The S=1/2 ferromagnetic (F) - antiferromagnetic (AF) random alternating Heisenberg quantum spin chain is investigated by the quantum Monte Carlo method. The randomness is only present on the strong bonds taking values of ±2J randomly, and the weak bonds are uniformly antiferromagnetic with J. The model corresponds to the quasi one-dimensional compound, (CH3)2CHNH3Cu(Clx, Br1-x)3, whose ground state interpolates the Haldane state of the F-AF alternating spin chain at x=1 and the singlet-dimer state of the AF-AF alternating spin chain at x=0. The nonequilibrium relaxation function of the staggered magnetic susceptibility exhibits algebraic divergence in the intermediate region of 0.44 ≪ x ≪ 0.87, which explains the experimental observation of the magnetic phase transition. The results suggest that the antiferromagnetic order becomes critical by the randomness of the bond distributions even in the presence of the rich ferromagnetic bonds.
We use a tensor network renormalization group method to study random
S=2 antiferromagnetic Heisenberg chains with alternating bond strength distributions. In the absence of randomness, an imposed dimerization with bond alternation induces two quantum critical points between the
S=2 Haldane phase, a partially dimerized phase, and a fully dimerized phase, depending on the strength of dimerization. These three phases, called ($\ensuremath{\sigma},4\ensuremath{-}\ensuremath{\sigma}$) = (2,2), (3,1), and (4,0) phases, are valence-bond solid (VBS) states characterized by $\ensuremath{\sigma}$ valence bonds (effective spin-1/2 singlet pairs) forming across even links and $4\ensuremath{-}\ensuremath{\sigma}$ valence bonds on odd links. Here we study the effects of bond randomness on the ground states of the dimerized spin chain, calculating disorder-averaged twist order parameters and spin correlations. We classify the types of random VBS phases depending on the strength of bond randomness
R and dimerization
D using the twist order parameter, which has a negative/positive sign for a VBS phase with odd/even $\ensuremath{\sigma}$. Our results demonstrate the existence of a multicritical point in the intermediate disorder regime with finite dimerization, where (2,2), (3,1), and (4,0) phases meet. This multicritical point is at the junction of three phase boundaries in the $R\text{\ensuremath{-}}D$ plane: the (2,2)-(3,1) and (3,1)-(4,0) boundaries that extend to zero randomness, and the (2,2)-(4,0) phase boundary that connects another multicritical point in the undimerized limit. The undimerized multicritical point separates a gapless Haldane phase and an infinite-randomness critical line with the diverging dynamic critical exponent in the large-
R limit at
D=0. Furthermore, we identify the (3,1)-(4,0) phase boundary as an infinite-randomness critical line even at small
R and find the signature of infinite randomness at the (2,2)-(3,1) phase boundary only in the vicinity of the multicritical point.
The S = 1/2 Heisenberg chains with bond alternation and randomness on the strong bonds are studied by the density matrix renormalization group method. It is assumed that the oddth bond is antiferromagnetic with strength J and even-th bond can take the values JA and JF (JA > J > 0 > JF) randomly. The ground state of this model interpolates between the Haldane and dimer phases via a randomness dominated intermediate phase. Based on the scaling of the low energy spectrum and mean field treatment of the interchain coupling, it is found that the magnetic long range order is induced by randomness in the intermediate regime. In the magnetization curves, there appears a plateau at the fractional value of thesaturated magnetization. The fine structures of the magnetization curves and low energy spectrum are understood based on the cluster picture. The relation with the recent experiment for (CH3)2CHNH3Cu(ClxBr1−x)3 is discussed.
Bond-dilution effects on the ground state of the square-lattice antiferromagnetic Heisenberg model, consisting of coupled bond-alternating chains, are investigated by means of the quantum Monte Carlo simulation. It is found that, when the ground state of the non-diluted system is a non-magnetic state with a finite spin gap, a sufficiently weak bond dilution induces a disordered state with a mid gap in the original spin gap, and under a further stronger bond dilution an antiferromagnetic long-range order emerges. While the site-dilution-induced long-range order is induced by an infinitesimal concentration of dilution, there exists a finite critical concentration in the case of bond dilution. We argue that this essential difference is due to the occurrence of two types of effective interactions between induced magnetic moments in the case of bond dilution, and that the antiferromagnetic long-range-ordered phase does not appear until the magnitudes of the two interactions become comparable.
The S = 1/2 Heisenberg chains with bond alternation and randomness on the strong bonds are studied by the density matrix renormalization group method. It is assumed that the odd-th bond is antiferromagnetic with strength J and the even-th bond can take the values JA and JF (JA > J > 0 > JF) randomly. The ground state of this model interpolates between the Haldane and dimer phases via a randomness dominated intermediate phase. On the basis of the scaling of the low energy spectrum and mean field treatment of the interchain coupling, we find that the magnetic long range order is induced by randomness in the intermediate regime. In the magnetization curves, there appears a plateau at the fractional value of the saturated magnetization. The fine structures of the magnetization curves and low energy spectrum are understood using the cluster picture. The relation to the recent experiment for (CH3)2CHNH3Cu(ClxBr1-x)3 is discussed.