Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:cond-mat/0306204 · Physical Review A

Spin-exchange interactions of spin-one bosons in optical lattices: Singlet, nematic, and dimerized phases

Adilet Imambekov, Mikhail D. Lukin, Eugene Demler

Published Dec 4, 2003• 242 citations
arXivHTMLPDF

Abstract

We consider insulating phases of cold spin-1 bosonic particles with antiferromagnetic interactions, such as ${}^{23}\mathrm{Na},$ in optical lattices. We show that spin-exchange interactions give rise to several distinct phases, which differ in their spin correlations. In two- and three-dimensional lattices, insulating phases with an odd number of particles per site are always nematic. For insulating states with an even number of particles per site, there is always a spin-singlet phase, and there may also be a first-order transition into the nematic phase. The nematic phase breaks spin rotational symmetry but preserves time reversal symmetry, and has gapless spin-wave excitations. The spin-singlet phase does not break spin symmetry and has a gap to all excitations. In one-dimensional lattices, insulating phases with an odd number of particles per site always have a regime where translational symmetry is broken and the ground state is dimerized. We discuss signatures of various phases in Bragg scattering and time-of-flight measurements.

DOI
10.1103/physreva.68.063602

Related papers

Spinful bosons in an optical lattice

Sara Bergkvist, Ian P. McCulloch, Anders Rosengren

We analyze the behavior of cold spin-1 particles with antiferromagnetic interactions in a one-dimensional optical lattice using density matrix renormalization group calculations. Correlation functions and the dimerization are shown and we also present results for the energy gap between ground state and the spin excited states. We confirm the anticipated phase diagram, with Mott-insulating regions of alternating dimerized $S=1$ chains for odd particle density versus on-site singlets for even density. We find no evidence for any additional ordered phases in the physically accessible region, however for sufficiently large spin interaction, on-site singlet pairs dominate leading, for odd density, to a breakdown of the Mott insulator or, for even density, a real-space singlet superfluid.

arXiv:cond-mat/0606265•Physical Review A•Nov 28, 2006•25 citations

Quantum Insulating States of F=2 Cold Atoms in Optical Lattices

Fei Zhou, Gordon Walter Semenoff

In this Letter we study various spin correlated insulating states of F=2 cold atoms in optical lattices. We find that the effective spin exchange interaction due to virtual hopping contains an octopole coupling between two neighboring lattice sites. Depending on scattering lengths and numbers of particles per site the ground states are either rotationally invariant dimer or trimer Mott insulators or insulating states with various spin orders. Three spin-ordered insulating phases are ferromagnetic, cyclic, and nematic Mott insulators. We estimate the phase boundaries for states with different numbers of atoms per lattice site.

arXiv:cond-mat/0607463•Physical Review Letters•Nov 2, 2006•47 citations

Spin and quadruple correlations in the insulating nematic phase of spin-1 bosons on optical lattices

Guang-Ming Zhang, Yu, Lu

We consider the effective model of $H=-J_{1}\sum_{}\mathbf{S}_{i}\cdot \mathbf{S}_{j}-J_{2}\sum_{}(\mathbf{S}_{i}\cdot \mathbf{S}_{j}) ^{2}$, describing the Mott insulating phase with odd number of spin-1 bosons in optical lattices ($J_{2}>J_{1}>0$). In terms of an SU(3) boson representation, a valence bond mean field theory is developed. In 1D, a \textit{first-order} quantum phase transition from a spin singlet to a spin nematic phase with \textit{gapful} excitations is identified at $ J_{1}/J_{2}=0.19833$, while on a 2D square lattice a spin nematic ordered phase with gapless excitations prevails. In both 1D and 2D cases, we predict that the spin structure factor displays dominant antiferromagnetic fluctuations, while the quadrupole structure factor exhibits strong ferroquadrupolar correlations.

arXiv:cond-mat/0507158•Jul 7, 2005•0 citations

Interacting spin-1 bosons in a two-dimensional optical lattice

Laurent de Forges de Parny, F. Hébert, V. G. Rousseau +1 more

We study, using quantum Monte Carlo (QMC) simulations, the ground state properties of spin-1 bosons trapped in a square optical lattice. The phase diagram is characterized by the mobility of the particles (Mott insulating or superfluid phase) and by their magnetic properties. For ferromagnetic on-site interactions, the whole phase diagram is ferromagnetic and the Mott insulators-superfluid phase transitions are second order. For antiferromagnetic on-site interactions, spin nematic order is found in the odd Mott lobes and in the superfluid phase. Furthermore, the superfluid-insulator phase transition is first or second order depending on whether the density in the Mott is even or odd. Inside the even Mott lobes we observe a singlet-to-nematic transition for certain values of the interactions. This transition appears to be first order.

