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arXiv:cond-mat/0412576 · Physical Review E

Exact dynamics of a reaction-diffusion model with spatially alternating rates

Mauro Mobilia, B. Schmittmann, Royce K. P. Zia

Published May 31, 2005• 10 citations
arXivHTMLPDF

Abstract

We present the exact solution for the full dynamics of a nonequilibrium spin chain and its dual reaction-diffusion model, for arbitrary initial conditions. The spin chain is driven out of equilibrium by coupling alternating spins to two thermal baths at different temperatures. In the reaction-diffusion model, this translates into spatially alternating rates for particle creation and annihilation, and even negative "temperatures" have a perfectly natural interpretation. Observables of interest include the magnetization, the particle density, and all correlation functions for both models. Two generic types of time dependence are found: if both temperatures are positive, the magnetization, density, and correlation functions decay exponentially to their steady-state values. In contrast, if one of the temperatures is negative, damped oscillations are observed in all quantities. They can be traced to a subtle competition of pair creation and annihilation on the two sublattices. We comment on the limitations of mean-field theory and propose an experimental realization of our model in certain conjugated polymers and linear chain compounds.

DOI
10.1103/physreve.71.056129

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We present the exact solution for the full dynamics of a nonequilibrium spin chain and its dual reaction-diffusion model, for arbitrary initial conditions. The spin chain is driven out of equilibrium by coupling alternating spins to two thermal baths at different temperatures. In the reaction-diffusion model, this translates into spatially alternating rates for particle creation and annihilation, and even negative "temperatures" have a perfectly natural interpretation. Observables of interest include the magnetization, the particle density, and all correlation functions for both models. Two generic types of time dependence are found: if both temperatures are positive, the magnetization, density, and correlation functions decay exponentially to their steady-state values. In contrast, if one of the temperatures is negative, damped oscillations are observed in all quantities. They can be traced to a subtle competition of pair creation and annihilation on the two sublattices. We comment on the limitations of mean-field theory and propose an experimental realization of our model in certain conjugated polymers and linear chain compounds.
Non-universal dynamics is shown to occur in a one-dimensional non-equilibrium system of hard-core particles. The stochastic processes included are pair creation and annihilation (with rates and ) and symmetric hopping rates which alternate from one bond to the next ( , ). A dynamical scaling relation between the relaxation time and the correlation length in the steady state is derived in a simple way for the case . We find that the dynamical exponent takes the non-universal value . For the special condition , where the stochastic system is in principle soluble by reduction to a free fermion system, the model is mapped to the Glauber dynamics of an Ising chain with alternating ferromagnetic bonds of values and , in contact with a quantum thermal bath. The full time dependence of the space-dependent magnetization and of the equal time spin-spin correlation function are studied by writing the master equation for this system in the quantum Hamiltonian formalism. In particular, we obtain the dispersion relations and rigorously confirm the results obtained for the correlation length and for the dynamical exponent.
Non-universal dynamics is shown to occur in a one-dimensional non-equilibrium system of hard-core particles. The stochastic processes included are pair creation and annihilation (with rates e and e') and symmetric hopping rates which alternate from one bond to the next (Pa, Pb). A dynamical scaling relation between the relaxation time and the correlation length in the steady state is derived in a simple way for the case e' > Pa >> Pb >> e. We find that the dynamical exponent takes the non-universal value z = 2 ln(e'/e) / ln[(Pb e')/(Pa e)]. For the special condition e + e'= Pa + Pb, where the stochastic system is in principle soluble by reduction to a free fermion system, the model is mapped to the Glauber dynamics of an Ising chain with alternating ferromagnetic bonds of values J1 and J2, in contact with a quantum thermal bath. The full time dependence of the space-dependent magnetization and of the equal time spin-spin correlation function are studied by writing the master equation for this system in the quantum Hamiltonian formalism. In particular we obtain the dispersion relations and rigorously confirm the results obtained for the correlation length and for the dynamical exponent.
