and condensed bosons on equal footing and thus includes the effects caused by their dynamic coupling. It reproduces all previously investigated limits in parameter space, such as the Beliaev-Popov and Hartree-Fock-Bogoliubov approximations, and generalizes the existing mean-field theories of interacting bosons. The self-consistency equations of the B-DMFT are those of a bosonic single-impurity coupled to two reservoirs corresponding to bosons in the condensate and in the normal state, respectively. We employ the B-DMFT to solve a model of itinerant and localized, interacting bosons analytically. The local correlations are found to enhance the condensate density and the BEC transition temperature TBEC{T}_{\text{BEC}}TBEC​. This effect may be used experimentally to increase TBEC{T}_{\text{BEC}}TBEC​ of bosonic atoms in optical lattices.
We present a phase diagram for a dilute two-dimensional Bose gas on a lattice. For one sort of boson we consider a realistic case of the van der Waals interaction between particles with a strong hard-core repulsion U and a van der Waals attractive tail V. For V<2t,V<2t,V<2t, t being a hopping amplitude, the phase diagram of the system contains regions of usual one-particle Bose-Einstein condensation (BEC). However for V>2tV>2tV>2t we have total phase separation on a Mott-Hubbard Bose solid and a dilute Bose gas. For two sorts of structureless bosons described by the two-band Hubbard model, an s-wave pairing of the two bosons of different sort $〈{b}_{1}{b}_{2}〉\ensuremath{\ne}0$ is possible. The results we obtained should be important for different Bose systems, including submonolayers of 4He,{}^{4}\mathrm{He},4He, excitons in semiconductors, Schwinger bosons in magnetic systems and holons in HTSC. In the HTSC case a possibility of two-holon pairing in the slave-boson theories of superconductivity can restore a required charge 2e2e2e of a Cooper pair.
The ground states of Bose-Einstein condensates (BECs) of spin-2 bosons are classified into three distinct phases (ferromagnetic, ``antiferromagnetic,'' and cyclic) depending on the s-wave scattering lengths of binary collisions for total-spin 0, 2, and 4 channels. Many-body spin correlations and magnetic response of the condensate in each of these phases are studied in a mesoscopic regime, while low-lying excitation spectra are investigated in the thermodynamic regime. In the mesoscopic regime, where the system is so tightly confined that the spatial degrees of freedom are frozen, the exact, many-body ground state for each phase is found to be expressed in terms of the creation operators of pair or trio bosons having spin correlations. These pairwise and trio-wise units are shown to bring about some unique features of spin-2 BECs such as a huge jump in magnetization from minimum to maximum possible values and the robustness of the minimum-magnetization state against an applied magnetic field. In the thermodynamic regime, where the system is spatially uniform, low-lying excitation spectra in the presence of magnetic field are obtained analytically using the Bogoliubov approximation. In the ferromagnetic phase, the excitation spectrum consists of one Goldstone mode and four single-particle modes. In the antiferromagnetic phase, where spin-singlet ``pairs'' undergo Bose-Einstein condensation, the spectrum consists of two Goldstone modes and three massive ones, all of which become massless when magnetic field vanishes. In the cyclic phase, where boson ``trios'' condense into a spin-singlet state, the spectrum is characterized by two Goldstone modes, one single-particle mode having a magnetic-field-independent energy gap, and a gapless single-particle mode that becomes massless in the absence of magnetic field.