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arXiv:cond-mat/0410559 · Physical Review B

Subgap states in dirty superconductors and their effect on dephasing in Josephson qubits

Alessandro Silva, L. B. Ioffe

Published Mar 7, 2005• 33 citations
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Abstract

We present a theory of the subgap tails of the density of states in a diffusive superconductor containing magnetic impurities. We show that the subgap tails have two contributions: one arising from mesoscopic gap fluctuations, previously discussed by Lamacraft and Simons, and the other associated to the long-wave fluctuations of the concentration of magnetic impurities. We study the latter both in small superconducting grains and in bulk systems $[d=1,2,3]$, and establish the dimensionless parameter that controls which of the two contributions dominates the subgap tails. We observe that these contributions are related to each other by dimensional reduction. We apply the theory to estimate the effects of a weak concentration of magnetic impurities $[\ensuremath{\approx}1\phantom{\rule{0.3em}{0ex}}\mathrm{ppm}]$ on the phase coherence of Josephson qubits. We find that at these typical concentrations, magnetic impurities are relevant for the dephasing in large qubits, designed around a $10\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{m}$ scale, where they limit the quality factor to be $Q<{10}^{4}\ensuremath{-}{10}^{5}$.

DOI
10.1103/physrevb.71.104502

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We present a theory of the subgap tails of the density of states in a diffusive superconductor containing magnetic impurities. We show that the subgap tails have two contributions: one arising from mesoscopic gap fluctuations, previously discussed by Lamacraft and Simons, and the other associated to the long-wave fluctuations of the concentration of magnetic impurities. We study the latter both in small superconducting grains and in bulk systems [d=1,2,3][d=1,2,3][d=1,2,3], and establish the dimensionless parameter that controls which of the two contributions dominates the subgap tails. We observe that these contributions are related to each other by dimensional reduction. We apply the theory to estimate the effects of a weak concentration of magnetic impurities [\ensuremath≈1ppm][\ensuremath{\approx}1\phantom{\rule{0.3em}{0ex}}\mathrm{ppm}][\ensuremath≈1ppm] on the phase coherence of Josephson qubits. We find that at these typical concentrations, magnetic impurities are relevant for the dephasing in large qubits, designed around a 10\ensuremathμm10\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{m}10\ensuremathμm scale, where they limit the quality factor to be Q<104\ensuremath−105Q<{10}^{4}\ensuremath{-}{10}^{5}Q<104\ensuremath−105.
We investigated decoherence of a Josephson vortex quantum bit (qubit) in dissipative and noisy environment. As the Josephson vortex qubit (JVQ) is fabricated by using a long Josephson junction (LJJ), we use the perturbed sine-Gordon equation to describe the phase dynamics representing a two-state system and estimate the effects of quasiparticle dissipation and weakly fluctuating critical and bias currents on the relaxation time T1{T}_{1}T1​ and on the dephasing time ${T}_{\ensuremath{\phi}}$. We show that the critical current fluctuation does not contribute to dephasing of the qubit in the lowest order approximation. Modeling the weak current variation from magnetic field fluctuations in the LJJ by using the Gaussian colored noise with long correlation time, we show that the coherence time T2{T}_{2}T2​ is limited by the low frequency current noise at very low temperatures. Also, we show that a ultra-long coherence time may be obtained from the JVQ by using experimentally accessible value of physical parameters.
Material inhomogeneities in a superconductor generically lead to broadening of the density of states and to subgap states. The latter are associated with spatial fluctuations of the gap in which quasiparticles can be trapped. Recombination between such localized quasiparticles is hindered by their spatial separation and hence their density could be higher than expectations based on the recombination between mobile quasiparticles. We show here that the recombination between localized and mobile excitations can be efficient at limiting the quasiparticle density. We comment on the significance of our findings for devices such as superconducting resonators and qubits. We find that for typical aluminum devices, the subgap states do not significantly influence the quasiparticle density.