arXiv:1306.5515•Physical Review B•Sep 10, 2013•26 citations

Magnetically stabilized nematic order: Three-dimensional bipartite optical lattices

Fei Zhou, Michiel Snoek, Jeroen Wiemer +1 more

We study magnetically stabilized nematic order for spin-one bosons in optical lattices. We show that the Zeeman field-driven quantum phase transitions between non-nematic Mott states and quantum spin nematic Mott states in the weak hopping limit are in the universality class of the ferromagnetic $XXZ$ $(S=1∕2)$ spin model. We further discuss these transitions as condensation of interacting magnons. The development of O(2) nematic order when external fields are applied corresponds to condensation of magnons, which breaks a U(1) symmetry. Microscopically, this results from a coherent superposition of two non-nematic states at each individual site. Nematic order and spin-wave excitations around critical points are studied and critical behaviors are obtained in a dilute gas approximation. We also find that spin-singlet states are unstable with respect to quadratic Zeeman effects and Ising nematic order appears in the presence of any finite quadratic Zeeman coupling. All discussions are carried out for states in three-dimensional bipartite lattices.

arXiv:cond-mat/0407259•Physical Review B•Nov 24, 2004•24 citations

Static and dynamic properties of interacting spin-1 bosons in an optical lattice

Stefan S. Natu, J. H. Pixley, S. Das Sarma

We study the physics of interacting spin-1 bosons in an optical lattice using a variational Gutzwiller technique. We compute the mean-field ground state wave function and discuss the evolution of the condensate, spin, nematic, and singlet order parameters across the superfluid-Mott transition. We then extend the Gutzwiller method to derive the equations governing the dynamics of low energy excitations in the lattice. Linearizing these equations, we compute the excitation spectra in the superfluid and Mott phases for both ferromagnetic and antiferromagnetic spin-spin interactions. In the superfluid phase, we recover the known excitation spectrum obtained from Bogoliubov theory. In the nematic Mott phase, we obtain gapped, quadratically dispersing particle and hole-like collective modes, whereas in the singlet Mott phase, we obtain a nondispersive gapped mode, corresponding to the breaking of a singlet pair. For the ferromagnetic Mott insulator, the Gutzwiller mean-field theory only yields particle-hole-like modes but no Goldstone mode associated with long-range spin order. To overcome this limitation, we supplement the Gutzwiller theory with a Schwinger boson mean-field theory which captures superexchange-driven fluctuations. In addition to the gapped particle-hole-like modes, we obtain a gapless quadratically dispersing ferromagnetic spin-wave Goldstone mode. We discuss the evolution of the singlet gap, particle-hole gap, and the effective mass of the ferromagnetic Goldstone mode as the superfluid-Mott phase boundary is approached from the insulating side. We discuss the relevance and validity of Gutzwiller mean-field theories to spinful systems, and potential extensions of this framework to include more exotic physics which appears in the presence of spin-orbit coupling or artificial gauge fields.