A kinetic one-dimensional Ising model on a ring evolves according to a generalization of Glauber rates, such that spins at even (odd) lattice sites experience a temperature T(e) (T(o)). Detailed balance is violated so that the spin chain settles into a nonequilibrium stationary state, characterized by multiple interactions of increasing range and spin order. We derive the equations of motion for arbitrary correlation functions and solve them to obtain an exact representation of the steady state. Two nontrivial amplitudes reflect the sublattice symmetries; otherwise, correlations decay exponentially, modulo the periodicity of the ring. In the long-chain limit, they factorize into products of two-point functions, in precise analogy to the equilibrium Ising chain. The exact solution confirms the expectation, based on simulations and renormalization group arguments, that the long-time, long-distance behavior of this two-temperature model is Ising-like, in spite of the apparent complexity of the stationary distribution.
The nonequilibrium dynamics of classical random Ising spin chains with nonconserved magnetization are studied using an asymptotically exact real space renormalization group (RSRG). We focus on random field Ising model (RFIM) spin chains with and without a uniform applied field, as well as on Ising spin glass chains in an applied field. For the RFIM we consider a universal regime where the random field and the temperature are both much smaller than the exchange coupling. In this regime, the Imry-Ma length that sets the scale of the equilibrium correlations is large and the coarsening of domains from random initial conditions (e.g., a quench from high temperature) occurs over a wide range of length scales. The two types of domain walls that occur diffuse in opposite random potentials, of the form studied by Sinai, and domain walls annihilate when they meet. Using the RSRG we compute many universal asymptotic properties of both the nonequilibrium dynamics and the equilibrium limit. We find that the configurations of the domain walls converge rapidly toward a set of system-specific time-dependent positions that are independent of the initial conditions. Thus the behavior of this nonequilibrium system is pseudodeterministic at long times because of the broad distributions of barriers that occur on the long length scales involved. Specifically, we obtain the time dependence of the energy, the magnetization, and the distribution of domain sizes (found to be statistically independent). The equilibrium limits agree with known exact results. We obtain the exact scaling form of the two-point equal time correlation function <S0(t)Sx(t)> and the two-time autocorrelations <S0(t('))S0(t)>. We also compute the persistence properties of a single spin, of local magnetization, and of domains. The analogous quantities for the +/-J Ising spin glass in an applied field are obtained from the RFIM via a gauge transformation. In addition to these we compute the two-point two-time correlation function <S0(t)Sx(t)><S0(t('))Sx(t('))> which can in principle be measured by experiments on spin-glass-like systems. The thermal fluctuations are studied and found to be dominated by rare events; in particular all moments of truncated equal time correlations are computed. Physical properties which are typically measured in aging experiments are also studied, focusing on the response to a small magnetic field which is applied after waiting for the system to equilibrate for a time t(w). The nonequilibrium fluctuation-dissipation ratio X(t,t(w)) is computed. We find that for (t-t(w)) approximately t(alpha)(w) with alpha;<1, the ratio equal to its equilibrium value X=1, although time translational invariance does not hold in this regime. For t-t(w) approximately t(w) the ratio exhibits an aging regime with a nontrivial X=X(t/t(w)) not equal to 1, but the behavior is markedly different from mean field theory. Finally the distribution of the total magnetization and of the number of domains is computed for large finite size systems. General issues about convergence toward equilibrium and the possibilities of weakly history-dependent evolution in other random systems are discussed.
A kinetic one-dimensional Ising model is coupled to two heat baths, such that spins at even (odd) lattice sites experience a temperature T-e (T-o). Spin-flips occur with Glauber-type rates generalized to the case of two temperatures. Driven by the temperature differential, the spin chain settles into a nonequilibrium steady state which corresponds to the stationary solution of a master equation. We construct a perturbation expansion of this master equation in terms of the temperature difference and compute explicitly the first two corrections to the equilibrium Boltzmann distribution. The key result is the emergence of additional spin operators in the steady state, increasing in spatial range and order of spin products. We comment on the violation of detailed balance and entropy production in the steady state.