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arXiv:cond-mat/0309140 · Reports on Progress in Physics

Metal–insulator transition in two-dimensional electron systems

S V Kravchenko, M P Sarachik

Published Dec 2, 2003• 448 citations
arXivHTMLPDF

Abstract

The interplay between strong Coulomb interactions and randomness has been a long-standing problem in condensed matter physics. According to the scaling theory of localization in two-dimensional systems of non-interacting or weakly interacting electrons, the ever-present randomness causes the resistance to rise as the temperature is decreased, leading to an insulating ground state. However, new evidence has emerged within the past decade indicating a transition from the insulating to metallic phase in two-dimensional systems of strongly interacting electrons. We review earlier experiments that demonstrate the unexpected presence of a metallic phase in two dimensions, and present an overview of recent experiments with emphasis on the anomalous magnetic properties that have been observed in the vicinity of the transition.

DOI
10.1088/0034-4885/67/1/r01

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The interplay between strong Coulomb interactions and randomness has been a long-standing problem in condensed matter physics. According to the scaling theory of localization in two-dimensional systems of non-interacting or weakly interacting electrons, the ever-present randomness causes the resistance to rise as the temperature is decreased, leading to an insulating ground state. However, new evidence has emerged within the past decade indicating a transition from the insulating to metallic phase in two-dimensional systems of strongly interacting electrons. We review earlier experiments that demonstrate the unexpected presence of a metallic phase in two dimensions, and present an overview of recent experiments with emphasis on the anomalous magnetic properties that have been observed in the vicinity of the transition.
(received; accepted) PACS. 71.30+h – Metal-insulator transitions and other electronic transitions. PACS. 72.15Rn – Quantum localization. PACS. 71.27+a – Strongly correlated electron systems. Abstract. – Extending finite size scaling theory to the many body ground state, one finds that Coulomb repulsion can drive a system of spinless fermions in a random potential from the Anderson insulator (Fermi glass of localized states) towards a new extended phase in dimension d = 2. The transition occurs at a Coulomb energy to Fermi energy ratio rs ≈ 4, where a change in the nature of the persistent currents has been previously observed. Relevance to the recently observed 2d metallic phase is suggested. Following the scaling theory of localization [1], all 2d systems of electrons (or holes) are localized when electron-electron interaction is negligible. This absence of metals in two dimensions is nowadays questioned after the observation of a transition towards a metallic behavior in silicon based 2d electron gases [2, 3, 4] when the carrier density is varied. This unexpected phenomenon occurs also for hole gases in GaAs heterostructures [5, 6], SiGe [7]
We present a theory of the metal-insulator transition in a disordered two-dimensional electron gas. A quantum critical point, separating the metallic phase, which is stabilized by electronic interactions, from the insulating phase, where disorder prevails over the electronic interactions, has been identified. The existence of the quantum critical point leads to a divergence in the density of states of the underlying collective modes at the transition, causing the thermodynamic properties to behave critically as the transition is approached. We show that the interplay of electron-electron interactions and disorder can explain the observed transport properties and the anomalous enhancement of the spin susceptibility near the metal-insulator transition.
We study the effects of electron-electron interactions in disordered metals in and close to two dimensions (2D). We consider physical situations in which localization effects are suppressed. The field-theoretical renormalization-group (RG) calculation performed recently by Finkelstein is interpreted and rederived in terms of perturbative results. Surprisingly, except for the density of states, the scaling behavior is independent of the interaction range. We further extend the model to several new universality classes. In the presence of a strong magnetic field the metal is unstable in 2D and undergoes a metal-insulator transition in $d=2+\ensuremath{\epsilon}$. The conductivity exponent, defined by $\ensuremath{\sigma}\ensuremath{\sim}{(n\ensuremath{-}{n}_{c})}^{\ensuremath{\mu}}$, is universal with $\ensuremath{\mu}=1+O(\ensuremath{\epsilon})$ but N(EF)N({E}_{F})N(EF​) depends not only on the range of the interaction but also on its strength for short-ranged interactions. In 2D the conductivity has a universal temperature dependence [$\ensuremath{\delta}\ensuremath{\sigma}(T)={\ensuremath{\sigma}}_{N}(2\ensuremath{-}2\mathrm{ln}2)\mathrm{ln}(T\ensuremath{\tau})$, ${\ensuremath{\sigma}}_{N}=\frac{{e}^{2}}{2{\ensuremath{\pi}}^{2}\ensuremath{\hbar}}$] if the interaction is Coulombic. If magnetic impurities (or strong spin-orbit scattering with a weak magnetic field) are present instead, the noninteracting fixed point is stable for short-ranged interactions ($\ensuremath{\mu}=\frac{1}{2}$). For the Coulomb interaction the interaction is relevant and drives a metal-insulator transition in $d=2+\ensuremath{\epsilon}$ with universal critical properties ($\ensuremath{\mu}=1$). In 2D the conductivity also has a universal temperature dependence [$\ensuremath{\delta}\ensuremath{\sigma}(T)={\ensuremath{\sigma}}_{N}\mathrm{ln}(T\ensuremath{\tau})$]. We also discuss the behavior of the dielectric constant on the insulator side and the frequency (temperature) dependence of the conductivity at criticality. Remarks are made on the relationship of the above to experiments.
We reconcile the possible presence of a quantum critical point in metal insulator transition phenomena in two-dimensional electron systems with observed electronic properties in the low resistivity region which are those of a weakly disordered Fermi liquid. The central issue of whether the ground state of an interacting 2D electron system in the presence of weak potential scattering from disorder is a metal or an insulator remains unresolved. Additional new effects which may become important at extremely low electron densities are briefly mentioned.
Abstract: The metal–insulator transition (MIT) constitutes one of the most profound and persistent problems in condensed matter physics, sitting at the intersection of electronic structure theory, many-body physics, and emergent quantum phenomena. Conventional band theory, which successfully classifies materials as metals or insulators according to the filling of their electronic bands, fails dramatically when confronted with a class of compounds transition metal oxides chief among them that ought to be metallic by band-counting arguments yet are robustly insulating in the laboratory. The resolution of this paradox required abandoning the independent-electron picture entirely and recognizing that strong Coulomb repulsion between electrons can, by itself, drive localization. This insight, formalized by Mott and later distilled into the Hubbard model, established correlation-driven insulation as a phenomenon distinct from band insulation. The present paper offers a theoretical exploration of the MIT problem, tracing its conceptual development from the Mott criterion through the Hubbard Hamiltonian, the Brinkman–Rice scenario of quasiparticle mass divergence, and the watershed development of dynamical mean-field theory (DMFT), which rendered the Mott transition quantitatively tractable for the first time. We argue that the competition between the electronic bandwidth and the on-site interaction encoded in the ratio U/W provides the unifying organizing principle for the field. Building toward the modern frontier, we examine how the Mott transition connects to quantum phase transitions and quantum criticality, where zero-temperature instabilities governed by quantum rather than thermal fluctuations produce non-Fermi-liquid behavior and anomalous scaling. Case studies of vanadium oxides, rare-earth nickelates, and doped cuprates illustrate the diversity and subtlety of real correlated materials. We conclude that the MIT remains a central and unresolved problem whose continued study is increasingly entangled with the development of quantum materials and quantum technologies. Keywords: Metal–Insulator Transition; Mott Insulator; Strongly Correlated Electrons; Hubbard Model; DMFT; Quantum Criticality; Quantum Materials; Condensed Matter Physics