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arXiv:cond-mat/0503631

Superfluid Weight, Free Carrier Density, and Specific Heat of the d=3 tJ Model at Finite Temperatures

Michael Hinczewski, A. Nihat Berker

Published Mar 28, 2005• 0 citations
arXivHTMLPDF

Abstract

The superfluid weight, free carrier density, and specific heat of the three-dimensional tJ model are calculated by renormalization-group theory. We find that optimal hole doping for superfluidity occurs in the electron density range of n_i approximately between 0.63 - 0.68, where the superfluid weight n_s/m* reaches a local maximum. This density range is within the novel tau phase, where the electron hopping strength renormalizes to infinity, the system remains partially filled at all length scales, and the electron-hopping expectation value remains distinctively non-zero at all length scales. The calculated superfluid weight drops off sharply in the overdoped region. Under hole doping, the calculated density of free carriers increases until optimal doping and remains approximately constant in the overdoped region, as seen experimentally in high-T_c materials. Furthermore, from calculation of the specific heat coefficient gamma, we see clear evidence of a gap in the excitation spectrum for the tau phase.

DOI
10.48550/arxiv.cond-mat/0503631

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The superfluid weight, free carrier density, and specific heat of the three-dimensional tJ model are calculated by renormalization-group theory. We find that optimal hole doping for superfluidity occurs in the electron density range of n_i approximately between 0.63 - 0.68, where the superfluid weight n_s/m* reaches a local maximum. This density range is within the novel tau phase, where the electron hopping strength renormalizes to infinity, the system remains partially filled at all length scales, and the electron-hopping expectation value remains distinctively non-zero at all length scales. The calculated superfluid weight drops off sharply in the overdoped region. Under hole doping, the calculated density of free carriers increases until optimal doping and remains approximately constant in the overdoped region, as seen experimentally in high-T_c materials. Furthermore, from calculation of the specific heat coefficient gamma, we see clear evidence of a gap in the excitation spectrum for the tau phase.
Based on an improved U(1) slave-boson approach to the t-J Hamiltonian, we invest igate a relationship between the superfluid weight ns/m∗n_s/m^*ns​/m∗(the superconducting charge carrier density/the effective mass of the charge carrier) and the superc onducting temperature TcT_cTc​. From the present study we find a linear increase of ns/m∗n_s/m^*ns​/m∗ with TcT_cTc​ with th e doping concentration in the underdoped region, a saturation around the optimal doping and a decrease in both ns/m∗n_s/m^*ns​/m∗ and TcT_cTc​ in the overdoped region. Such a trend of the `boomerang' shaped locus in ns/m∗n_s/m^*ns​/m∗ vs. TcT_cTc​ with increas ing doping concentration from the underdoped to the heavily overdoped region is predicted to be in complete agreement with muon-spin-relaxation measurements. The boomerang behavior is found to occur in correlation with reduction in the sp in singlet pairing(spinon pairing) order in the heavily overdoped region.
Using the improved U(1) and SU(2) slave-boson approaches of the $t\ensuremath{-}J$ Hamiltonian [S.-S. Lee and Sung-Ho Suck Salk, Phys. Rev. B 64, 052501 (2001)] that we developed recently, we study the doping and temperature dependence of superfluid weight and spectral function and discuss our finding of the universal scaling behavior of the pseudogap. It is shown that at low hole doping concentrations xxx and at low temperatures TTT, there exists a propensity of linear decrease in the superfluid weight ns∕m∗{n}_{s}∕{m}^{*}ns​∕m∗ with temperature TTT, and a tendency of doping independence in the linearly decreasing slopes of (ns∕m∗)(x,T)({n}_{s}∕{m}^{*})(x,T)(ns​∕m∗)(x,T) with TTT in qualitative agreement with the experimentally observed relation; that is, $({n}_{s}∕{m}^{*})(x,T)=({n}_{s}∕{m}^{*})(x,0)\ensuremath{-}\ensuremath{\alpha}T$, where $\ensuremath{\alpha}$ is a constant. It is also demonstrated that there exists a boomerang behavior; that is, both Tc{T}_{c}Tc​ and ns∕m∗{n}_{s}∕{m}^{*}ns​∕m∗ increase with hole doping concentration xxx in the underdoped region, reach a saturation (maximum) at a hole doping above optimal doping, and decrease beyond the saturation point in the overdoped region, in agreement with $\ensuremath{\mu}\mathrm{SR}$ measurements. Based on our improved SU(2) slave-boson approach to the $t\ensuremath{-}J$ Hamiltonian, we further investigate the doping and temperature dependence of the spectral function and discuss our theoretical finding of a scaling behavior of the pseudogap. In addition, we discuss the cause of the hump and quasiparticle peak in the observed spectral functions of high Tc{T}_{c}Tc​ cuprates. It is demonstrated that the sharpening of the observed quasiparticle peak below Tc{T}_{c}Tc​ is