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arXiv:cond-mat/0505024 · Laser Physics Letters

Absence of spin superradiance in resonatorless magnets

Vyacheslav I. Yukalov, Elizaveta P. Yukalova

Published Dec 16, 2004• 17 citations

Abstract

A spin system is considered with a Hamiltonian typical of molecular magnets, having dipole-dipole interactions and a single-site magnetic anisotropy. In addition, spin interactions through the common radiation field are included. A fully quantum-mechanical derivation of the collective radiation rate is presented. An effective narrowing of the dipole-dipole attenuation, due to high spin polarization is taken into account. The influence of the radiation rate on spin dynamics is carefully analysed. It is shown that this influence is completely negligible. No noticeable collective effects, such as superradiance, can appear in molecular magnets, being caused by electromagnetic spin radiation. Spin superradiance can arise in molecular magnets only when these are coupled to a resonant electric circuit, as has been suggested earlier by one of the authors in Laser Phys. 12, 1089 (2002).

DOI: 10.1002/lapl.200410170

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The main part of this review is devoted to the comprehensive description of coherent radiation by nuclear spins. The theory of nuclear spin superradiance is developed and the experimental observations of this phenomenon are considered. The intriguing problem of how coherence develops from initially incoherent quantum fluctuations is analysed. All main types of coherent radiation by nuclear spins are discussed, which are: free nuclear induction, collective induction, maser generation, pure superradiance, triggered superradiance, pulsing superradiance, punctuated superradiance, and induced emission. The influence of electron-nuclear hyperfine interactions and the role of magnetic anisotropy are studied. Conditions for realizing spin superradiance by magnetic molecules are investigated. The possibility of nuclear matter lasing, accompanied by pion or dibaryon radiation, is briefly touched.