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arXiv:cond-mat/0308459 · Physical Review Letters

Controlling a Mesoscopic Spin Environment by Quantum Bit Manipulation

Jacob M. Taylor, Ataç İmamoğlu, Mikhail D. Lukin

Published Dec 10, 2003• 130 citations
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Abstract

We present a unified description of cooling and manipulation of a mesoscopic bath of nuclear spins via coupling to a single quantum system of electronic spin (quantum bit). We show that a bath cooled by the quantum bit rapidly saturates. Although the resulting saturated states of the spin bath ("dark states") generally have low degrees of polarization and purity, their symmetry properties make them a valuable resource for the coherent manipulation of quantum bits. Specifically, we demonstrate that the dark states of nuclear ensembles can be used to coherently control the system-bath interaction and to provide a robust, long-lived quantum memory for qubit states.

DOI
10.1103/physrevlett.91.246802

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We present a unified description of cooling and manipulation of a mesoscopic bath of nuclear spins via coupling to a single quantum system of electronic spin (quantum bit). We show that a bath cooled by the quantum bit rapidly saturates. Although the resulting saturated states of the spin bath ("dark states") generally have low degrees of polarization and purity, their symmetry properties make them a valuable resource for the coherent manipulation of quantum bits. Specifically, we demonstrate that the dark states of nuclear ensembles can be used to coherently control the system-bath interaction and to provide a robust, long-lived quantum memory for qubit states.
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We describe a technique to create long-lived quantum memory for quantum bits in mesoscopic systems. Specifically we show that electronic spin coherence can be reversibly mapped onto the collective state of the surrounding nuclei. The coherent transfer can be efficient and fast and it can be used, when combined with standard resonance techniques, to reversibly store coherent superpositions on the time scale of seconds. This method can also allow for "engineering" entangled states of nuclear ensembles and efficiently manipulating the stored states. We investigate the feasibility of this method through a detailed analysis of the coherence properties of the system.
We describe a technique for quantum information processing based on localized en sembles of nuclear spins. A qubit is identified as the presence or absence of a collective excitation of a mesoscopic ensemble of nuclear spins surrounding a single quantum dot. All single and two-qubit operations can be effected using hyperfine interactions and single-electron spin rotations, hence the proposed scheme avoids gate errors arising from entanglement between spin and orbital degrees of freedom. Ultra-long coherence times of nuclear spins suggest that this scheme could be particularly well suited for applications where long lived memory is essential.
The key challenge in experimental quantum information science is to identify isolated quantum mechanical systems with long coherence times that can be manipulated and coupled together in a scalable fashion. We describe the coherent manipulation of an individual electron spin and nearby individual nuclear spins to create a controllable quantum register. Using optical and microwave radiation to control an electron spin associated with the nitrogen vacancy (NV) color center in diamond, we demonstrated robust initialization of electron and nuclear spin quantum bits (qubits) and transfer of arbitrary quantum states between them at room temperature. Moreover, nuclear spin qubits could be well isolated from the electron spin, even during optical polarization and measurement of the electronic state. Finally, coherent interactions between individual nuclear spin qubits were observed and their excellent coherence properties were demonstrated. These registers can be used as a basis for scalable, optically coupled quantum information systems.
Spin degrees of freedom have been extensively explored in the context of quantum information processing. Many proposals of quantum computation architectures use spins as carriers of quantum of information. A central problem is to efficiently generate quantum entanglement between spin qubits which proves to be a crucial resource for quantum information tasks. On the other hand, uncontrollable spin degrees of freedom in the environment of spin qubits are the major causes of errors at low temperature, for example, the lattice nuclear spins hyperfine coupled to single electron spin qubit localized in semiconductor nano-structures. An outstanding problem for scalable quantum computation is to suppress the collective fluctuations from such spin baths so that the coherence time of the spin qubit can be improved. With these two motivations, the problems of suppressing collective spin fluctuations and generating entanglement in various spin ensembles are addressed in this thesis.\n\n\n\nIn the first half of the thesis, two approaches are introduced for suppressing the collective fluctuations in the nuclear spin bath so that the quantum coherence time of electron spin qubit in semiconductor quantum dots can be improved. The first approach works for a coupled double dot system. A theory for the interaction with the nuclear spins is developed when the two-electron singlet state is in resonance with one of the triplet state in moderate external magnetic field. At this resonance condition, the nuclear-electron flip-flop process caused by the hyperfine interaction can lead to a feedback mechanism, which can be used to suppress the nuclear hyperfine field. The second approach works for a single dot system. It is shown that strong pumping of the nuclear spins in dynamic nuclear polarization processes can saturate the nuclear spin bath towards the collective “dark states”. In such dark states, the transverse nuclear field fluctuation can be substantially suppressed compared to the value at thermal equilibrium. Two physical schemes are proposed to realize the nuclear dark states for suppression of the nuclear field fluctuations.\n\n\n\nIn the second half of the thesis, schemes are presented for generating large scale quantum entanglement in two types of spin qubit systems. For atomic spin qubits in optical lattices, schemes are proposed on how to prepare pure spin coherent state (SCS) with low collective spin by incoherent pumping with collective spin raising and lowering operations. Such SCS realize networks of mutually entangled spins which can be idea resources for the quantum telecloning algorithm. For donor nuclear spin qubits in silicon architecture, proposals are shown on how to deterministic prepare Dicke states which constitute an important class of multipartite entangled states. Our scheme is capable of preparing both symmetric and asymmetric Dicke states which form a complete basis set of the spin Hilbert space. The required controls are in situ to the prototype Kane’s quantum computer. The preparation is robust because each desired Dicke state is the steady state under designed pumping process. The schemes presented here also make possible the construction of decoherence free subspaces where quantum information is protected from collective noises.