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arXiv:cond-mat/0410501 · Physical Review A

Static properties and spin dynamics of the ferromagnetic spin-1 Bose gas in a magnetic field

Krisztián Kis-Szabó, P. Szépfalusy, Gergely Szirmai

Published Aug 26, 2005• 13 citations
arXivHTMLPDF

Abstract

The properties of spin-1 Bose gases with ferromagnetic interactions in the presence of a nonzero magnetic field are studied. The equation of state and thermodynamic quantities are worked out with the help of a mean-field approximation. The phase diagram besides Bose-Einstein condensation contains a first-order transition where two values of the magnetization coexist. The dynamics is investigated with the help of the random phase approximation. The soft mode corresponding to the critical point of the magnetic phase transition is found to behave like in conventional theory.

DOI
10.1103/physreva.72.023617

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The properties of spin-1 Bose gases with ferromagnetic interactions in the presence of a nonzero magnetic field are studied. The equation of state and thermodynamic quantities are worked out with the help of a mean-field approximation. The phase diagram besides Bose-Einstein condensation contains a first-order transition where two values of the magnetization coexist. The dynamics is investigated with the help of the random phase approximation. The soft mode corresponding to the critical point of the magnetic phase transition is found to behave like in conventional theory.
We investigate the thermodynamics of a spin-1 Bose gas with fixed magnetization including the quadratic Zeeman energy shift. Our calculations are based on the grand canonical description for the ideal gas and the classical field approximation for atoms with ferromagnetic and antiferromagnetic interactions. We confirm the occurrence of a double phase transition in the system that takes place due to two global constraints. We show analytically for the ideal gas how critical temperatures and condensed fractions are changed by a nonzero magnetic field. The interaction strongly affects the condensate scenario below the second critical temperature. The effect imposed by interaction energies becomes diminished in high magnetic fields where condensation of both ferromagnetic and antiferromagnetic atoms agrees with the ideal gas results.
Thermodynamics of a spin-1 Bose gas with ferromagnetic interactions is investigated via the mean-field theory. It is apparently shown in the specific-heat curve that the system undergoes two phase transitions, the ferromagnetic transition and Bose-Einstein condensation, with the Curie point above the condensation temperature. Above the Curie point, the susceptibility fits the Curie-Weiss law perfectly. At a fixed temperature, the reciprocal susceptibility is also in a good linear relationship with the ferromagnetic interaction.
The magnetic properties of a charged spin-1 Bose gas with ferromagnetic interactions are investigated within mean-field theory. It is shown that a competition between paramagnetism, diamagnetism and ferromagnetism exists in this system. It is shown that diamagnetism, being concerned with spontaneous magnetization, cannot exceed ferromagnetism in a very weak magnetic field. The critical value of reduced ferromagnetic coupling of the paramagnetic phase to ferromagnetic phase transition I[combining overline](c) increases with increasing temperature. The Landé-factor g is introduced to describe the strength of the paramagnetic effect which comes from the spin degree of freedom. The magnetization density M[combining overline] increases monotonically with g for fixed reduced ferromagnetic coupling I[combining overline] as I[combining overline] > I[combining overline](c). In a weak magnetic field, ferromagnetism makes an immense contribution to the magnetization density. On the other hand, at a high magnetic field, the diamagnetism tends to saturate. Evidence for condensation can be seen in the magnetization density at a weak magnetic field.
The thermodynamic properties of a Bose gas of particles with nonzero spin and magnetic moment in states with and without a Bose-Einstein condensate are studied as a function of the external magnetic field. It is shown that there exists a temperature interval where a transition into a state with a Bose-Einstein condensate occurs in a Bose gas with constant temperature and particle number density when the magnetic field is increasing and reaches a critical magnitude. The temperature and magnetic field derivatives of the specific heat at constant volume and the magnetic susceptibility undergo a jump at such a transition.
Since the experimental realization of Bose-Einstein condensation in 1995, the field of ultracold atoms has expanded rapidly, and has become an important arena for exploring diverse quantum many-body physics, as highlighted by the experimental observation of quantum phase transitions in the system of bosons in a periodic potential, which is described by the Bose-Hubbard model.Recently, ultracold atoms with spin degrees of freedom are actively studied because the coupling between the internal spin degrees of freedom and the spatial degrees of freedom can give rise to novel and interesting physics.A minimal model for studying such physics is the spin-1 Bose-Hubbard model, which describes spin-1 bosons in a periodic potential.The model has a spin-dependent interaction, which can be ferromagnetic or antiferromagnetic, and it is known that although the ferromagnetic model resembles the spinless counterpart, the antiferromagnetic model exhibits totally different features, which make the model much more intensively studied compared with the ferromagnetic one.However, the presence of an external magnetic field can change the situation, because the positive quadratic Zeeman energy competes with the ferromagnetic interaction, which can give rise to rich phases.In this thesis, we explore the ground-state and nonzero-temperature phase diagrams of the spin-1 Bose-Hubbard model under an external magnetic field.To analyze the model, we use an approximation method called the decoupling approximation, or equivalently, the Gutzwiller variational ansatz.It is shown that, in addition to the Mott insulator phase, the model possesses two superfluid phases.Moreover, for large values of a spin-dependent interaction, the phase transitions between the two superfluid phases can be discontinuous.Such discontinuous phase transitions are shown to survive at nonzero but sufficiently low temperature.The discontinuous phase transitions are in clear contrast to the mean-field theory of weakly interacting spin-1 bosons without a lattice, which predicts that the corresponding phase transition is continuous, signifying the importance of the effect of strong interactions on the interplay between the spatial and spinor degrees of freedom. 4.1.2The grand Hamiltonian . . . . . . . . .
The strongly ferromagnetic spin-1 Bose-Einstein condensate has recently been realized with atomic Li7 . It was predicted that a strong ferromagnetic interaction can drive the normal gas into a magnetized phase at a temperature above the superfluid transition, and Li7 likely satisfies the criterion. We reexamine this theoretical proposal employing the two-particle-irreducible effective potential, and conclude that there exists no stable normal magnetized phase for a dilute ferromagnetic Bose gas. For Li7 , we predict that the normal gas undergoes a joint first-order transition and jumps directly into a state with finite condensate density and magnetization. We estimate the size of the first-order jump and examine how a partial spin polarization in the initial sample affects the first-order transition. We propose a qualitative phase diagram at fixed temperature for the trapped gas. Published by the American Physical Society 2024