attributed to the bose condensation of holon pair, in agreement with observations. From the predicted ratios of the pseudogap ${\ensuremath{\Delta}}_{0}$ to both the superconducting temperature Tc{T}_{c}Tc​ and the pseudogap temperature T∗{T}^{*}T∗, i.e., $2{\ensuremath{\Delta}}_{0}∕{k}_{B}{T}_{c}$ and $2{\ensuremath{\Delta}}_{0}∕{k}_{B}{T}^{*}$, respectively, as a function of hole doping concentration xxx, we find that there exists a universal scaling behavior (sample independence) of these ratios with doping, by showing a nonlinearly decreasing behavior of the former; that is, $2{\ensuremath{\Delta}}_{0}∕{k}_{B}{T}_{c}\ensuremath{\sim}{x}^{\ensuremath{-}\ensuremath{\alpha}}$ with $\ensuremath{\alpha}\ensuremath{\sim}2$ and a near doping independence of the latter; that is, $2{\ensuremath{\Delta}}_{0}∕{k}_{B}{T}^{*}\ensuremath{\approx}4--6$.
The finite-temperature phase diagram of the t-J model of electronic conduction is calculated in d dimensions, using the Migdal-Kadanoff renormalization-group procedure. No finite-temperature phase transition in d=1 and a finite-temperature first-order boundary ending at a critical point in d=2 are found. In d=3, a remarkably complex multicritical phase diagram is found, with a new phase, between hole dopings of 0.3 and 0.4 and temperatures 1/J below 0.4, in which the hopping strength t renormalizes to infinity under rescaling. Our results are confirmed by comparison of calculated electron densities, kinetic energies, and nearest-neighbor density-density and spin-spin correlation functions with exact finite-cluster results.
We report results of large-scale ground-state density matrix renormalization group (DMRG) calculations on t-[Formula: see text]-J cylinders with circumferences 6 and 8. We determine a rough phase diagram that appears to approximate the two-dimensional (2D) system. While for many properties, positive and negative [Formula: see text] values ([Formula: see text]) appear to correspond to electron- and hole-doped cuprate systems, respectively, the behavior of superconductivity itself shows an inconsistency between the model and the materials. The [Formula: see text] (hole-doped) region shows antiferromagnetism limited to very low doping, stripes more generally, and the familiar Fermi surface of the hole-doped cuprates. However, we find [Formula: see text] strongly suppresses superconductivity. The [Formula: see text] (electron-doped) region shows the expected circular Fermi pocket of holes around the [Formula: see text] point and a broad low-doped region of coexisting antiferromagnetism and d-wave pairing with a triplet p component at wavevector [Formula: see text] induced by the antiferromagnetism and d-wave pairing. The pairing for the electron low-doped system with [Formula: see text] is strong and unambiguous in the DMRG simulations. At larger doping another broad region with stripes in addition to weaker d-wave pairing and striped p-wave pairing appears. In a small doping region near [Formula: see text] for [Formula: see text], we find an unconventional type of stripe involving unpaired holes located predominantly on chains spaced three lattice spacings apart. The undoped two-leg ladder regions in between mimic the short-ranged spin correlations seen in two-leg Heisenberg ladders.
The role of next nearest neighbor (NNN) hopping (t') and next to NNN hopping (t'') on hole pairing and thermodynamic properties such as specific heat, entropy have been investigated using two dimensional (2D) hole-doped t-t'-t''-J model based on exact diagonalization (ED) method. Standard Periodic boundary conditions are applied to minimize error due to finite size effect as the calculations are made using small sized cluster geometry. The attraction between holes increases with the inclusion of third neighbor hopping term. The maximum probability of hole pairing is at NNN site. The system goes to more disordered and ordered state with the increase of long range hopping terms at temperature T≤0.35t and T>0.35t, respectively. A single peak nature is observed in specific heat graph.
Recent experiments on cuprates show that as a function of doping, the normal-state specific heat sharply peaks at the doping ${\ensuremath{\delta}}^{*}$, where the pseudogap ends at low temperature. This finding is taken as the thermodynamic signature of a quantum critical point, whose nature has not yet been identified. Here we present calculations for the two-dimensional Hubbard model in the doped Mott insulator regime, which indicate that the specific heat anomaly can arise from the finite-temperature critical end point of a first-order transition between a pseudogap phase with dominant singlet correlations and a metal. As a function of doping at the temperature of the end point, the specific heat diverges. Upon increasing temperature, the peak becomes broader. The diverging correlation length is associated with uniform density fluctuations. No broken symmetries are needed. These anomalies also occur at half-filling as a function of interaction strength, and are relevant for organic superconductors and ultracold atoms.