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arXiv:cond-mat/0406312 · Physical Review Letters

Frequency-Dependent Transport through a Quantum Dot in the Kondo Regime

Michael Sindel, Walter Hofstetter, Jan von Delft, M. Kindermann

Published May 19, 2005• 30 citations
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Abstract

We study the ac conductance and equilibrium current fluctuations of a Coulomb-blockaded quantum dot in the Kondo regime. To this end we have developed an extension of the numerical renormalization group suitable for the nonperturbative calculation of finite-frequency transport properties. We demonstrate that ac transport gives access to the many-body resonance in the equilibrium spectral density. It provides a new route for measuring this key signature of Kondo physics, which so far has defied direct experimental observation.

DOI
10.1103/physrevlett.94.196602

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We study the ac conductance and equilibrium current fluctuations of a Coulomb-blockaded quantum dot in the Kondo regime. To this end we have developed an extension of the numerical renormalization group suitable for the nonperturbative calculation of finite-frequency transport properties. We demonstrate that ac transport gives access to the many-body resonance in the equilibrium spectral density. It provides a new route for measuring this key signature of Kondo physics, which so far has defied direct experimental observation.
We study the ac conductance and equilibrium current fluctuations of a Coulomb blockaded quantum dot in the Kondo regime. To this end we have developed an extension of the numerical renormalization group suitable for the nonperturbative calculation of finite‐frequency transport properties. We demonstrate that ac transport gives access to the many‐body resonance in the equilibrium spectral density. It provides a new route to measuring this key signature of Kondo physics, which so far has defied direct experimental observation.
We construct a real time current-conserving functional renormalization group (RG) scheme on the Keldysh contour to study frequency-dependent transport and noise through a quantum dot in the local moment regime. We find that the current vertex develops a nontrivial nonlocal structure in time that is governed by a new set of RG equations. Solving these RG equations, we compute the complete frequency and temperature dependence of the noise spectrum. For voltages that are large compared to the Kondo temperature (i.e., $\mathit{eV}\ensuremath{\gg}{k}_{B}{T}_{K}$), two sharp antiresonances are found in the noise spectrum at frequencies $\ensuremath{\hbar}\ensuremath{\omega}=\ifmmode\pm\else\textpm\fi{}eV$ and, correspondingly, two Kondo-assisted peaks appear in the ac conductance through the dot.
We study finite-frequency transport properties of the double dot system recently constructed to observe the two-channel Kondo effect [R. M. Potok et al., Nature 446, 167 (2007)]. We derive an analytical expression for the frequency-dependent linear conductance of this device in the Kondo regime. We show how the features characteristic of the two-channel Kondo quantum critical point emerge in this quantity, which we compute using the results of conformal field theory as well as numerical renormalization group methods. We determine the universal crossover functions describing non-Fermi-liquid vs Fermi-liquid crossovers and also investigate the effects of a finite magnetic field.
Correlations are a central ingredient of modern condensed matter physics. With the advent of mesoscopic physics, it became possible to study correlated systems in non-equilibrium situations, which can be reached by e.g. driving a constant current through a quantum dot. A basic question is how correlations on the one hand and a non-equilibrium current on the other hand influence each other. Here this interplay is studied for the model system of a quantum dot in the Kondo regime using the real time renormalization group (RTRG) method. This method is a functional renormalization group (RG) method allowing a non-perturbative description of correlated systems in non-equilibrium. For the Kondo quantum dot the method is generalized to the case of double vertices. The RTRG method not only provides equations for the calculation of the renormalized coupling between the quantum dot spin and the reservoir electrons, but also equations for the calculation of the non-equilibrium decoherence rate and the non-equilibrium current.The RG equations are derived to second order. This approximation is expected to be valid as long as the quantum dot does not enter the strong coupling regime, i.e. the effective coupling strength between the quantum dot spin and the electrons does not become too large. It is found that this is the case if the bias voltage applied to the dot or the temperature is much larger than the Kondo temperature.It is shown that the RG equations lead to coupling functions depending on the energy of the incident and the scattered electron. This dependence is simplified to the dependence on the average energy of the incident and the scattered electron in the weak coupling