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arXiv:cond-mat/0304548 · Physical Review A

Properties of a dilute Bose gas near a Feshbach resonance

Lan Yin, Zhenhua Ning

Published Sep 19, 2003• 8 citations
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Abstract

In this paper, properties of a homogeneous Bose gas with a Feshbach resonance are studied in the dilute region at zero temperature. The stationary state contains condensations of atoms and molecules. The ratio of the molecule density to the atom density is $\ensuremath{\pi}{\mathrm{na}}^{3}.$ There are two types of excitations, molecular excitations and atomic excitations. Atomic excitations are gapless, consistent with the traditional theory of a dilute Bose gas. The molecular excitation energy is finite in the long-wavelength limit as observed in recent experiments on ${}^{85}\mathrm{Rb}.$ In addition, the decay process of the condensate is studied. The coefficient of the three-body recombination rate is about 140 times larger than that of a Bose gas without a Feshbach resonance, in reasonably good agreement with the experiment on ${}^{23}\mathrm{Na}.$

DOI
10.1103/physreva.68.033608

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In this paper, properties of a homogeneous Bose gas with a Feshbach resonance are studied in the dilute region at zero temperature. The stationary state contains condensations of atoms and molecules. The ratio of the molecule density to the atom density is \ensuremathπna3.\ensuremath{\pi}{\mathrm{na}}^{3}.\ensuremathπna3. There are two types of excitations, molecular excitations and atomic excitations. Atomic excitations are gapless, consistent with the traditional theory of a dilute Bose gas. The molecular excitation energy is finite in the long-wavelength limit as observed in recent experiments on 85Rb.{}^{85}\mathrm{Rb}.85Rb. In addition, the decay process of the condensate is studied. The coefficient of the three-body recombination rate is about 140 times larger than that of a Bose gas without a Feshbach resonance, in reasonably good agreement with the experiment on 23Na.{}^{23}\mathrm{Na}.23Na.
In this paper, we study the three-body recombination rate of a homogeneous dilute Bose gas with a Feshbach resonance at zero temperature. The ground state and excitations of this system are obtained. The three-body recombination in the ground state is due to the breakup of an atom pair in the quantum depletion and the formation of a molecule by an atom from the broken pair and an atom from the condensate. The rate of this process is in good agreement with the experiment on 23Na^{23}\mathrm{Na}23Na in a wide range of magnetic fields.
Bose-Einstein condensation (BEC) of Feshbach molecules in a homogeneous Bose gas is studied at finite temperatures in a single-channel mean-field approach where the Hartree-Fock energy and pairing gap are determined self-consistently. In the molecular-BEC state, the atomic excitation is gapped and the molecular excitation is gapless. The binding energy of Feshbach molecules is shifted from the vacuum value by many-body effects. When the scattering length as{a}_{s}as​ of the atoms is negative, the system is subject to mechanical collapse due to negative compressibility. The system is stable in most regions with positive scattering lengths. However, at low temperatures near the resonance, the molecular-BEC state vanishes, and the coherent mixture of atomic and molecular BEC is subject to mechanical collapse.
In this paper, we study the phase diagram of a homogeneous Bose gas with a repulsive interaction near a wide Feshbach resonance at zero temperature. The Bose-Einstein-condensation (BEC) state of atoms is a metastable state. When the scattering length aaa exceeds a critical value depending on the atom density nnn, na3>0.035n{a}^{3}>0.035na3>0.035, the molecular excitation energy is imaginary and the atomic BEC state is dynamically unstable against molecule formation. The BEC state of diatomic molecules has lower energy, where the atomic excitation is gapped and the molecular excitation is gapless. However, when the scattering length is above another critical value, na3>0.0164n{a}^{3}>0.0164na3>0.0164, the molecular BEC state becomes an unstable coherent mixture of atoms and molecules. In both BEC states, the binding energy of diatomic molecules is reduced due to the many-body effect.
We study the steady state of a zero-temperature Bose gas near a Feshbach or photoassociation resonance using a two-channel mean-field model that incorporates atomic and molecular condensates, as well as correlated atom pairs originating from dissociation of molecules into pairs of atoms. We start from a many-body Hamiltonian for atom-molecule conversion, and derive the time-dependent version of the mean-field theory. The stationary solution of the time-dependent model is rendered unique with an approximation that entails that all noncondensate atoms are correlated, as if emerging from dissociation of molecules. The steady state is solved numerically, but limiting cases are also found analytically. The system has a phase transition in which the atomic condensate emerges in a nonanalytic fashion. We quantify the scaling of the observable quantities, such as fractions of atomic and molecular condensates, with the detuning and the atom-molecule conversion strength. Qualitatively, the dependence on detuning rounds out with increasing coupling strength. A study of the thermodynamics shows that the pressure of the atom-molecule system is negative, even on the molecule side of the resonance. This indicates the possibility of mechanical instability.
We explore the Bose condensed phases of an atomic gas on the molecular side of a Feshbach resonance. In the absence of atom-molecule and molecule-molecule scattering, we show that the atomic condensate is either a saddle point of the free energy with energy always exceeding that of the molecular condensate, or has a negative compressibility (hence unstable to density fluctuations). Therefore no phase transition occurs between the atomic and molecular condensates. We also show that a repulsive molecule-molecule scattering can stabilize a sufficiently dense atomic condensate, leading to the possibility of a phase transition. We caution that three-body processes may render this transition unobservable.
This article reviews recent advances in the theory of the three-dimensional dilute homogeneous Bose gas at zero and finite temperature. Effective-field-theory methods are used to formulate a systematic perturbative framework that can be used to calculate the properties of a system at T=0.T=0.T=0. The perturbative expansion of these properties is essentially an expansion in the gas parameter na3,\sqrt{{\mathrm{na}}^{3}},na3​, where aaa is the sss-wave scattering length and nnn is the number density. In particular, the leading quantum corrections to the ground-state energy density, the condensate depletion, and long-wavelength collective excitations are rederived in an efficient and economical manner. Nonuniversal effects are also discussed. These effects are higher-order corrections that depend on properties of the interatomic potential other than the scattering length, such as the effective range. The article critically examines various approaches to the dilute Bose gas in equilibrium at finite temperature. These include the Bogoliubov approximation, the Popov approximation, the Hartree-Fock-Bogoliubov approximation, the \ensuremath{\Phi}-derivable approach, optimized perturbation theory, and renormalization-group techniques. The article ends with a look at recent calculations of the critical temperature of the dilute Bose gas, which include 1/N1/N1/N techniques, lattice simulations, self-consistent calculations, and variational perturbation theory.