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arXiv:cond-mat/0408322 · Physical Review B

Reducing decoherence of the confined exciton state in a quantum dot by pulse-sequence control

V. M. Axt, Paweł Machnikowski, T. Kühn

Published Apr 6, 2005• 55 citations
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Abstract

We study the phonon-induced dephasing of the exciton state in a quantum dot excited by a sequence of ultrashort pulses. We show that the multiple-pulse control leads to a considerable improvement of the coherence of the optically excited state. For a fixed control time window, the optimized pulsed control often leads to a higher degree of coherence than the control by a smooth, single Gaussian pulse. The reduction of dephasing is considerable already for 2--3 pulses.

DOI
10.1103/physrevb.71.155305

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We quantitatively investigate the usefulness and viability of the scheme developed by Viola and Lloyd [Phys. Rev. A 58, 2733 (1998)] to control dephasing in the context of exciton-based quantum computation with self-assembled quantum dots. We demonstrate that optical coherence of a confined exciton qubit exposed to phonon-induced dephasing can be substantially enhanced through the application of a simple periodic sequence of control pulses. The shape of the quantum dot has a significant effect on the dephasing properties. Remarkably, we find that quantum dots with parameters optimized for implementing quantum computation are among the most susceptible to dephasing, yet periodic decoupling is most efficient for exactly that type of dot. We also show that the presence of an electric field, which is a necessary ingredient for many exciton-based quantum computing schemes, may further increase the control efficiency. Our results suggest that dynamical decoupling may be a method of choice for robust storage of exciton qubits during idle stages of quantum algorithms.
We study phonon-assisted dephasing in optically excited semiconductor quantum dots within the frameworks of the independent Boson model and optimal control. Using a realistic description for the quantum dot states and the phonon coupling, we demonstrate that such dephasing has a drastic impact on the coherent optical response. We employ optimal control theory to search for control strategies that allow to fight decoherence, and show that appropriate tailoring of laser pulses allows a complete control of the optical excitation despite the phonon dephasing.
We report on coherent control of the resonantly driven exciton state in a single quantum dot in the strong coupling regime. With picosecond laser pulses, the two-level system undergoes Rabi oscillations and a given coherent superposition of states can be addressed. Using a pair of phase-locked pulses, optical manipulation is achieved during the coherence time of the qu-bit. The dephasing processes are also studied and we show that in typical quantum dots, the coherence time T 2 can be of the same order of magnitude as the effective lifetime of the exciton T 1 (a few hundreds of ps) although not reaching the upper theoretical limit of 2T 1 . We conclude that energy relaxation and pure dephasing processes due to virtual scattering with phonons contribute on an equal footing to the loss of coherence.
The paper discusses coherent control of charge and spin states of a biexciton system in a quantum dot via coherent two-photon transitions. Rabi oscillations between the ground state of a quantum dot and the biexciton state, as well as oscillations between the two single-exciton states induced by laser pulses with different circular or linear polarizations are studied. The effect of phonon-induced decoherence on these processes is described. System properties and driving conditions that lead to optimal coherent control are identified. It is shown that proper optimization allows one to control the two-qubit biexciton system via two-photon transitions with a high fidelity.