regime.A closer inspection of the RG equations for the couplings shows that they not only contain terms leading to a logarithmic increase of the coupling strength but also subleading terms which are unimportant in the weak coupling regime. The RG equations are solved analytically for the case where the subleading terms are neglected. It is found that the coupling functions develop resonances at energies associated with the chemical potentials of the reservoirs. The height of these resonances is determined by the decoherence rate. However, for bias voltages much larger than the Kondo temperature these resonances do not affect the conductance for a two terminal setup, so the conductance does not provide a measure for the decoherence rate in this case. It is found that the conductance for the two terminal setup is a universal function of voltage/Kondo temperature and temperature/Kondo temperature in the weak coupling regime. This function is calculated analytically in the limits of vanishing voltage or temperature. Furthermore, it is found that for zero temperature the decoherence rate is proportional to the non-equilibrium current flowing through the system. This supports the physical picture that a non-equilibrium current is associated with a decoherence rate, which cuts the logarithmic scaling of the coupling strength.Finally, the RG equations are solved numerically for zero temperature including the subleading corrections found before. As expected, the subleading corrections have no impact on the decoherence rate and the conductance in the weak coupling regime. On the other hand, it is found that they lead to strong deviations from the results of the analytic leading logarithmic approximation if the bias voltage approaches the Kondo temperature. Generally, it is found that the subleading corrections lead to a saturation of the decoherence rate and the conductance to some finite value. However, for the numerical solution a numerical regularization parameter has to be introduced. It turns out that the saturation value found depends on its value, so no statements on the precise value of the decoherence rate and the current can be made in this regime.
The resonant-level model represents a paradigmatic quantum system which serves as a basis for many other quantum impurity models. We provide a comprehensive analysis of the nonequilibrium transport near a quantum phase transition in a spinless dissipative resonant-level model, extending earlier work [Phys. Rev. Lett 102, 216803 (2009)]. A detailed derivation of a rigorous mapping of our system onto an effective Kondo model is presented. A controlled energy-dependent renormalization-group approach is applied to compute the nonequilibrium current in the presence of a finite bias voltage VVV. In the linear-response regime $V\ensuremath{\rightarrow}0$, the system exhibits as a function of the dissipative strength a localized-delocalized quantum transition of the Kosterlitz-Thouless (KT) type. We address fundamental issues of the nonequilibrium transport near the quantum phase transition: Does the bias voltage play the same role as temperature to smear out the transition? What is the scaling of the nonequilibrium conductance near the transition? At finite temperatures, we show that the conductance follows the equilibrium scaling for V<TV<TV<T, while it obeys a distinct nonequilibrium profile for V>TV>TV>T. We furthermore provide different signatures of the transition in the finite-frequency current noise and ac conductance via a recently developed functional renormalization group (FRG) approach. The generalization of our analysis to nonequilibrium transport through a resonant level coupled to two chiral Luttinger liquid leads, generated by fractional quantum Hall edge states, is discussed. Our work on the dissipative resonant level has direct relevance to experiments on a quantum dot coupled to a resistive environment, such as H. Mebrahtu et al., [Nature (London) 488, 61 (2012)].
We apply the real-time renormalization group (RG) in nonequilibrium to an arbitrary quantum dot in the Coulomb blockade regime. Within one-loop RG equations, we include self-consistently the kernel governing the dynamics of the reduced density matrix of the dot. As a result, we find that relaxation and dephasing rates generically cut off the RG flow. In addition, we include all other cutoff scales defined by temperature, energy excitations, frequency, and voltage. We apply the formalism to transport through single molecular magnets, realized by the fully anisotropic Kondo model (with three different exchange couplings Jx{J}_{x}Jx​, Jy{J}_{y}Jy​, and Jz{J}_{z}Jz​) in a magnetic field hz{h}_{z}hz​. We calculate the differential conductance as function of bias voltage VVV and discuss a quantum phase transition which can be tuned by changing the sign of JxJyJz{J}_{x}{J}_{y}{J}_{z}Jx​Jy​Jz​ via the anisotropy parameters. Finally, we calculate the noise $S(\ensuremath{\Omega})$ at finite frequency $\ensuremath{\Omega}$ for the isotropic Kondo model and find that the dephasing rate determines the height of the shoulders in $dS(\ensuremath{\Omega})∕d\ensuremath{\Omega}$ near $\ensuremath{\Omega}=V$.