arXiv:1502.01041•Physical Review A•Apr 14, 2015•23 citations
We consider insulating phases of cold spin-1 bosonic particles with antiferromagnetic interactions, such as 23Na,{}^{23}\mathrm{Na},23Na, in optical lattices. We show that spin-exchange interactions give rise to several distinct phases, which differ in their spin correlations. In two- and three-dimensional lattices, insulating phases with an odd number of particles per site are always nematic. For insulating states with an even number of particles per site, there is always a spin-singlet phase, and there may also be a first-order transition into the nematic phase. The nematic phase breaks spin rotational symmetry but preserves time reversal symmetry, and has gapless spin-wave excitations. The spin-singlet phase does not break spin symmetry and has a gap to all excitations. In one-dimensional lattices, insulating phases with an odd number of particles per site always have a regime where translational symmetry is broken and the ground state is dimerized. We discuss signatures of various phases in Bragg scattering and time-of-flight measurements.
We analyze the behavior of cold spin-1 particles with antiferromagnetic interactions in a one-dimensional optical lattice using density matrix renormalization group calculations. Correlation functions and the dimerization are shown and we also present results for the energy gap between ground state and the spin excited states. We confirm the anticipated phase diagram, with Mott-insulating regions of alternating dimerized S=1S=1S=1 chains for odd particle density versus on-site singlets for even density. We find no evidence for any additional ordered phases in the physically accessible region, however for sufficiently large spin interaction, on-site singlet pairs dominate leading, for odd density, to a breakdown of the Mott insulator or, for even density, a real-space singlet superfluid.
In this Letter we study various spin correlated insulating states of F=2 cold atoms in optical lattices. We find that the effective spin exchange interaction due to virtual hopping contains an octopole coupling between two neighboring lattice sites. Depending on scattering lengths and numbers of particles per site the ground states are either rotationally invariant dimer or trimer Mott insulators or insulating states with various spin orders. Three spin-ordered insulating phases are ferromagnetic, cyclic, and nematic Mott insulators. We estimate the phase boundaries for states with different numbers of atoms per lattice site.
We consider the effective model of H=−J1∑Si⋅Sj−J2∑(Si⋅Sj)2H=-J_{1}\sum_{}\mathbf{S}_{i}\cdot \mathbf{S}_{j}-J_{2}\sum_{}(\mathbf{S}_{i}\cdot \mathbf{S}_{j}) ^{2}H=−J1​∑​Si​⋅Sj​−J2​∑​(Si​⋅Sj​)2, describing the Mott insulating phase with odd number of spin-1 bosons in optical lattices (J2>J1>0J_{2}>J_{1}>0J2​>J1​>0). In terms of an SU(3) boson representation, a valence bond mean field theory is developed. In 1D, a \textit{first-order} quantum phase transition from a spin singlet to a spin nematic phase with \textit{gapful} excitations is identified at $ J_{1}/J_{2}=0.19833$, while on a 2D square lattice a spin nematic ordered phase with gapless excitations prevails. In both 1D and 2D cases, we predict that the spin structure factor displays dominant antiferromagnetic fluctuations, while the quadrupole structure factor exhibits strong ferroquadrupolar correlations.
We study, using quantum Monte Carlo (QMC) simulations, the ground state properties of spin-1 bosons trapped in a square optical lattice. The phase diagram is characterized by the mobility of the particles (Mott insulating or superfluid phase) and by their magnetic properties. For ferromagnetic on-site interactions, the whole phase diagram is ferromagnetic and the Mott insulators-superfluid phase transitions are second order. For antiferromagnetic on-site interactions, spin nematic order is found in the odd Mott lobes and in the superfluid phase. Furthermore, the superfluid-insulator phase transition is first or second order depending on whether the density in the Mott is even or odd. Inside the even Mott lobes we observe a singlet-to-nematic transition for certain values of the interactions. This transition appears to be first order.
We study magnetically stabilized nematic order for spin-one bosons in optical lattices. We show that the Zeeman field-driven quantum phase transitions between non-nematic Mott states and quantum spin nematic Mott states in the weak hopping limit are in the universality class of the ferromagnetic XXZXXZXXZ (S=1∕2)(S=1∕2)(S=1∕2) spin model. We further discuss these transitions as condensation of interacting magnons. The development of O(2) nematic order when external fields are applied corresponds to condensation of magnons, which breaks a U(1) symmetry. Microscopically, this results from a coherent superposition of two non-nematic states at each individual site. Nematic order and spin-wave excitations around critical points are studied and critical behaviors are obtained in a dilute gas approximation. We also find that spin-singlet states are unstable with respect to quadratic Zeeman effects and Ising nematic order appears in the presence of any finite quadratic Zeeman coupling. All discussions are carried out for states in three-dimensional bipartite lattices.
We study the physics of interacting spin-1 bosons in an optical lattice using a variational Gutzwiller technique. We compute the mean-field ground state wave function and discuss the evolution of the condensate, spin, nematic, and singlet order parameters across the superfluid-Mott transition. We then extend the Gutzwiller method to derive the equations governing the dynamics of low energy excitations in the lattice. Linearizing these equations, we compute the excitation spectra in the superfluid and Mott phases for both ferromagnetic and antiferromagnetic spin-spin interactions. In the superfluid phase, we recover the known excitation spectrum obtained from Bogoliubov theory. In the nematic Mott phase, we obtain gapped, quadratically dispersing particle and hole-like collective modes, whereas in the singlet Mott phase, we obtain a nondispersive gapped mode, corresponding to the breaking of a singlet pair. For the ferromagnetic Mott insulator, the Gutzwiller mean-field theory only yields particle-hole-like modes but no Goldstone mode associated with long-range spin order. To overcome this limitation, we supplement the Gutzwiller theory with a Schwinger boson mean-field theory which captures superexchange-driven fluctuations. In addition to the gapped particle-hole-like modes, we obtain a gapless quadratically dispersing ferromagnetic spin-wave Goldstone mode. We discuss the evolution of the singlet gap, particle-hole gap, and the effective mass of the ferromagnetic Goldstone mode as the superfluid-Mott phase boundary is approached from the insulating side. We discuss the relevance and validity of Gutzwiller mean-field theories to spinful systems, and potential extensions of this framework to include more exotic physics which appears in the presence of spin-orbit coupling or artificial gauge fields.