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arXiv:cond-mat/0403425 · Physical Review Letters

Multiphoton Transitions in a Macroscopic Quantum Two-State System

Shiro Saito, Michael Thorwart, Hirotaka Tanaka, Masahito Ueda, H. Nakano, Kouichi Semba, Hideaki Takayanagi

Published Jul 15, 2004• 82 citations
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Abstract

We have observed multiphoton transitions between two macroscopic quantum-mechanical superposition states formed by two opposite circulating currents in a superconducting loop with three Josephson junctions. Resonant peaks and dips of up to three-photon transitions were observed in spectroscopic measurements when the system was irradiated with a strong rf-photon field. The widths of the multiphoton absorption dips are shown to scale with the Bessel functions in agreement with theoretical predictions derived from the Bloch equation or from a spin-boson model.

DOI
10.1103/physrevlett.93.037001

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We present a simple model to describe multiphoton transitions between the quasi-bound states of a current-driven Josephson junction. The transitions are induced by applying an ac voltage with controllable frequency and amplitude across the junction. The voltage induces transitions across the junction when the frequency $\ensuremath{\omega}$ satisfies $n\ensuremath{\hbar}\ensuremath{\omega}=\ensuremath{\Delta}{E}_{10}$, where $\ensuremath{\Delta}{E}_{10}$ is the splitting between the ground and first excited quasi-bound state of the junction. We calculate the matrix elements of the transitions as a function of the dc bias current III, and the frequency $\ensuremath{\omega}$ and amplitude Vac{V}_{\text{ac}}Vac​ of the microwave voltage, for representative junction parameters. We also calculate the frequency-dependent absorption coefficient by solving the relevant Bloch equations when the ac voltage is sufficiently weak. In this regime, the absorption coefficient is a sum of Lorentzian lines centered at the nnn-photon absorption frequency, of strength proportional to the squared matrix elements. For fixed Vac{V}_{\text{ac}}Vac​, the transition rate for an nnn-photon process usually decreases with increasing nnn. We also find a characteristic even-odd effect: The absorption coefficient typically increases with III for nnn even but decreases for nnn odd. Our results agree qualitatively with recent experiments.
The escape of a current-biased Josephson tunnel junction from the zero-voltage state in the presence of weak microwave radiation is investigated experimentally at low temperatures. The measurements of the junction switching current distribution indicate the macroscopic quantum tunneling of the phase below a crossover temperature of T small star, filled approximately 280 mK. At temperatures below T small star, filled we observe both single-photon and multiphoton transitions between the junction energy levels by applying microwave radiation in the frequency range between 10 and 38 GHz to the junction. These observations reflect the anharmonicity of the junction potential containing only a small number of levels.
Microwave spectroscopy experiments have been performed on two quantum levels of a macroscopic superconducting loop with three Josephson junctions. Level repulsion of the ground state and first excited state is found where two classical persistent-current states with opposite polarity are degenerate, indicating symmetric and antisymmetric quantum superpositions of macroscopic states. The two classical states have persistent currents of 0.5 microampere and correspond to the center-of-mass motion of millions of Cooper pairs.