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arXiv:cond-mat/0506282 · Physical Review Letters

Dressed Feshbach Molecules in the BEC-BCS Crossover

M. W. J. Romans, Henk T. C. Stoof

Published Dec 28, 2005• 29 citations
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Abstract

We present the random phase approximation (RPA) theory of the Bose-Einstein-condensation-Bardeen-Cooper-Schrieffer crossover in an atomic Fermi gas near a Feshbach resonance that includes the relevant two-body atomic physics exactly. This allows us to determine the probability for the dressed molecules in the Bose-Einstein condensate to be in the closed channel of the Feshbach resonance and to compare with the recent experiments of Partridge et al. [95, 020404 (2005)10.1103/PhysRevLett.95.020404] with , who have measured the same quantity.

DOI
10.1103/physrevlett.95.260407

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We present the random phase approximation (RPA) theory of the Bose-Einstein-condensation-Bardeen-Cooper-Schrieffer crossover in an atomic Fermi gas near a Feshbach resonance that includes the relevant two-body atomic physics exactly. This allows us to determine the probability for the dressed molecules in the Bose-Einstein condensate to be in the closed channel of the Feshbach resonance and to compare with the recent experiments of Partridge et al. [95, 020404 (2005)10.1103/PhysRevLett.95.020404] with , who have measured the same quantity.
We study the crossover of a quasi-two-dimensional Fermi gas trapped in the radial plane from the Bardeen-Cooper-Schrieffer (BCS) regime to the Bose-Einstein condensation (BEC) regime by crossing a wide Feshbach resonance. We consider two effective two-dimensional Hamiltonians within the mean-field level, and calculate the zero-temperature cloud size and number density distribution. For a model 1 Hamiltonian with renormalized atom-atom interaction, we observe a constant cloud size for arbitrary detunings. For a model 2 Hamiltonian with renormalized interactions between atoms and dressed molecules, the cloud size deceases from the BCS to BEC side, which is consistent with the picture of BCS-BEC crossover. This qualitative discrepancy between the two models indicates that the inclusion of dressed molecules is essential for a mean-field description of quasi-two-dimensional Fermi systems, especially on the BEC side of the Feshbach resonance.
A self-consistent theory is derived to describe the BCS--Bose-Einstein-condensate crossover for a strongly interacting Fermi gas with a Feshbach resonance. In the theory the fluctuation of the dressed molecules, consisting of both preformed Cooper pairs and ``bare'' Feshbach molecules, has been included within a self-consistent TTT-matrix approximation, beyond the Nozi\`eres and Schmitt-Rink strategy considered by Ohashi and Griffin. The resulting self-consistent equations are solved numerically to investigate the normal-state properties of the crossover at various resonance widths. It is found that the superfluid transition temperature Tc{T}_{c}Tc​ increases monotonically at all widths as the effective interaction between atoms becomes more attractive. Furthermore, a residue factor Zm{Z}_{m}Zm​ of the molecule's Green function and a complex effective mass have been determined to characterize the fraction and lifetime of Feshbach molecules at Tc{T}_{c}Tc​. Our many-body calculations of Zm{Z}_{m}Zm​ agree qualitatively well with recent measurments of the gas of 6Li^{6}\mathrm{Li}6Li atoms near the broad resonance at 834G834\phantom{\rule{0.3em}{0ex}}\mathrm{G}834G. The crossover from narrow to broad resonances has also been studied.
We present the Bogoliubov theory for the Bose-Einstein condensation of Feshbach molecules in a balanced Fermi mixture. Because the Bogoliubov theory includes (Gaussian) fluctuations, we can in this manner accurately incorporate both the two-body and many-body aspects of the BEC-BCS crossover that occurs near a Feshbach resonance. We apply the theory in particular to the very broad Feshbach resonance in atomic 6Li^{6}\mathrm{Li}6Li at a magnetic field of B0=834G{B}_{0}=834\phantom{\rule{0.3em}{0ex}}\mathrm{G}B0​=834G and find good agreement with experiments in that case. The BEC-BCS crossover for more narrow Feshbach resonances is also discussed.
We discuss the superfluid phase transition in a gas of Fermi atoms with a Feshbach resonance. A tunable pairing interaction associated with the Feshbach resonance is shown to naturally lead to the BCS-BEC crossover, where the character of superfluidity continuously changes from the weak-coupling Bardeen-Cooper-Schrieffer (BCS) type to the Bose-Einstein condensation (BEC) of tightly bound molecules, as one decreases the threshold energy 2ν of the Feshbach resonance. We also discuss effects of a trap, as well as the p-wave BCS-BEC crossover adjusted by a p-wave Feshbach resonance.
The use of Feshbach resonances in the field of ultracold gases has received a lot of attention recently. In first instance it was realized that these resonances can be used to alter the interaction strength in an atomic gas, by means of tuning an external magnetic field. Furthermore, by sweeping the magnetic field from one side of the resonance to the other, a degenerate gas of bosonic molecules can be created, a significant accomplishment. By making the interactions between fermionic atoms strongly attractive, a fermionic superfluid was recently made, a feat that has drawn a lot of attention in the physics community and from the media. We present work that describes these many-particle systems near a Feshbach resonance in a comprehensive way by using the concept of dressed molecules. These dressed molecules are essentially two-particle states that are a superposition of a tightly bound bare molecule, and two unbound bare atoms. This description reduces to the correct paired wave-function in the two-body limit. Moreover it gives a physically correct description of all the phenomena mentioned above: the Bose-condensation of a gas near a Feshbach resonance, that contains molecules, is more correctly interpreted as a Bose-condensation of dressed molecules. The fermionic superfluid contains a condensate of bosonic pairs, normally called Cooper pairs, that can be understood as the dressed molecules. For the latter case, the dressed-molecule picture also gives an elegant characterization of the crossover between a Bose condensate of pure molecules on one side of the resonance, to a fermionic Bardeen-Cooper-Schrieffer superfluid on the other side. Then, the dressed molecules change continuously from being mostly a bare molecule, to being mostly a loose pair of two atoms. It is clear that the nature of the dressed molecules is much determined by the probability for it to be in the bare-molecular state. This probability we denote with a single parameter Z. We present various ways of calculating it, and study how it affects the macroscopic physics.
We investigate the Bose-Einstein condensation of fermionic pairs in a uniform two-component Fermi gas, obtaining an explicit formula for the condensate density as a function of the chemical potential and the energy gap. We analyze the condensate fraction in the crossover from the Bardeen-Cooper-Schrieffer (BCS) state of weakly interacting Cooper pairs to the Bose-Einstein condensate of molecular dimers. By using the local-density approximation we study confined Fermi vapors of alkali-metal atoms for which there is experimental evidence of condensation also on the BCS side of the Feshbach resonance. Our theoretical results are in agreement with these experimental data and give the behavior of the condensate on both sides of the Feshbach resonance at zero temperature.