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arXiv:cond-mat/0309619 · Physical Review Letters

Negative Differential Conductance Induced by Spin-Charge Separation

Fabio Cavaliere, Alessandro Braggio, Jürgen T. Stockburger, Maura Sassetti, B. Krämer

Published Jul 13, 2004• 40 citations
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Abstract

Spin-charge states of correlated electrons in a one-dimensional quantum dot attached to interacting leads are studied in the nonlinear transport regime. With nonsymmetric tunnel barriers, regions of negative differential conductance induced by spin-charge separation are found. They are due to a correlation-induced trapping of higher-spin states without magnetic field and are associated with a strong increase in the fluctuations of the electron spin.

DOI
10.1103/physrevlett.93.036803

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Spin-charge states of correlated electrons in a one-dimensional quantum dot attached to interacting leads are studied in the nonlinear transport regime. With nonsymmetric tunnel barriers, regions of negative differential conductance induced by spin-charge separation are found. They are due to a correlation-induced trapping of higher-spin states without magnetic field and are associated with a strong increase in the fluctuations of the electron spin.
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We study the charge conductivity in one-dimensional prototype models of interacting particles, such as the Hubbard and the $t\text{\ensuremath{-}}V$ spinless fermion models, when coupled to some external baths injecting and extracting particles at the boundaries. We show that, if these systems are driven far from equilibrium, a negative differential conductivity regime can arise. The above electronic models can be mapped into Heisenberg-like spin ladders coupled to two magnetic baths, so that charge transport mechanisms are explained in terms of quantum spin transport. The negative differential conductivity is due to oppositely polarized ferromagnetic domains that arise at the edges of the chain and therefore inhibit spin transport: we propose a qualitative understanding of the phenomenon by analyzing the localization of one-magnon excitations created at the borders of a ferromagnetic region. We also show that negative differential conductivity is stable against breaking of integrability. Numerical simulations of nonequilibrium time evolution have been performed by employing a Monte Carlo wave function approach and a matrix product operator formalism.
Interactions in one-dimensional (1D) electron systems are expected to cause a dynamical separation of electronic spin and charge degrees of freedom. A promising system for experimental observation of this non-Fermi-liquid effect consists of two quantum wires coupled via tunneling through an extended uniform barrier. Here we consider the minimal model of an interacting 1D electron system exhibiting spin-charge separation, and calculate the differential tunneling conductance as well as the density-density response function. Both quantities exhibit distinct strong features arising from spin-charge separation. Our analysis of these features within the minimal model neglects interactions between electrons of opposite chirality, and therefore applies directly to chiral 1D electron systems realized, e.g., at the edge of integer quantum Hall systems. Physical insight gained from our results is useful for interpreting current experiment in quantum wires, as our main conclusions still apply with nonchiral interactions present. In particular, we discuss the effect of charging due to applied voltages, and the possibility to observe spin-charge separation in a time-resolved experiment.
Several recent results concerning frequency dependent and nonlinear transport of one-dimensional correlated electrons are reviewed. The frequency dependent conductance of a Luttinger liquid is discussed. For zero-range interaction the conductance is similar to that of a non-interacting ideal quantum wire, with a renormalized zero-frequency limit. For a screened Coulomb potential, the conductance as a function of the frequency shows features of the elementary excitations. They can be simulated in terms of a capacitance, an inductance and a resistance. The non-linear DC-conductance of the Luttinger liquid in presence of a tunnel barrier shows Coulomb blockade if the interaction is of finite range. The capacitance scales in the same way as for the system without the tunnel barrier. The linear DC-response of a tunnel barrier as a function of the frequency and the voltage of a monochromatic driving field shows oscillations which can be interpreted as signature of a frequency-induced depinning of a charge density wave.
Semiconductor double‐quantum dots represent an ideal system for studying the novel spin physics of localized spins. On each quantum dot when the number of electrons is odd and the net spin is 1/2, a strong coupling of this localized spin to conducting electrons in the leads gives rise to Kondo correlation. On the other hand, in the coupled double‐quantum‐dot if the inter‐dot antiferromagnetic interaction is strong, the two spins can form a correlated spin‐singlet state, quenching the Kondo effect. This competition between Kondo and antiferromagnetic correlation is studied in a controlled manner by tuning the inter‐dot tunnel coupling. Increasing the inter‐dot tunneling, we observe a continuous transition from a single‐peaked to a double‐peaked Kondo resonance in the differential conductance. On the double‐peaked side, the differential conductance becomes suppressed at zero source‐drain bias. The observed strong suppression of the differential conductance at zero bias provides direct evidence signaling the formation of an entangled spin‐singlet state. This evidence for entanglement and the tunability of our devices bode well for quantum computation applications.
We study low energy spin and charge transport through a 1D Mott-Hubbard insulator of finite length LLL attached to Fermi liquid reservoirs characterized by different chemical potentials for electrons of opposite spin polarizations as it happens in quantum spin Hall insulators. We calculate the average currents (charge and spin) and their correlators and demonstrate how a transition induced by the reservoirs to the low energy Fermi liquid regime results in breakdown of the spin-charge separation, which is visible in the presence of the spin dependent voltages and a weak one electron scattering in the system. These calculations are carried out under assumption that the Hubbard gap 2M is large enough: M>TL≡vc/LM > T_L \equiv v_c/LM>TL​≡vc​/L (vcv_cvc​: charge velocity in the wire) and the scattering rate Γs≪TLΓ_s \ll T_LΓs​≪TL​. Relation of these results to Kondo dot transport in the Toulouse limit is also clarified.