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arXiv:cond-mat/0309284 · Lecture notes in physics

Dynamics of Dissipative Quantum Systems: From Path Integrals to Master Equations

Joachim Ankerhold

Published Jan 1, 2003• 8 citations
arXivHTMLPDF
DOI
10.1007/3-540-44874-8_9

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The time-convolutionless quantum master equation is widely used to simulate reduced dynamics of a quantum system coupled to a bath. However, except for several special cases, applications of this equation are based on perturbative calculation of the dissipative tensor, and are limited to the weak system-bath coupling regime. In this paper, we derive an exact time-convolutionless quantum master equation from the path integral approach, which provides a new way to calculate the dissipative tensor nonperturbatively. Application of the new method is demonstrated in the case of an asymmetrical two-level system linearly coupled to a harmonic bath.
A systematic procedure for deriving the master equation of a dissipative system is reported in the framework of stochastic description. For the Caldeira-Leggett model of the harmonic-oscillator bath, a detailed and elementary derivation of the bath-induced stochastic field is presented. The dynamics of the system is thereby fully described by a stochastic differential equation, and the desired master equation would be acquired with statistical averaging. It is shown that the existence of a closed-form master equation depends on the specificity of the system as well as the feature of the dissipation characterized by the spectral density function. For a dissipative harmonic oscillator it is observed that the correlation between the stochastic field due to the bath and the system can be decoupled, and the master equation naturally results. Such an equation possesses the Lindblad form in which time-dependent coefficients are determined by a set of integral equations. It is proved that the obtained master equation is equivalent to the well-known Hu-Paz-Zhang equation based on the path-integral technique. The procedure is also used to obtain the master equation of a dissipative harmonic oscillator in time-dependent fields.
Consistent dynamics which couples classical and quantum degrees of freedom exists. This dynamics is linear in the hybrid state, completely positive and trace preserving. Starting from completely positive classical-quantum master equations, we derive a general path integral representation for such dynamics in terms of a classical-quantum action, which includes the necessary and sufficient conditions for complete positivity and trace preservation. The path integral we study is a generalization of the Feynman path integral for quantum systems, and the stochastic path integral used to study classical stochastic processes, allowing for interaction between the classical and quantum systems. When the classical-quantum Hamiltonian is at most quadratic in the momenta we are able to derive a configuration space path integral, providing a map between master equations and covariant classical-quantum path integrals.