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arXiv:cond-mat/0309652 · Physical Review E

Comment on “Fluctuation-dissipation relations in the nonequilibrium critical dynamics of Ising models”

Michel Pleimling

Published Jul 2, 2004• 12 citations
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Abstract

Recently Phys. Rev. E 68, 016116 (2003)]] proposed an alternative way to compute numerically the fluctuation-dissipation ratios in nonequilibrium critical systems. Using well-known facts of nonequilibrium critical dynamics I show that the leading contributions of the quantities they consider are in fact one-time quantities which are independent of the waiting time. The ratio of these one-time quantities determines the slope of the straight lines observed in the fluctuation-dissipation plots of Mayer et al.

DOI
10.1103/physreve.70.018101

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We have recently shown that in nonequilibrium spin systems at criticality the limit ${X}^{\ensuremath{\infty}}$ of the fluctuation-dissipation ratio $X(t,{t}_{w})$ for $t⪢{t}_{w}⪢1$ can be measured using observables such as magnetization or energy [Phys. Rev. E 68, 016116 (2003)]. Pleimling argues in a Comment [preceding paper, Phys. Rev. 70, 018101 (2004)] on our paper that for such observables correlation and response functions are dominated by one-time quantities dependent only on $t$, and are therefore not suitable for a determination of ${X}^{\ensuremath{\infty}}$. Using standard scaling forms of correlation and response functions, as used by Pleimling, we show that our data do have a genuine two-time dependence and allow $X(t,{t}_{w})$ and ${X}^{\ensuremath{\infty}}$ to be measured, so that Pleimling's criticisms are easily refuted. We also compare with predictions from renormalization-group calculations, which are consistent with our numerical observation of a fluctuation-dissipation plot for the magnetization that is very close to a straight line. A key point remains that coherent observables make measurements of ${X}^{\ensuremath{\infty}}$ easier than the traditionally used incoherent ones, producing fluctuation-dissipation plots whose slope is close to ${X}^{\ensuremath{\infty}}$ over a much larger range.

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Recently Phys. Rev. E 68, 016116 (2003)]] proposed an alternative way to compute numerically the fluctuation-dissipation ratios in nonequilibrium critical systems. Using well-known facts of nonequilibrium critical dynamics I show that the leading contributions of the quantities they consider are in fact one-time quantities which are independent of the waiting time. The ratio of these one-time quantities determines the slope of the straight lines observed in the fluctuation-dissipation plots of Mayer et al.
We have recently shown that in nonequilibrium spin systems at criticality the limit ${X}^{\ensuremath{\infty}}$ of the fluctuation-dissipation ratio X(t,tw)X(t,{t}_{w})X(t,tw​) for t⪢tw⪢1t⪢{t}_{w}⪢1t⪢tw​⪢1 can be measured using observables such as magnetization or energy [Phys. Rev. E 68, 016116 (2003)]. Pleimling argues in a Comment [preceding paper, Phys. Rev. 70, 018101 (2004)] on our paper that for such observables correlation and response functions are dominated by one-time quantities dependent only on ttt, and are therefore not suitable for a determination of ${X}^{\ensuremath{\infty}}$. Using standard scaling forms of correlation and response functions, as used by Pleimling, we show that our data do have a genuine two-time dependence and allow X(t,tw)X(t,{t}_{w})X(t,tw​) and ${X}^{\ensuremath{\infty}}$ to be measured, so that Pleimling's criticisms are easily refuted. We also compare with predictions from renormalization-group calculations, which are consistent with our numerical observation of a fluctuation-dissipation plot for the magnetization that is very close to a straight line. A key point remains that coherent observables make measurements of ${X}^{\ensuremath{\infty}}$ easier than the traditionally used incoherent ones, producing fluctuation-dissipation plots whose slope is close to ${X}^{\ensuremath{\infty}}$ over a much larger range.
We investigate the non-equilibrium critical evolution of statistical systems and describe of its some features, such as aging and violation of the fluctuation-dissipation theorem. We consider some theoretical results of computations for universal quantities that have been obtained in recent years, such as the exponents determining the scaling behavior of dynamic response and correlation functions and the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics. We derive our original Monte Carlo simulation results for 3D pure and diluted Ising models with Glauber and Metropolis dynamics. For these models, we analyze the influence of critical fluctuations, different non-equilibrium initial states, and the presence of nonmagnetic impurities on the two-time dependence of correlation and response functions on characteristic time variables, such as waiting time |twt_{\rm w}tw​| and time of observation |t−twt - t_{\rm w}t−tw​| with |t>twt>t_{\rm w}t>tw​|⁠. We discuss the obtained values of the non-equilibrium exponents for the autocorrelation and response functions and values of the universal long-time limit of the fluctuation-dissipation ratio |X∞X^{\infty }X∞|⁠. Our simulation results demonstrate that the insertion of disorder leads to new values of |X∞X^{\infty }X∞| with |Xdiluted∞>Xpure∞X_{\rm diluted}^{\infty }>X_{\rm pure}^{\infty }Xdiluted∞​>Xpure∞​|⁠.
It is considered the non-equilibrium critical evolution of statistical systems which displays some features, such as ageing and violation of the fluctuation-dissipation theorem. We review here some theoretical results of computations that have been obtained in recent years for universal quantities, such as the exponents determining the scaling behaviour of dynamic response and correlation functions and the fluctuation-dissipation ratio, associated with the non-equilibrium critical dynamics, with particular focus on the 3D pure and diluted Ising models with Glauber dynamics. We analyse an influence of critical fluctuations, different non-equilibrium initial states and presence of nonmagnetic impurities in spin systems on two-time dependence of correlation and response functions on characteristic time variables as waiting time t w and time of observation t – t w with t > t w . We discuss the obtained values of non-equilibrium exponents for autocorrelation and response functions and values of the universal long-time limit of the fluctuation-dissipation ratio X ∞ . Analysis of simulation results show that the insertion of disorder leads to new values of X ∞ with X ∞ diluted > X ∞ pure .
Available mathematical results entail the absence of a proper ordering transition taking place at finite temperature in the case d=1,d=1,d=1, $\ensuremath{\sigma}=1.1,$ where the authors of the article commented on find evidence of such a transition. Moreover, in contrast to the findings of the authors of the article, the case d=2,d=2,d=2, $\ensuremath{\sigma}=0$ entails a ground-state energy per particle diverging logarithmically with increasing sample size, hence an infinite transition temperature.