In superconducting qubits, the interaction of the qubit degree of freedom with quasiparticles defines a fundamental limitation for the qubit coherence. We develop a theory of the pure dephasing rate ${\ensuremath{\Gamma}}_{\ensuremath{\phi}}$ caused by quasiparticles tunneling through a Josephson junction and of the inhomogeneous broadening due to changes in the occupations of Andreev states in the junction. To estimate ${\ensuremath{\Gamma}}_{\ensuremath{\phi}}$, we derive a master equation for the qubit dynamics. The tunneling rate of free quasiparticles is enhanced by their large density of states at energies close to the superconducting gap. Nevertheless, we find that ${\ensuremath{\Gamma}}_{\ensuremath{\phi}}$ is small compared to the rates determined by extrinsic factors in most of the current qubit designs (phase and flux qubits, transmon, fluxonium). The split transmon, in which a single junction is replaced by a SQUID loop, represents an exception that could make possible the measurement of ${\ensuremath{\Gamma}}_{\ensuremath{\phi}}$. Fluctuations of the qubit frequency leading to inhomogeneous broadening may be caused by the fluctuations in the occupation numbers of the Andreev states associated with a phase-biased Josephson junction. This mechanism may be revealed in qubits with small-area junctions, since the smallest relative change in frequency it causes is of the order of the inverse number of transmission channels in the junction.
We propose a microscopic model of critical current noise in Josephson junctions based on individual trapping centers in the tunnel-barrier hybridized with electrons in the superconducting leads. We calculate the noise exactly in the limit of no on-site Coulomb repulsion. Our result reveals a noise spectrum that is dramatically different from the usual Lorentzian assumed in simple models. We show that the noise is dominated by sharp subgap resonances associated to the formation of pairs of Andreev bound states, thus providing a possible explanation for the spurious two-level systems (microresonators) observed in Josephson-junction qubits [R. W. Simmonds et al., Phys. Rev. Lett. 93, 077003 (2004).]. Another implication of our model is that each trapping center will contribute a sharp dielectric resonance only in the superconducting phase, providing an effective way to validate our results experimentally. We derive an effective Hamiltonian for a qubit interacting with Andreev bound states, establishing a direct connection between phenomenological models and the microscopic parameters of a Fermionic bath.
We consider a superconducting phase qubit consisting of a monocrystalline sapphire Josephson junction with its symmetry axis perpendicular to the junction interfaces. Via the London gauge, we present a theoretical model of Fe3+ magnetic impurities within the junction that describes the effect of a low concentration of such impurities on the operation of the qubit. Specifically, we derive an interaction Hamiltonian expressed in terms of angular momentum states of magnetic impurities and low-lying oscillator states of a current-biased phase qubit. We discuss the coupling between the qubit and impurities within the model near resonance. When the junction is biased at an optimal point for acting as a phase qubit, with a phase difference of π/2 and impurity concentration no greater than 0.05%, we find only a slight decrease in the Q factor of less than 0.01%.
The boson lattice Hubbard model is used to study the role of quantum fluctuations of the phase and local density of the superfluid component in establishing a global superconducting state for a system of mesoscopic Josephson junctions or grains. The quantum Monte Carlo method is used to calculate the density of the superfluid component and fluctuations in the number of particles at sites of the two-dimensional lattice for various average site occupation numbers n 0 (i.e., number of Cooper pairs per grain). For a system of strongly interacting bosons, the phase boundary of the ordered superconducting state lies above the corresponding boundary for its quasiclassical limit—the quantum XY -model—and approaches the latter as n 0 increases. When the boson interaction is weak in the boson Hubbard model (i.e., the quantum fluctuations of the phase are small), the relative fluctuations of the order parameter modulus are significant when n 0 <10, while quantum fluctuations in the phase are significant when n 0 <8; this determines the region of mesoscopic behavior of the system. Comparison of the results of numerical modeling with theoretical calculations show that mean-field theory yields a qualitatively correct estimate of the difference between the phase diagrams of the quantum XY -model and the Hubbard model. For a quantitative estimate of this difference the free energy and thermodynamic averages of the Hubbard model are expanded in powers of 1/ n 0 using the method of functional integration.